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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/86731完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 邱雅萍(Ya-Ping Chiu) | |
| dc.contributor.author | Yu-Shi Her | en |
| dc.contributor.author | 何昱熙 | zh_TW |
| dc.date.accessioned | 2023-03-20T00:14:06Z | - |
| dc.date.copyright | 2022-08-05 | |
| dc.date.issued | 2022 | |
| dc.date.submitted | 2022-07-29 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/86731 | - |
| dc.description.abstract | 太陽能電池這個研究課題的討論在近幾年的熱絡程度可見一斑，而作為太陽能電池表現性能的指標，能量轉換效率值(PCE)的突破是研究學者們一直以來所追求的目標。其中，有機–無機混態的鈣鈦礦材料在這項數值上展現了可觀的進步幅度，背後諸多的特殊物理性質也吸引了研究者的注意。甲基胺溴化鉛，作為混態鈣鈦礦材料的一員，具有的不僅僅是在作為太陽能電池材料上佔據優勢的光電特性，其本質上的強自旋軌道藕荷更讓它成為自旋電子學上的研究材料之一。 該材料的表面原子及電子結構正是這些特性與現象的關鍵成因，然而這其中依然有諸多揣想及未被證明的地方。我們透過剖面掃描穿隧式電子顯微鏡與能譜術，建立出甲基胺溴化鉛在表面照光之下的完整結電子結構。另外，從實驗結果分析來看，表面電子的能量與動量關係確實符合自旋軌道藕荷作用下的趨勢。 | zh_TW |
| dc.description.abstract | Solar cell has become prevailing these few years and achieving upmost power conversion efficiency (PCE) is the ultimate goal scientists seek for. Among tons of candidates, organic-inorganic hybrid perovskite (OIHP) shows its amazingly progressive pace in PCE, besides which there are also other unique characters of this material that attract researchers’ attention. MAPbBr3, as a member of the OIHP family, is not only a promising material in solar cell, but its intrinsic strong spin-orbit interaction also makes it interesting in spintronics application. It is its surface electronic characteristics that makes it such anticipated, but a more detailed insight is still blurred, and the actual mechanism is yet in argument. With the aid of Cross-section Scanning Tunneling Microscopy/Spectroscopy (XSTM/S), we reveal a complete scheme of the surface electronic structure of MAPbBr3 upon laser irradiation, and further demonstrate the considerable influence that spin-orbit interaction exerts on it. | en |
| dc.description.provenance | Made available in DSpace on 2023-03-20T00:14:06Z (GMT). No. of bitstreams: 1 U0001-2807202214213500.pdf: 7919962 bytes, checksum: e7188674db043397576d6f526c0f7a5c (MD5) Previous issue date: 2022 | en |
| dc.description.tableofcontents | 口試委員會審定書 # 誌謝 i 中文摘要 ii ABSTRACT iii CONTENTS iv LIST OF FIGURES vi Chapter 1 Introduction 1 Chapter 2 Theory 3 2.1 Scanning Tunneling Microscopy 3 2.1.1 Quantum tunneling effect 3 2.1.2 Bardeen’s method for single-electron transition rate 6 2.1.3 Total transition rate under Fermi’s Golden Rule 11 2.1.4 Matrix element approximation 14 2.2 Quasiparticle Interference 15 2.3 Rashba Effect 18 2.3.1 Spin-orbit coupling (SOC) 18 2.3.2 SOC combined with inversion asymmetry 19 2.3.3 Surface Rashba effect in perovskite material MAPbBr3 24 2.3.4 Permitted scattering channels of the two Rashba splitting cases 29 Chapter 3 Experimental Method 33 3.1 UHV Chamber and Cryostat for LT-STM 33 3.2 In-situ Cleavage 35 3.3 Scanning Tunneling Microscopy and Spectroscopy 36 3.3.1 Scanning Tunneling Microscopy (STM) 36 3.3.2 Scanning Tunneling