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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 劉懷勝(Hwai-Shen Liu) | |
| dc.contributor.author | Pei-Sheng Tang | en |
| dc.contributor.author | 唐沛陞 | zh_TW |
| dc.date.accessioned | 2021-06-16T13:01:26Z | - |
| dc.date.available | 2015-08-22 | |
| dc.date.copyright | 2013-08-22 | |
| dc.date.issued | 2013 | |
| dc.date.submitted | 2013-08-07 | |
| dc.identifier.citation | Adam, J.,Lindblad, N.,Hendricks, C., (1968) The collision, coalescence, and disruption of water droplets. Journal of Applied Physics. 39 (11) 5173-5180.
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/61349 | - |
| dc.description.abstract | 本研究為錯流式旋轉填充床內同時吸收甲苯與異丙醇的質傳程序，甲苯為疏水性揮發有機物，而異丙醇為親水性揮發有機物，分別使用水、矽油以及矽油加水混合物作為吸收劑進行吸收程序。單獨用水時，異丙醇最高吸收分率可達到0.99，而甲苯最高吸收分率只有0.1，顯示對於親水性揮發有機物水是一個適當的吸收劑；單獨使用矽油時，甲苯最佳吸收分率為0.78，而異丙醇只有0.33，明顯可看出矽油適合作為疏水性揮發有機物的吸收劑。
接著，使用矽油加水混合物吸收甲苯與異丙醇實驗，其結果顯示，甲苯與異丙醇皆可達到0.9以上的吸收分率。為了探討矽油加水混合物對於甲苯與異丙醇的吸收是正向或負向幫助，透過E factor(enhancement factor)的計算進行分析。甲苯的E值在矽油流量為0.1L/min時，隨水流量增加而上升到最大值為2.5，當矽油流量越大，能提昇的E值幅度就越小，而異丙醇的E值在水流量為0.01 L/min與0.03L/min時皆小於1，隨著水量的增加回逐漸上升到1左右。以上的結果主要來自碰撞包覆效應與總液體流量效應兩個因素所影響，碰撞包覆效應會使得矽油包覆在水的外面，造成矽油與氣體接觸面積增加，但讓水與氣體接觸面積減少，因此有利於甲苯的吸收，卻不利於吸收異丙醇；總液體流量效應可藉由水使得黏度高的矽油均勻分布於床體中，使得甲苯與矽油接觸面積大幅提升，使得甲苯的質傳效果變好。 | zh_TW |
| dc.description.abstract | This work presented a mass transfer process of absorbing toluene and isopropanol in a cross-flow rotating packed bed (RPB) at the same time. Toluene is a hydrophobic volatile organic compound (VOC) while isopropanol is a hydrophilic VOC. Water, silicone oil, as well as the mixture of silicone oil and water were used as absorbents for these absorption processes. When using water as the only absorbent, the best absorption fraction of isopropanol was 0.99, but it was only 0.1 for toluene. It obviously indicated that water is a suitable absorbent for hydrophilic VOCs. When silicone oil was the absorbent alone, the best absorption fraction for toluene was 0.78, and 0.33 for isopropanol. It suggested that silicone oil is a appropriate absorbent for hydrophobic VOCs.
