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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/80455完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 黃慶怡(Ching-I Huang) | |
| dc.contributor.author | YA-JUAN PENG | en |
| dc.contributor.author | 彭雅絹 | zh_TW |
| dc.date.accessioned | 2022-11-24T03:07:00Z | - |
| dc.date.available | 2026-12-03 | |
| dc.date.available | 2022-11-24T03:07:00Z | - |
| dc.date.copyright | 2022-01-17 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-12-06 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/80455 | - |
| dc.description.abstract | "本研究探討在高效率PM6:Y6系統中加入不同共軛聚合物供體材料J51、FTAZ和PTO2形成供體/供體/受體系統的三元太陽能電池，我們使用紫外-可見光光譜儀(Ultraviolet–visible spectroscopy, UV-Vis)、光致發光光譜儀(Photoluminescence, PL)、原子力顯微鏡(Atomic Force Microscope, AFM)和低掠角廣角X射線散射(Grazing-Incidence Wide-Angle X-ray Scattering, GIWAXS)來分析材料之間的混溶性對三元共混薄膜的光電和型態特性的影響。其中，第三元材料J51、FTAZ和PTO2都展現出與PM6具有良好相溶性，並出現在富含PM6的區域中。值得注意的是，χJ51/Y6(1.79 K)和χJ51/PM6(0.34 K)之間較大的差異增強了Y6的分子堆積，然而，J51分子構型容易產生空間位阻而限制供體相內的電荷轉移和收集，從而導致光伏性能下降。當加入FTAZ時，則同樣觀察到Y6的分子堆疊強度增強(χY6/FTAZ=1.24 K)，並因為具有較低的χFTAZ/PM6(0.13 K)使FTAZ/PM6形成良好混和的供體相，因此有效提升供體材料的HOMO能階使三元元件之VOC增加，並促進電荷傳遞和收集從而增強FF，進而提升能量轉換效率(power conversion efficiency, PCE)從14.3%(二元)提高至15.3%(三元)。在這三種測試的第三元聚合物供體中，PTO2展現出與PM6的最高混溶性大大增強了供體相有序的堆疊型態，並具有比PM6更深的HOMO能階有效提升VOC，因此，元件的PCE從14.8%(二元)提升至15.6%(三元)。最後，我們還研究了1-chloronaphthalene(CN)作為溶劑添加劑時，對PM6:PTO2:Y6和PM6:PTO2:BTP-eC9三元混摻系統的影響，證實少量的CN可以有效優化共混形態並實現元件的長期穩定性，獲得最高PCE為17.05和18.01%的優異表現。因此，通過我們對供體/供體/受體三元系統中的混合形態和光伏性能的一系列研究，期望我們的結果可以提供未來研究學者們設計穩定的高性能三元太陽能電池提供了有效的策略。" | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-24T03:07:00Z (GMT). No. of bitstreams: 1 U0001-0312202111272900.pdf: 5210220 bytes, checksum: a06c1b6f60b190a6d752b1c3175f9567 (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | 致謝 i 摘要 ii ABSTRACT iii 目錄 v 圖目錄 vi 表目錄 xi 第一章 前言 1 第二章 實驗設計 10 2.1 實驗藥品 12 2.1.1主動層材料 12 2.1.2傳輸層材料和使用溶劑 14 2.1.3製程設備及檢測儀器 15 2.2 高分子太陽能電池元件製備步驟 16 2.3 光學性質分析 19 2.4 光電性質分析 20 2.5 表面性質分析與內部共混型態 25 第三章 結果討論 29 3.1 添加聚合物供體J51和FTAZ於PM6:Y6二元系統 29 3.2 添加聚合物供體PTO2於PM6:Y6和PM6:BTPeC9二元系統 47 3.3 第三元供體材料對元件性能的影響 70 第四章 結論 74 參考文獻 76 | |
| dc.language.iso | zh-TW | |
| dc.subject | 能量轉換效率 | zh_TW |
| dc.subject | 三元太陽能電池 | zh_TW |
| dc.subject | 共軛聚合物 | zh_TW |
| dc.subject | 混溶性 | zh_TW |
| dc.subject | ternary organic photovoltaics | en |
| dc.subject | miscibility | en |
| dc.subject | conjugated polymer | en |
| dc.title | 共軛聚合物混溶性於高效三元有機太陽能電池光伏性能和堆疊型態的影響 | zh_TW |
| dc.title | Effects of the Miscibility of Conjugated Polymer Donors on Photovoltaic Performance and Stacking Type of Highly Efficiencnt Ternary Organic Solar Cells | en |
| dc.date.schoolyear | 110-1 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 陳志平(Hsin-Tsai Liu),王立義(Chih-Yang Tseng) | |
| dc.subject.keyword | 三元太陽能電池,共軛聚合物,混溶性,能量轉換效率, | zh_TW |
| dc.subject.keyword | ternary organic photovoltaics,conjugated polymer,miscibility, | en |
| dc.relation.page | 81 | |
| dc.identifier.doi | 10.6342/NTU202104508 | |
| dc.rights.note | 同意授權(限校園內公開) | |
| dc.date.accepted | 2021-12-06 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 高分子科學與工程學研究所 | zh_TW |
| dc.date.embargo-lift | 2026-12-03 | - |
| 顯示於系所單位： | 高分子科學與工程學研究所 | |
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