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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/84748完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 楊志忠(Chih-Chung Yang) | |
| dc.contributor.author | Chen-Hua Chen | en |
| dc.contributor.author | 陳振華 | zh_TW |
| dc.date.accessioned | 2023-03-19T22:23:38Z | - |
| dc.date.copyright | 2022-09-06 | |
| dc.date.issued | 2022 | |
| dc.date.submitted | 2022-09-04 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/84748 | - |
| dc.description.abstract | 本研究中，我們首先探討在沒有量子井的多孔隙結構內綠光和紅光量子點的發射與福斯特共振能量轉換行為。在這部分研究中，我們觀察到奈米多孔隙結構內量子點的發射與福斯特共振能量轉換效率增強，證實了奈米級共振腔效應。接著，我們將奈米多孔隙結構製作在具有藍光量子井的樣品內，為了使紅光及綠光量子點靠近藍光量子井，我們將奈米多孔隙結構製作在藍光量子井附近。在這部分實驗，我們也可以透過奈米級共振腔效應得到從量子井到量子點福斯特共振能量轉換的增強效果。 我們還觀察到複雜的級聯福斯特共振能量轉換，福斯特共振能量轉換過程包括從量子井到綠光量子點、從量子井到紅光量子點以及從綠光量子點到紅光量子點的過程。在另一個實驗中，我們將銀奈米顆粒沉積在樣品表面上，以產生量子井和表面下孔隙內量子點之間的表面電漿子耦合。表面電漿子耦合可以進一步增強從量子井到量子點的福斯特共振能量轉換。整體而言，於本研究中，我們的結果證實奈米級共振腔效應可以增強多孔隙結構中的發射和福斯特共振能量轉換，同時也展示了從量子井到孔隙內量子點的福斯特共振能量轉換有增強的效果。此外，藉由表面電漿子耦合的效果可以進一步增強從量子井到量子點的福斯特共振能量轉換。 | zh_TW |
| dc.description.abstract | In this research, we first study the emission and Förster resonance energy transfer (FRET) behaviors of green-emitting quantum dot (GQD) and red-emitting QD (RQD) in porous structures without a quantum well (QW) structure. In this part of study, the enhancements of the emission efficiencies and FRET of QDs inside a porous structure are observed, confirming the nanoscale-cavity effect. Then, we fabricate a porous structure near a blue-emitting QW structure in a QW template for accommodating GQD and RQD. Here, enhanced FRET processes from QW into QD can be observed also through the nanoscale-cavity effect. We also observe the complicated cascading FRET behavior, i.e., the FRET system includes the processes from QW into GQD, from QW into RQD, and from GQD into RQD. Next, surface Ag NPs are deposited onto the sample surface to induce surface plasmon (SP) couplings with the embedded QWs and subsurface QDs. The SP coupling can further enhance the FRET from QWs into QDs. The observations in this study support the nanoscale-cavity effect for enhancing the emission and FRET in a porous structure. They also demonstrate the enhanced FRET from a nearby QW into an inserted QD. Meanwhile, SP coupling can further enhance the FRET from the QW into QD. | en |
| dc.description.provenance | Made available in DSpace on 2023-03-19T22:23:38Z (GMT). No. of bitstreams: 1 U0001-0109202216533000.pdf: 10054720 bytes, checksum: 8a896a8956748e05950b1e02c7b5c1a5 (MD5) Previous issue date: 2022 | en |
| dc.description.tableofcontents | 口試委員會審定書 i 誌謝 ii 摘要 iii Abstract iv Contents v List of Figure vii List of Table xxiii Chapter 1 Introduction 1 1.1 Surface plasmon coupling and Förster resonance energy transfer for color conversion 1 1.2 Subsurface GaN porous structures 2 1.3 Results of an earlier study 3 1.4 Research motivations 7 1.5 Thesis structure 8 Chapter 2 Sample Structures and Fabrication Procedures 14 2.1 Epitaxial samples for porous structure fabrication 14 2.2 Fabrication of a porous structure and insertion of quantum dots into pores 14 2.3 Sample structures and fabrication procedures 17 2.4 Optical characterization methods 18 Chapter 3 Emission and Förster Resonance Energy Transfer of Quantum Dots Inserted into a Subsurface Nano-porous Structure in a GaN Template 28 3.1 General sample descriptions 28 3.2 Time-resolved photoluminescence results 29 3.3 Continuous photoluminescence results 32 Chapter 4 Emission and Förster Resonance Energy Transfer of Quantum Dots Inserted into a Subsurface Nano-porous Structure in a Quantum-well Template 60 4.1 General sample descriptions 60 4.2 Time-resolved photoluminescence results 61 4.3 Continuous photoluminescence results 65 Chapter 5 Emission and Förster Resonance Energy Transfer of Quantum Dots Inserted into a Subsurface Nano-porous Structure in a Quantum-well Template under the Surface Plasmon Coupling of Surface Ag Nanoparticles 99 5.1 General sample descriptions 99 5.2 Time-resolved photoluminescence results 102 5.3 Continuous photoluminescence results 105 Chapter 6 Discussions 139 Chapter 7 Conclusions 141 References 142 | |
| dc.language.iso | en | |
| dc.subject | 福斯特共振能量轉換 | zh_TW |
| dc.subject | 量子點 | zh_TW |
| dc.subject | 表面電漿子耦合 | zh_TW |
| dc.subject | 量子井 | zh_TW |
| dc.subject | 奈米級共振腔效應 | zh_TW |
| dc.subject | Quantum well | en |
| dc.subject | quantum dot | en |
| dc.subject | Förster resonance energy transfer | en |
| dc.subject | surface plasmon coupling | en |
| dc.subject | nanoscale-cavity effect | en |
| dc.title | 塞入量子井結構表面下側向延伸孔洞內部膠體量子點的發光、福斯特共振能量轉換與表面電漿子耦合行為 | zh_TW |
| dc.title | Emission, Förster Resonance Energy Transfer and Surface Plasmon Coupling Behaviors of Colloidal Quantum Dots Inserted into Subsurface Laterally-extended Pores in a Quantum-well Structure | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 110-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 黃建璋(Jian-Jang Huang),陳奕君(I-Chun Cheng),林建中(Chien-Chung Lin),郭仰(Yang Kuo) | |
| dc.subject.keyword | 量子點,福斯特共振能量轉換,表面電漿子耦合,奈米級共振腔效應,量子井, | zh_TW |
| dc.subject.keyword | quantum dot,Förster resonance energy transfer,surface plasmon coupling,nanoscale-cavity effect,Quantum well, | en |
| dc.relation.page | 145 | |
| dc.identifier.doi | 10.6342/NTU202203073 | |
| dc.rights.note | 同意授權(限校園內公開) | |
| dc.date.accepted | 2022-09-05 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| dc.date.embargo-lift | 2022-09-06 | - |
| 顯示於系所單位： | 光電工程學研究所 | |
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