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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 李君浩(Jiun-Haw Lee) | |
| dc.contributor.author | Jhih-Hao Lin | en |
| dc.contributor.author | 林志豪 | zh_TW |
| dc.date.accessioned | 2021-06-17T06:04:52Z | - |
| dc.date.available | 2019-01-30 | |
| dc.date.copyright | 2019-01-30 | |
| dc.date.issued | 2019 | |
| dc.date.submitted | 2019-01-21 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/71624 | - |
| dc.description.abstract | 本論文有三個主題，第一部分為小分子太陽能元件之研究，第二部分為三重態-三重態-湮滅藍色有機發光二極體，第三部分為有機發光二極體光萃取之研究。
第三章中，我們利用結構為施體-受體-受體型小分子電子施體材料和碳70電子受體材料作為太陽能元件之主動層於塊材異質混和界面架構下，藉由主動層濃度及厚度的變化，進行四個小分子材料7-(4-(di-p-tolylamino)phenyl)-6-fluorobenzo[c][1,2,5]thiadiazole-4,5-dicarbonitrile (DTCPiFBTCN), 7-(4-(di-p-tolylamino)phenyl)benzo[c][1,2,5]thiadiazole-4,5-dicarbonitrile (DTCPBTCN2), 7-(4-(di-p-tolylamino)phenyl)benzo[c][1,2,5]thiadiazole-4,5,6-tricarbonitrile (DTCPBTCN¬3) 及7-(5-(di-p-tolylamino)thiophen-2-yl)benzo[c][1,2,5]thiadiazole-4,5,6-tricarbonitrile (DTCTBTCN3¬) 的比較，DTCPBTCN2作為電子受體之太陽能元件有著最佳功率轉化為5.41%，其開路電壓、短路電流密度和填充因子分別為0.89 V、10.81 mA /cm2 及56.26%。 在第四章中，我們使用兩個新的蒽核衍生物材料1-phenyl-2-(10-phenylanthracen-9-yl)-1H-benzo[d]imidazole (monoBizAn) 及 4,4,5,5-tetramethyl-2-(10-(naphthalene-2-yl)-1,3,2-dioxaborolane (NpBorAn) 作為三重態-三重態-湮滅藍色有機發光二極體之發光體，以純膜及客體材料高濃度混入9,9'-(2-(1-Phenyl-1H-benzo[d]imidazol-2-yl)-1,3-phenylene)bis(9H-carbazole) (o-DiCbzBz) 製作藍色有機發光二極體，元件以monoBizAn作為客體材料濃度60%混入o-DiCbzBz中有著最佳元件表現，在電流效率、功率效率及外部量子效率方面達到5.74 cd /A、4.71 lm/W 和5.56%。 在第五章中，使用三種不同週期的光柵 (833.33, 416.67, 277.78奈米)來製作藍色磷光有機發光二極體元件，藉由氧化銦鋅進行氧電漿時間、陽極厚度及元件電洞傳輸層厚度之優化，週期為416.67奈米的光柵作為內部結構且搭配半球透鏡作外部結構製作元件，最高可以得到52.51%的外部量子效率以及82.52%的外部量子效率提升，並且利用偏振片的量測進行表面電漿態與波導模態的光萃取分析。 | zh_TW |
| dc.description.abstract | There are three parts in this thesis. First, we study on the small molecule solar cell. Second, we do the research about the triplet-triplet annihilation blue organic light-emitting diode. Last, we discuss light extraction through nanostructure in organic light-emitting diode.