Spectroscopy (STS) 38 Chapter 4 Results and Discussion 42 4.1 Structural and Electronic Properties of the MAPbBr3 Surface 42 4.1.1 Identification of the surface phase 42 4.1.2 Characteristic I-V curve of the MAPbBr3 surface from STS 48 4.2 Scanning Criteria for QPI Measurement on Rashba Splitting 55 4.2.1 Limitation on the scanning area and the bias voltage 55 4.2.2 Phase-boundary scattering off the massive hole-shaped breakage 60 4.3 In-depth Exploration of Surface Conduction Band via QPI over a Wide Range of Energy 67 4.3.1 Surface topography and FFT 67 4.3.2 Normalized differential conductance mapping and FFT 73 4.3.3 Voltage dependence of interference signals in reciprocal space 76 4.3.4 Evidence to SIA-based band splitting mechanism and Rashba effect from QPI characteristics 86 Chapter 5 Conclusion 101 Future Prospective 102 REFERENCE 103 | |
| dc.language.iso | zh-TW | |
| dc.subject | 自旋軌道藕荷 | zh_TW |
| dc.subject | 有機無機混態鈣鈦礦 | zh_TW |
| dc.subject | 剖面掃描穿隧顯微鏡與能譜 | zh_TW |
| dc.subject | 照光 | zh_TW |
| dc.subject | 表面電子結構 | zh_TW |
| dc.subject | 類粒子散射 | zh_TW |
| dc.subject | 拉什巴效應 | zh_TW |
| dc.subject | 有機無機混態鈣鈦礦 | zh_TW |
| dc.subject | 剖面掃描穿隧顯微鏡與能譜 | zh_TW |
| dc.subject | 照光 | zh_TW |
| dc.subject | 表面電子結構 | zh_TW |
| dc.subject | 自旋軌道藕荷 | zh_TW |
| dc.subject | 類粒子散射 | zh_TW |
| dc.subject | 拉什巴效應 | zh_TW |
| dc.subject | illumination | en |
| dc.subject | Cross-section Scanning Tunneling Microscopy/Spectroscopy | en |
| dc.subject | surface electronic structure | en |
| dc.subject | organic-inorganic hybrid perovskite | en |
| dc.subject | Rashba effect | en |
| dc.subject | quasi-particle scattering | en |
| dc.subject | spin-orbit coupling | en |
| dc.subject | organic-inorganic hybrid perovskite | en |
| dc.subject | Cross-section Scanning Tunneling Microscopy/Spectroscopy | en |
| dc.subject | illumination | en |
| dc.subject | surface electronic structure | en |
| dc.subject | spin-orbit coupling | en |
| dc.subject | quasi-particle scattering | en |
| dc.subject | Rashba effect | en |
| dc.title | 以掃描穿隧顯微術探討鈣鈦礦太陽能材料表面的拉什巴效應 | zh_TW |
| dc.title | Exploration of Surface Rashba Effect on Perovskite Single Crystal through Cross-sectional STM/S | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 110-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 張嘉升(Chia-Seng Chang),魏金明(Ching-Ming Wei) | |
| dc.subject.keyword | 有機無機混態鈣鈦礦,剖面掃描穿隧顯微鏡與能譜,照光,表面電子結構,自旋軌道藕荷,類粒子散射,拉什巴效應, | zh_TW |
| dc.subject.keyword | organic-inorganic hybrid perovskite,Cross-section Scanning Tunneling Microscopy/Spectroscopy,illumination,surface electronic structure,spin-orbit coupling,quasi-particle scattering,Rashba effect, | en |
| dc.relation.page | 118 | |
| dc.identifier.doi | 10.6342/NTU202201828 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2022-07-29 | |
| dc.contributor.author-college | 理學院 | zh_TW |
| dc.contributor.author-dept | 物理學研究所 | zh_TW |
| dc.date.embargo-lift | 2024-07-31 | - |
| 顯示於系所單位： | 物理學系 | |
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