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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79844完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 鄭如忠(Ru-Jong Jeng) | |
| dc.contributor.author | Bing-Huang Jiang | en |
| dc.contributor.author | 江炳煌 | zh_TW |
| dc.date.accessioned | 2022-11-23T09:13:35Z | - |
| dc.date.available | 2021-08-11 | |
| dc.date.available | 2022-11-23T09:13:35Z | - |
| dc.date.copyright | 2021-08-11 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-08-06 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79844 | - |
| dc.description.abstract | 本研究旨在探討影響高性能PM6:Y6主動層共混形態之因素，我們總結了主要影響主動層共混形態之因素，並針對尚未被充分研究的部分著手，所以選擇了探討傳輸層表面特性與固體添加劑對於PM6:Y6主動層共混形態之影響。首先，我們選用PEDOT:PSS、氧化鎳(NiOx)、溶膠凝膠法所製備的氧化鋅(ZnO(sol-gel))與奈米顆粒型的氧化鋅(ZnO(NP))來做為PM6:Y6衍生有機太陽能電池的傳輸層。這些傳輸層表面具有不一樣的表面能、表面形態與表面粗糙度，將會影響PM6:Y6主動層的沉積，進而產生不一樣的共混形態。因此我們也近一步藉由原子力顯微鏡與低略角繞射技術來瞭解PM6:Y6共混形態上的變化。並在其中觀察到傳輸層誘導效果會隨主動層溶劑不同而有所差異。接著將不同共混形態的PM6:Y6主動層製備成有機光伏元件，並探討共混形態與元件性能之間的關係。其中PEDOT:PSS上chlorobenzene (CB)所製備的主動層展現出大的相域與高的結晶性，使得對應元件展現11.5 %的PCE。ZnO(sol-gel)上的CB衍生元件則展現截然不同的共混形態，但獲得與PEDOT:PSS衍生元件類似的PCE。導入1-chloronaphthalene (CN)添加劑後，共混形態被近一步的改善，進而使元件PCE超過13 %。同時不封裝的ZnO(sol-gel)衍生元件在環境穩定中展現良好的表現。此外，我們評估了不同共混形態的PM6:Y6主動層在室內光下的元件性質表現，其中在ZnO上chloroform (CF)所製備的元件在室內光伏元件的測試中展現出十足的潛力。最後我們也總結了固體添加劑對於PM6:Y6共混形態與元件性能的影響，並總結出高性能固體添加劑須具備的特性。 | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-23T09:13:35Z (GMT). No. of bitstreams: 1 U0001-0408202110124500.pdf: 11233670 bytes, checksum: 9f3563a398f420c632b59081a5152444 (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | 論文口試委員審定書 i 序言 iii 中文摘要 iv Abstract v 目錄 vii 圖目錄 ix 表目錄 xii 第一章 緒論 1 1-1 前言 1 1-1-1 有機光電材料之特性 4 1-2 有機光伏元件 6 1-2-1 有機光伏元件之工作原理 6 1-2-2 有機光伏元件之元件結構 8 1-2-3 有機光伏元件之主動層材料 11 1-2-4 有機太陽能電池 13 1-2-5 室內光有機太陽能電池 24 1-3 主動層共混形態 30 1-3-1 主動層共混形態的生成 31 1-3-2 控制主動層共混形態的方法 34 1-4 研究動機 41 第二章 PM6/Y6混摻形態對於有機光伏元件性能之影響探討 42 2-1 材料特性 42 2-2 實驗設計 44 2-3 結果與討論 45 2-3-1 傳輸層的表面特性 45 2-3-2 傳輸層對於主動層共混形態之影響 48 2-3-3 不同溶劑或添加劑對於傳輸層誘導主動層形態之影響 54 2-3-4 不同共混形態對於有機太陽能電池性能之影響 62 2-3-5 不同共混形態對於室內光有機太陽能電池性能之影響 69 2-3-6 固體添加劑對於主動層共混形態與元件性能之影響 73 第三章 結論 76 第四章 未來展望 77 第五章 實驗細節 78 4-1 使用藥品與溶劑 78 4-2 使用儀器 79 4-3 元件製程 81 參考文獻 83 作者介紹 95 發表著作 96 | |
| dc.language.iso | zh-TW | |
| dc.subject | 能量轉換效率 | zh_TW |
| dc.subject | 有機太陽能電池 | zh_TW |
| dc.subject | 共軛高分子 | zh_TW |
| dc.subject | 非富勒烯 | zh_TW |
| dc.subject | power conversion efficiency | en |
| dc.subject | organic photovoltaic | en |
| dc.subject | conjugated polymer | en |
| dc.subject | non-fullerene | en |
| dc.title | PM6/Y6混摻形態對於有機光伏元件性能之影響探討 | zh_TW |
| dc.title | Investigate the effect of PM6/Y6 blend morphology on the performance of organic photovoltaics | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 博士 | |
| dc.contributor.coadvisor | 陳志平(Chih-Ping Chen) | |
| dc.contributor.oralexamcommittee | 汪根欉(Hsin-Tsai Liu),闕居振(Chih-Yang Tseng),賴育英 | |
| dc.subject.keyword | 有機太陽能電池,共軛高分子,非富勒烯,能量轉換效率, | zh_TW |
| dc.subject.keyword | organic photovoltaic,conjugated polymer,non-fullerene,power conversion efficiency, | en |
| dc.relation.page | 97 | |
| dc.identifier.doi | 10.6342/NTU202102065 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2021-08-09 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 高分子科學與工程學研究所 | zh_TW |
| 顯示於系所單位： | 高分子科學與工程學研究所 | |
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