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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79858完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 王尚禮(Shan-Li Wang) | |
| dc.contributor.author | Emily Karen Kin | en |
| dc.contributor.author | 金琬芹 | zh_TW |
| dc.date.accessioned | 2022-11-23T09:14:09Z | - |
| dc.date.available | 2023-08-01 | |
| dc.date.available | 2022-11-23T09:14:09Z | - |
| dc.date.copyright | 2021-08-06 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-08-03 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79858 | - |
| dc.description.abstract | 近年由農業廢棄物所製造的生物炭被施佈於土壤作為土壤改良劑，但其對於不同質地的土壤的養分移動的機制及效益卻尚未被充分了解。由於文獻中生物炭對於土壤中磷(P)的吸附和遷移能力的作用呈現出正反的結果，因此本研究之目的為探討生物炭對於酸性土壤中磷的滯留和移動的影響。生物炭是由稻殼分別在350 和 600 °C 且限制氧氣條件下加熱處理2 小時獲得的，並指定為 BC350 和 BC600。將以上兩種生物炭以 5% 的施用率添加到兩種質地不同的酸性土壤中， Tn（砂壤土）和 Pc（粘土）土壤，構成六個實驗組，Tn (對照組)、Tn+5%BC350 (Tn350)、Tn+5%BC600 (Tn600)、Pc (對照組)、Pc+5%BC350 (Pc350) 和 Pc+5%BC600 (Pc600) ，分別進行了批次吸附與管柱淋洗實驗。吸附參數是通過將吸附數據擬合到 Langmuir 和 Freundlich等溫吸附曲線所獲得的；而滯留及傳輸相關參數則是使用 CXTFIT-Studio of Analytical MODels (STANMOD)從管柱淋洗實驗數據中所獲得的。使用吸附實驗推導出的滯留係數作為預測 P-breakthrough curve (BTC) 的模型參數會高估滯留程度，而低估添加生物炭的土壤中 P 的遷移性。管柱實驗可觀察到，在黏質土壤中的磷阻滯性強，而在砂質土壤中磷阻滯較弱。使用two-site非平衡模型可以充分地描述 P 貫穿曲線的不對稱和延遲，而結果顯示，除了 Tn600 外，將生物炭施用於 Tn 和 Pc 土壤中磷的滯保性和吸附能力皆總體下降。這些發現可以讓我們更深入了解 P 是如何保留在土壤中的，以及生物炭的適當管理以保護水質免受 P 汙染和最有效地增加土壤肥力。 | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-23T09:14:09Z (GMT). No. of bitstreams: 1 U0001-0308202100045200.pdf: 3392402 bytes, checksum: 3b4c4a80e34ff51cfce6a7c605ede964 (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | "口試委員會審定書 (APPROVAL PAGE) I 誌謝 (ACKNOWLEDGEMENTS) II 摘要 III ABSTRACT IV TABLE OF CONTENTS VI LIST OF FIGURES X LIST OF TABLES XII CHAPTER 1. INTRODUCTION 1 CHAPTER 2. LITERATURE REVIEW 4 2.1 PHOSPHORUS 4 2.1.1 Importance of phosphorus 4 2.1.2 Use of rice biowaste as alternate source of phosphorous 11 2.2 CHARACTERISTICS OF BIOCHAR 12 2.2.1 Rice husk biochar 13 2.2.2 Effects of pyrolysis temperature on biochar 15 2.2.3 Phosphorous adsorption to biochar 21 2.2.4 Interactive effects of biochar on P in soils 23 2.3 STUDY OF ADSORPTION ISOTHERM 27 2.4 STUDY OF BREAKTHROUGH MODELING 27 CHAPTER 3. MATERIAL AND METHODS 30 3.1 MATERIAL PREPARATION 30 3.1.1 Soil collection: 30 3.1.2 Biochar preparation 30 3.2 PROPERTY ANALYSIS OF SOIL AND BIOCHAR 31 3.2.1 Soil and biochar pseudo-total analysis 31 3.2.2 Analysis of soil property 33 3.2.2.1 Soil organic matter 36 3.2.2.2 Soil CEC and exchangeable K, Ca, and Mg 37 3.2.3 Analysis of biochar property 38 3.2.3.1 Zeta potential of biochar 40 3.2.3.2 FTIR analysis of biochar 40 3.2.4 Soil and biochar particle density 41 3.2.5 Soil and biochar mass water content 42 3.3 EXPERIMENTAL DESIGN 42 3.3.1 Batch experiments 42 3.3.2 Leaching Column Experimental Design 47 3.3.2.1 Leaching Column Porosity 50 3.3.2.2 Chemical analysis 50 3.4 TRANSPORT MODEL 51 3.4.1 Breakthrough modeling 53 3.4.2 Initial and flux boundary conditions 55 3.4.3 Estimation of transport and sorption parameters 56 3.4.4 STANMODE-CXTFIT 57 3.5 EVALUATION OF MODEL PERFORMANCE 60 CHAPTER 4. RESULTS AND DISCUSSION 61 4.1 SOIL PROPERTIES 61 4.2 BIOCHAR PROPERTIES 65 4.2.1 Elemental compositions 65 4.2.2 Surface charge properties of BC350 and BC600 70 4.2.3 Characterization of biochar by FTIR 72 4.3 BATCH EXPERIMENTS 75 4.4 LEACHING COLUMN EXPERIMENTS 81 4.4.1 CHEMICAL ANALYSIS ON LEACHING SAMPLES 91 CHAPTER 5. CONCLUSIONS 98 REFERENCES 100 " | |
| dc.language.iso | en | |
| dc.subject | 磷移動 | zh_TW |
| dc.subject | 磷吸附 | zh_TW |
| dc.subject | 生物炭 | zh_TW |
| dc.subject | 酸性土壤 | zh_TW |
| dc.subject | CXTFIT 模型 | zh_TW |
| dc.subject | 貫穿曲線 | zh_TW |
| dc.subject | breakthrough curve | en |
| dc.subject | phosphorus mobility | en |
| dc.subject | phosphorus sorption | en |
| dc.subject | biochar | en |
| dc.subject | CXTFIT | en |
| dc.subject | acidic soil | en |
| dc.title | 在酸性土壤中添加稻殼生物炭對於磷吸附與移動之影響 | zh_TW |
| dc.title | The Effects of Rice Husk-Derived Biochar on Phosphorus Sorption and Mobility in Acidic Soils | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 李達源(Hsin-Tsai Liu),許正一(Chih-Yang Tseng),鄒裕民,簡士濠 | |
| dc.subject.keyword | CXTFIT 模型,貫穿曲線,酸性土壤,生物炭,磷吸附,磷移動, | zh_TW |
| dc.subject.keyword | CXTFIT,breakthrough curve,acidic soil,biochar,phosphorus sorption,phosphorus mobility, | en |
| dc.relation.page | 121 | |
| dc.identifier.doi | 10.6342/NTU202102020 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2021-08-04 | |
| dc.contributor.author-college | 生物資源暨農學院 | zh_TW |
| dc.contributor.author-dept | 農業化學研究所 | zh_TW |
| dc.date.embargo-lift | 2023-08-01 | - |
| 顯示於系所單位： | 農業化學系 | |
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