In chapter 3, we compared four electron donor-acceptor-acceptor (D-A-A) type electron donor materials, 7-(4-(di-p-tolylamino)phenyl)-6-fluorobenzo[c][1,2,5]thiadiazole-4,5-dicarbonitrile (DTCPiFBTCN), 7-(4-(di-p-tolylamino)phenyl)benzo[c][1,2,5]thiadiazole-4,5-dicarbonitrile (DTCPBTCN2), 7-(4-(di-p-tolylamino)phenyl)benzo[c][1,2,5]thiadiazole-4,5,6-tricarbonitrile (DTCPBTCN¬3) and 7-(5-(di-p-tolylamino)thiophen-2-yl)benzo[c][1,2,5]thiadiazole-4,5,6-tricarbonitrile (DTCTBTCN3¬)¬, with fullerene-based material C70 as the electron acceptor material in the active layer of small organic solar cells (SMOSCs) with bulk-heterojunction (BHJ) configuration. Among these D-A-A materials, DTCPBTCN2 as electron donor material with C70 as the electron acceptor material at the mixing ratio D:A=1:1.4 and 60 nm of active layer showed the highest power conversion efficiency of 5.41%, with open circuit voltage (Voc), short circuit current density (J¬sc) and fill factor (FF) of 0.89 V, 10.81 mA/cm2, and 56.26%, respectively. In chapter 4, we employed two new anthracene-core derivatives, 1-phenyl-2-(10-phenylanthracen-9-yl)-1H-benzo[d]imidazole (monoBizAn) and 4,4,5,5-tetramethyl-2-(10-(naphthalene-2-yl)-1,3,2-dioxaborolane (NpBorAn) as the blue triplet-triplet annihilation (TTA) emitters in the OLEDs with non-doped configuration and high doping concentrations in the host, 9,9'-(2-(1-Phenyl-1H-benzo[d]imidazol-2-yl)-1,3-phenylene)bis(9H-carbazole) (o-DiCbzBz). Device efficiency of TTA OLED with monoBizAn doped in o-DiCbzBz at 60% concentration showed the highest efficiency which achieved 5.74 cd/A, 4.71 lm/W and 5.56% in terms of current efficiency, power efficiency and EQE, respectively. In chapter 5, we studied the light extraction of blue phosphorescent organic light emitting diodes (PHOLEDs) with nanostructure (pitch = 833.33, 416.67, and 277.78 nm) between the substrate and the indium-zinc-oxide (IZO) anode. After optimizing plasma time、thickness of IZO and thickness of hole transport layer (HTL), blue PHOLED with nanostructure and macrolens can reach EQE value of 52.52% and enhancement ratio of 82.52%. Besides, we separate surface plasmon (SP) mode and waveguide mode to understand light extraction mechanism. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-17T06:04:52Z (GMT). No. of bitstreams: 1 ntu-108-R04941085-1.pdf: 9061159 bytes, checksum: 697cf082521e85cb27d158f4253e2faf (MD5) Previous issue date: 2019 | en |
| dc.description.tableofcontents | 摘要 i
Abstract iii Content vi Figure content viii Table content xiv Chapter 1 Introduction 1 1.1 Overview 1 1.2 Organic solar cell (OSC) 1 1.2.1 Introduction of working principle of OSC 1 1.2.2 Fluorine atoms and cyano-substitution on the polymer and small molecules OSCs 4 1.2.3 Asymmetric configuration of SMOSCs 7 1.2.4 Motivation 11 1.3 Organic light-emitting diodes (OLEDs) 11 1.3.1 Operation principle of OLEDs 11 1.3.2 Emission mechanisms of OLEDs 12 1.3.3 Blue TTA OLEDs 13 1.3.4 Motivation 18 1.4 Light extraction 19 1.4.1 Introduction of light extraction in OLEDs 19 1.4.2 High efficiency blue OLEDs 20 1.4.3 Highly efficiency OLEDs by light extraction technique 24 1.5 References 29 Chapter 2 Fabrication processes and measurements 36 2.1 Device fabrication and measurement systems of OSCs 36 2.1.1 Device fabrication 36 2.1.2 Measurement systems of OSCs 37 2.2 Device fabrication and measurement systems of OLEDs 39 2.2.1 Device fabrication 39 2.2.2 Measurement systems of OLEDs 39 2.2.3 Transient electroluminescence (TrEL) measurement 40 2.3 Nano-imprinting technique and IZO sputtering 40 2.3.1 Nano-imprinting technique 40 2.3.2 