Then, we implemented the absorption processes of toluene and isopropanol by the mixture of silicone oil and water. Both absorption fractions for these two compounds could reach more than 0.9. We calculated the enhancement factor (E) to evaluate the impacts on absorptions of toluene and isopropanol by this mixed absorbent. As the silicone oil flow rate was 0.1, the E value of toluene rose significantly to 2.5 with increasing water flow rate. Higher the silicone oil flow rate resulted in less enhancements. However, the E value of isopropanol was less than 1 when the water flow rate were 0.01 and 0.03 L/min, and it would gradually increase to about 1 with the increase of water flow rate. The “insertive merging effect” and the total liquid flow rate effect could be used to explain the results above. The insertive merging effect means that the water droplet inserted into silicone oil droplet. This effect increased the effective gas-liquid contact area of oil but hindered that of water. Thus it was favorable for absorption of toluene but not for isopropanol. The total liquid flow rate effect means that water lead silicone oil of high viscosity to distribute better inside the RPB, and it causes higher gas-liquid contact area between toluene and silicone oil. Therefore, it could enhance mass transfer for hydrophobic VOCs. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-16T13:01:26Z (GMT). No. of bitstreams: 1 ntu-102-R00524067-1.pdf: 4435601 bytes, checksum: 2dcd600c4da50845981e95704a806770 (MD5) Previous issue date: 2013 | en |
| dc.description.tableofcontents | 摘要 I
Abstract II 目錄 IV 表目錄 VII 圖目錄 XII 第一章 緒論 1 1-1 序言 1 1-2 研究方向 2 第二章 文獻回顧 3 2-1 旋轉填充床 (Rotating packed bed, RPB) 3 2-1.1旋轉填充床之構造與床體設計 4 2-1.2 壓降 10 2-1.3 旋轉填充床之液體流態、液體滯留量、液體滯留時間 14 2-1.4 旋轉填充床之有效質傳界面積 18 2-1.5 液膜質傳係數 20 2-1.6 氣膜質傳係數 23 2-1.7 旋轉填充床之微觀混合 26 2-1.8 錯流式旋轉填充床之回顧 29 2-1.9 旋轉填充床之應用與發展 33 2-2 揮發性有機物質處理方法 43 2-3旋轉填充床中液滴的碰撞 47 2-3.1相同液滴之碰撞行為 47 2-3.2 具有表面張力差異之雙液滴碰撞 49 第三章 實驗與分析方法 54 3-1 實驗裝置 54 3-2實驗藥品與分析儀器 56 3-3 實驗方法 58 3-3.1 實驗流程 58 3-3.2平衡常數實驗方法 60 3-4總括氣膜體積質傳係數(overall volumetric mass transfer coefficient)分析 62 3-4.1雙膜理論(two-film theory) 62 3-4.2 錯流式旋轉填充床之氣膜質傳係數分析 65 第四章 結果與討論 70 4-1 以吸收分率評估質傳效果 70 4-1.1 以水為吸收劑吸收甲苯與異丙醇氣體 71 4-1.2 以矽油為吸收劑吸收甲苯與異丙醇氣體 71 4-1.3 矽油加水混合作為吸收劑吸收甲苯與異丙醇氣體 72 4-1.3-1 水與油碰撞包覆效應以及總液體流量對吸收分率之影響 74 4-2 矽油加水與單獨水或矽油之吸收效果比較，E factor 84 4-2.1-1 水的流量(Lw)對於E factor的影響 84 4-2.1-2矽油的流量(Lo)對於E factor的影響 86 4-2.2 轉速對於E factor之影響 98 4-3 總液體流量效應與碰撞包覆效應對於矽油加水吸收程序的影響 104 4-3.1 觀察總液體流量對於吸收效果之影響 104 4-3.2 觀察碰撞包覆效應對於吸收效果之影響 110 4-4 以質傳係數評估質傳的效果 113 4-4.1 平衡常數的估算 113 4-4.2矽油加水對於質傳係數(KGa)的影響 116 第五章 結論 122 參考文獻 125 符號說明 134 | |
| dc.language.iso | zh-TW | |
| dc.subject | 旋轉填充床 | zh_TW |
| dc.subject | 吸收 | zh_TW |
| dc.subject | 質傳 | zh_TW |
| dc.subject | 疏水性揮發有機物 | zh_TW |
| dc.subject | 親水性揮發有機物 | zh_TW |
| dc.subject | Mass transfer | en |
| dc.subject | Hydrophilic VOCs | en |
| dc.subject | Hydrophobic VOCs | en |
| dc.subject | Absorption | en |
| dc.subject | Rotating packed bed (RPB) | en |
| dc.title | 在旋轉填充床內吸收親疏水性有機揮發物之研究 | zh_TW |
| dc.title | Absorption of hydrophilic and hydrophobic volatile organic compounds in a rotating packed bed | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 101-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 林佳璋(Chia-Chang Lin),陳昱劭(Yu-Shao Chen),江佳穎(Chia-Ying Chiang) | |
| dc.subject.keyword | 旋轉填充床,吸收,質傳,疏水性揮發有機物,親水性揮發有機物, | zh_TW |
| dc.subject.keyword | Rotating packed bed (RPB),Absorption,Mass transfer,Hydrophilic VOCs,Hydrophobic VOCs, | en |
| dc.relation.page | 138 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2013-08-07 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
| 顯示於系所單位： | 化學工程學系 | |
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