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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/91435完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 陳建彰 | zh_TW |
| dc.contributor.advisor | Jian-Zhang Chen | en |
| dc.contributor.author | 詹智麟 | zh_TW |
| dc.contributor.author | Chih-Lin Chan | en |
| dc.date.accessioned | 2024-01-26T16:29:36Z | - |
| dc.date.available | 2024-01-27 | - |
| dc.date.copyright | 2024-01-26 | - |
| dc.date.issued | 2024 | - |
| dc.date.submitted | 2024-01-15 | - |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/91435 | - |
| dc.description.abstract | 本研究透過低壓電漿對石墨紙表面進行塗覆催化劑層之前處理，並將塗覆催化劑之石墨紙應用於紙基流道式鋁空氣電池之陰極。在低壓電漿處理下，石墨紙表面產生物理及化學性變化，並對電化學性能有所影響。透過SEM、XPS及水接觸角，可觀察電漿處理前後石墨紙表面之形貌變化、表面元素及特定官能基含量之差異，以及表面親水性的不同；藉由LSV、CCD及EIS，可得知不同電漿參數下，組成鋁空氣電池後電化學性能之改變。整體而言，在10秒的低壓電漿處理下，鋁空氣電池將有最佳之電化學性能改善。 | zh_TW |
| dc.description.abstract | This study involves the pretreatment of the surface of graphite foil with low pressure plasma before coating a catalyst layer, and the application of the catalyst-coated graphite foil as the cathode in a paper-based fluidic aluminum air battery. Under low pressure plasma treatment, the surface of the graphite foil undergoes physical and chemical changes, affecting its electrochemical performance. The morphological changes, surface elemental differences, and variations in specific functional group content before and after plasma treatment can be observed through SEM, XPS, and water contact angle measurements. LSV, CCD, and EIS analyses reveal changes in the electrochemical performance of aluminum air batteries assembled under different plasma parameters. Overall, a 10 s low pressure plasma treatment yields the optimal improvement in electrochemical performance for the aluminum air battery. | en |
| dc.description.provenance | Submitted by admin ntu (admin@lib.ntu.edu.tw) on 2024-01-26T16:29:36Z No. of bitstreams: 0 | en |
| dc.description.provenance | Made available in DSpace on 2024-01-26T16:29:36Z (GMT). No. of bitstreams: 0 | en |
| dc.description.tableofcontents | 誌謝 i
摘要 ii ABSTRACT iii 目次 iv 表次 viii 圖次 ix 1 第一章 緒論 1 1.1 前言 1 1.2 研究動機 1 1.3 論文大綱 1 2 第二章 文獻探討 3 2.1 鋁空氣電池簡介 3 2.1.1 鋁空氣電池之介紹 3 2.1.2 鋁空氣電池之放電機制 4 2.1.3 鋁空氣電池之電極材料 6 2.1.4 鋁空氣電池之電解液 8 2.1.5 紙基流道式鋁空氣電池 10 2.1.6 可充電式鋁空氣電池 10 2.2 電漿技術簡介 10 2.2.1 電漿介紹 10 2.2.2 影響電漿的因素 14 2.3 低壓電漿之應用 21 2.3.1 低壓電漿應用於半導體製程 21 2.3.2 低壓電漿應用於材料之表面改質 24 3 第三章 實驗步驟與各項儀器 25 3.1 實驗材料 25 3.2 製程儀器 26 3.2.1 氮氣手套箱 26 3.2.2 低壓電漿系統 27 3.3 分析儀器 29 3.3.1 掃描式電子顯微鏡 (SEM) 29 3.3.2 X射線光電子能譜 (XPS) 30 3.3.3 接觸角儀 31 3.3.4 電化學工作站 32 3.4 實驗流程 34 3.4.1 石墨紙表面清潔 34 3.4.2 低壓電漿處理石墨紙 35 3.4.3 催化材料及附著劑之塗覆 35 3.4.4 KOH電解液之調配及流道之設計 35 3.4.5 PMMA基板清洗 36 3.4.6 紙基流道式鋁空氣電池之組裝 36 4 第四章 研究結果 37 4.1 石墨紙之掃描式電子顯微鏡分析 37 4.2 石墨紙之X光電子能譜分析 38 4.3 石墨紙之表面親水性分析 41 4.4 流道式鋁空氣電池之電化學表現 42 4.4.1 線性伏安法Linear sweep voltammetry (LSV) 42 4.4.2 定電流放電法Constant current discharge (CCD) 44 4.5 電化學阻抗頻譜分析 (EIS) 46 4.6 與先前以常壓介電層放電電漿改質石墨紙用於鋁空氣電池之研究之比較 48 4.7 流道式鋁空氣電池用於點亮LED燈之展示 49 5 第五章 結論與未來展望 51 6 第六章 附錄A－紙基流道式鋅空氣電池 52 6.1 研究動機與實驗流程 52 6.2 研究結果 53 6.2.1 低壓電漿處理前後之鋅空氣電池 53 6.2.2 使用不同濃度KOH及乙醇添加劑之鋅空氣電池 54 6.3 結論與未來展望 56 7 第七章 附錄B－PVA/KOH凝膠應用於鈕扣型鋁空氣電池 57 7.1 研究動機 57 7.2 文獻探討 57 7.2.1 固態電解質應用於金屬空氣電池 57 7.2.2 PVA/KOH電解質應用於鋁空氣電池 58 7.3 實驗步驟與各項材料 59 7.3.1 實驗材料 59 7.3.2 製程儀器 60 7.3.3 量測儀器 63 7.3.4 實驗流程 63 7.4 研究結果 66 7.4.1 PVA/KOH凝膠結合流道式鋁空氣電池 66 7.4.2 PVA/KOH與PVA/KOH@KOH凝膠電解質之離子電導率 67 7.4.3 PVA/KOH與PVA/KOH@KOH凝膠電解質組成之鈕扣型鋁空氣電池 68 7.5 結論與未來展望 70 參考文獻 71 8 個人期刊發表 90 | - |
| dc.language.iso | zh_TW | - |
| dc.title | 低壓電漿改質石墨紙用於紙基流道式鋁空氣電池以改善其電化學性能之研究 | zh_TW |
| dc.title | Low pressure plasma modified graphite foil as the cathode of paper-based fluidic Al-air battery for improved electrochemical performance | en |
| dc.type | Thesis | - |
| dc.date.schoolyear | 112-1 | - |
| dc.description.degree | 碩士 | - |
| dc.contributor.oralexamcommittee | 陳奕君;陳志鴻;徐振哲 | zh_TW |
| dc.contributor.oralexamcommittee | I-Chun Cheng;Chih-Hung Chen;Cheng-Che Hsu | en |
| dc.subject.keyword | 鋁空氣電池,低壓電漿,電化學性能, | zh_TW |
| dc.subject.keyword | aluminum air battery,low pressure plasma,electrochemical performance, | en |
| dc.relation.page | 91 | - |
| dc.identifier.doi | 10.6342/NTU202400016 | - |
| dc.rights.note | 同意授權(全球公開) | - |
| dc.date.accepted | 2024-01-16 | - |
| dc.contributor.author-college | 工學院 | - |
| dc.contributor.author-dept | 應用力學研究所 | - |
| 顯示於系所單位： | 應用力學研究所 | |
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