Sputtering system 41 2.4 References 41 Chapter 3 Small Organic Solar Cells (SMOSCs) 42 3.1 Introduction 42 3.2 Photophysical properties of D-A-A materials 43 3.3 Comparison of optimized device structures among four D-A-A donor materials 46 3.3.1 Device performances of these SMOSCs 46 3.4 Optimization of SMOSCs with DTCPBTCN2 as donor 50 3.4.1 Tuning the ratio of BHJ layer 51 3.4.2 Tuning the thickness of BHJ layer 54 3.5 Optimization of SMOSCs with DTCPiFBTCN as donor 56 3.5.1 Tuning the ratio of BHJ layer 57 3.5.2 Tuning the thickness of BHJ layer 59 3.6 Ternary structure of OSCs 61 3.6.1 Adding TAPC in DTCPBTCN2:C70 as ternary structure 62 3.6.2 Adding DTCPBTCN2 in TAPC:C70 as ternary structure 64 3.7 References 67 Chapter 4 Blue Triplet-Triplet Annihilation (TTA) Organic light-emitting diode (OLED) 68 4.1 Introduction 68 4.2 Photophysical properties and molecular structure of these anthracene-core derivatives 69 4.3 Non-doped blue TTA OLEDs 73 4.3.1 Device performances of the TTA OLEDs 73 4.3.2 TrEL analysis and operation lifetime 76 4.4 Optimization of non-doped TTA OLED with monoBizAn as emitter 79 4.4.1 Tuning the thickness of EML 80 4.4.2 Tuning the thickness of ETL 85 4.5 Investigating TTA doping concentration with o-DiCbzBz as host 90 4.5.1 Tuning monoBizAn doping concentration with o-DiCbzBz as host 90 4.5.2 Tuning NpBorAn doping concentration with o-DiCbzBz as host 96 4.6 References 99 Chapter 5 Light extraction through grating nanostructure 100 5.1 Introduction 100 5.2 Properties of sputtered indium zinc oxide thin films 102 5.3 Optimization procedure of blue PHOLEDs with IZO anode 104 5.3.1 Tuning oxygen plasma time 104 5.3.2 Tuning IZO thickness 107 5.3.3 Tuning HTL thickness 110 5.4 Blue PHOLED with nanostructure and macrolens 112 5.4.1 EQE, J-V characteristics, EL spectra and ω-k plots 113 5.4.2 Experiment and simulation results of dispersion relation 129 5.5 References 135 Chapter 6 Summary 136 Appendix A 138 A-1 Device performance of non-doped monoOXDAn 138 A-2 Device performance of doping ADN with o-DiCbzBz as host 141 A-2-1 Tuning ADN doping concentration with o-DiCbzBz as host 141 | |
| dc.language.iso | zh-TW | |
| dc.subject | 三重態-三重態-湮滅 | zh_TW |
| dc.subject | 波導模態 | zh_TW |
| dc.subject | 表面電漿態 | zh_TW |
| dc.subject | 奈米結構 | zh_TW |
| dc.subject | 塊材異質接面 | zh_TW |
| dc.subject | 光萃取 | zh_TW |
| dc.subject | 有機太陽能電池 | zh_TW |
| dc.subject | 有機發光二極體 | zh_TW |
| dc.subject | surface plasmon mode | en |
| dc.subject | bulk heterojunction | en |
| dc.subject | triplet-triplet annihilation | en |
| dc.subject | organic light-emitting diode | en |
| dc.subject | light extraction | en |
| dc.subject | nanostructure | en |
| dc.subject | Organic solar cells | en |
| dc.subject | waveguide mode | en |
| dc.title | 有機太陽能電池及有機發光二極體之研究 | zh_TW |
| dc.title | Study on organic solar cell and organic light-emitting diode | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 107-1 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 梁文傑(Man-kit Leung),汪根欉(Ken-Tsung Wong),魏茂國(Mau-Kuo Wei),邱天隆(Tien-Lung Chiu) | |
| dc.subject.keyword | 有機太陽能電池,塊材異質接面,三重態-三重態-湮滅,有機發光二極體,光萃取,奈米結構,表面電漿態,波導模態, | zh_TW |
| dc.subject.keyword | Organic solar cells,bulk heterojunction,triplet-triplet annihilation,organic light-emitting diode,light extraction,nanostructure,surface plasmon mode,waveguide mode, | en |
| dc.relation.page | 146 | |
| dc.identifier.doi | 10.6342/NTU201900148 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2019-01-22 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| 顯示於系所單位： | 光電工程學研究所 | |
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