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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 李克強(Eric Lee) | |
| dc.contributor.author | Fang-Yi Wu | en |
| dc.contributor.author | 吳芳儀 | zh_TW |
| dc.contributor.author | f05423001 | |
| dc.date.accessioned | 2022-11-23T09:06:57Z | - |
| dc.date.available | 2021-09-11 | |
| dc.date.available | 2022-11-23T09:06:57Z | - |
| dc.date.copyright | 2021-09-11 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-09-01 | |
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Wuzhang, J., et al., Electrophoretic mobility of oil droplets in electrolyte and surfactant solutions. Electrophoresis, 2015. 36(19): p. 2489-2497. | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79668 | - |
| dc.description.abstract | 本研究以位於電解質溶液中的帶電介電液滴為主體，探討兩項重要的電動力學現象：電泳與擴散泳。液滴模型可模擬為真實物理系統的微乳液、奈米乳液、微脂體與胞外體等。而分別以外加電場與外加濃度場作為驅動力的電泳和擴散泳，從首次被提出以來，一直在各領域有著卓越且進步的發展。從民生工業的食品、化妝品到重工業的煉油、膜過濾、沉積，乃至於生技產業的製藥、生化、醫材等領域都有著舉足輕重的地位，是可以全方面應用的技術。 本研究採用假性光譜法中的正交配位法來做數值處理。透過空間映射、多區聯解、擾動法、子問題法等手法，搭配系統相對應的電動力學方程組和邊界條件來求解介電液滴之泳動度。探討電解質溶液和介電液滴的各項物理參數，包含電雙層厚度、介電液滴內外黏度比、表面帶電量、粒子大小等，對於泳動度的影響。 第一部分為電泳，本研究發現一有趣的現象，在不同的電雙層厚度區間，時而出現氣泡跑得較固體硬球快的情形；時而出現固體硬球跑得較氣泡快的情形。這可以歸因於液滴額外切線電驅動力與電滲流之交互作用，致使其相應而生的內外部渦流。並且可以發現一不論介電液滴內外黏度比為多少，泳動度不隨電雙層厚度改變而改變的臨界點。 第二部分為擴散泳，本研究發現擴散泳中的電泳效應和化學泳效應處於互相競爭的狀態，且兩者的數量級相當。此外，當電解質溶液陰陽離子擴散係數不相等時，可能會出現負的泳動度，在實務應用上須特別小心。 本研究對介電液滴之電泳與擴散泳現象提供了深入的分析與探討，可作為其實際應用之基礎。 | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-23T09:06:57Z (GMT). No. of bitstreams: 1 U0001-3108202115254000.pdf: 4802399 bytes, checksum: 5e1391e7d95375eb3e45de275fba36c0 (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | 誌謝 I 中文摘要 III 英文摘要 V 目錄 VII 圖目錄 IX 表目錄 XII 第一章 緒論 1 1-1 研究目的與論文架構 1 1-2 液滴系統介紹 2 1-3 以液滴模型模擬之物理系統介紹 3 1-4 如何使膠體粒子表面帶電 10 1-5 介電液滴與導電液滴之性質 11 1-6 液滴的變形 13 1-7 電泳概論 14 1-8 擴散泳概論 24 第二章 數值方法 33 2-1 計算流程 33 2-2 假性光譜法（正交配位法） 34 2-3 空間映射 40 2-4 多區聯解之補綴式假性光譜法 41 2-5 牛頓-拉福森疊代法 44 2-6 擾動態多變數聯解 47 2-7 數值積分 49 第三章 結果與討論-介電液滴之電泳現象探討 51 3-1 系統描述 51 3-2 理論分析 53 3-3 表面帶電量選擇 67 3-4 程式比對 68 3-5 液滴表面附近之渦流與電泳動度之關係：與硬球比較 71 3-6 內外黏度比 (σ_H) 對電泳動度之影響 74 3-7 表面電位 (ϕr) 對電泳動度之影響 76 3-8 電雙層厚度 (κa) 對電泳動度之影響 78 3-9 結論 86 第四章 結果與討論-介電液滴之擴散泳現象探討 87 4-1 系統描述 87 4-2 理論分析 89 4-3 程式比對 103 4-4 擴散泳的化學泳效應 106 4-5 擴散泳的電泳效應 113 4-6 結論 120 第五章 總結 121 附錄 122 參考文獻 125 | |
| dc.language.iso | zh-TW | |
| dc.title | 介電液滴之泳動行為：電泳與擴散泳 | zh_TW |
| dc.title | Phoretic Motions of a Dielectric Droplet: Electrophoresis and Diffusiophoresis | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 博士 | |
| dc.contributor.oralexamcommittee | 游佳欣(Hsin-Tsai Liu),陳賢燁(Chih-Yang Tseng),唐于博,朱智瑋 | |
| dc.subject.keyword | 介電液滴,泳動行為,電泳,擴散泳,電動力學現象,藥物輸送,電雙層極化效應,自旋運動,渦流, | zh_TW |
| dc.subject.keyword | Dielectric Droplet,Drug Delivery,Diffusiophoresis,Electrokinetic Phenomena,Electrophoresis,Electrical Double Layer Polarization,Phoretic Motions,Spinning Motion,Vortex Flow, | en |
| dc.relation.page | 134 | |
| dc.identifier.doi | 10.6342/NTU202102907 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2021-09-02 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
| 顯示於系所單位： | 化學工程學系 | |
文件中的檔案：
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| U0001-3108202115254000.pdf | 4.69 MB | Adobe PDF | 檢視/開啟 |
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