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  1. NTU Theses and Dissertations Repository
  2. 理學院
  3. 物理學系
請用此 Handle URI 來引用此文件: http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/56561
完整後設資料紀錄
DC 欄位值語言
dc.contributor.advisor陳永芳(Yang-Fang Chen)
dc.contributor.authorChen-You Suen
dc.contributor.author蘇宸右zh_TW
dc.date.accessioned2021-06-16T05:34:56Z-
dc.date.available2022-08-11
dc.date.copyright2020-09-15
dc.date.issued2020
dc.date.submitted2020-08-11
dc.identifier.citation(1) Wiersma, D. S.; Lagendijk, A., Light diffusion with gain and random lasers. Phys. Rev. E 1996, 54, 4256.
(2) Lawandy, N. M.; Balachandran, R. M.; Gomes, A. S. L.; Sauvain, E., Laser Action in Strongly Scattering Media. Nature 1994, 369, 340-340.
(3) Wiersma, D. S., The physics and applications of random lasers. Nat. Phys. 2008, 4, 359-367.
(4) Luan, F.; Gu, B. B.; Gomes, A. S. L.; Yong, K. T.; Wen, S. C.; Prasad, P. N., Lasing in nanocomposite random media. Nano Today 2015, 10, 168-192.
(5) Cao, H.; Zhao, Y. G.; Ho, S. T.; Seelig, E. W.; Wang, Q. H.; Chang, R. P. H., Random laser action in semiconductor powder. Phys. Rev. Lett. 1999, 82, 2278-2281.
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(8) Caixeiro, S.; Gaio, M.; Marelli, B.; Omenetto, F. G.; Sapienza, R., Silk-Based Biocompatible Random Lasing. Adv. Opt. Mater. 2016, 4, 998-1003.
(9) Shi, Z. F.; Sun, X. G.; Wu, D.; Xu, T. T.; Tian, Y. T.; Zhang, Y. T.; Li, X. J.; Du, G. T., Near-infrared random lasing realized in a perovskite CH3NH3PbI3 thin film. J. Mater. Chem. C 2016, 4, 8373-8379.
(10) Silva-Neto, M. L.; de Oliveira, M. C. A.; Dominguez, C. T.; Lins, R. E. M.; Rakov, N.; de Araujo, C. B.; Menezes, L. D.; de Oliveira, H. P.; Gomes, A. S. L., UV random laser emission from flexible ZnO-Ag-enriched electrospun cellulose acetate fiber matrix. Sci. Rep. 2019, 9, 11765.
(11) Dixit, T.; Arora, A.; Krishnan, A.; Ganapathi, K. L.; Nayak, P. K.; Rao, M. S. R., Near Infrared Random Lasing in Multilayer MoS2. ACS Omega 2018, 3, 14097-14102.
(12) Chang, S. W.; Liao, W. C.; Liao, Y. M.; Lin, H. I.; Lin, H. Y.; Lin, W. J.; Lin, S. Y.; Perumal, P.; Haider, G.; Tai, C. T.; Shen, K. C.; Chang, C. H.; Huang, Y. F.; Lin, T. Y.; Chen, Y. F., A White Random Laser. Sci. Rep. 2018, 8, 2720.
(13) Redding, B.; Choma, M. A.; Cao, H., Speckle-free laser imaging using random laser illumination. Nat. Photonics 2012, 6, 355-359.
(14) Peng, H. Y.; Bi, S. G.; Ni, M. L.; Xie, X. L.; Liao, Y. G.; Zhou, X. P.; Xue, Z. G.; Zhu, J. T.; Wei, Y.; Bowman, C. N.; Mai, Y. W., Monochromatic Visible Light 'Photoinitibitor': Janus-Faced Initiation and Inhibition for Storage of Colored 3D Images. J. Am. Chem. Soc. 2014, 136, 8855-8858.
(15) Juels, A., RFID security and privacy: A research survey. IEEE J. Sel. Area. Comm. 2006, 24, 381-394.
(16) Andres, J.; Hersch, R. D.; Moser, J. E.; Chauvin, A. S., A New Anti-Counterfeiting Feature Relying on Invisible Luminescent Full Color Images Printed with Lanthanide-Based Inks. Adv. Funct. Mater. 2014, 24, 5029-5036.
(17) Yoon, B.; Lee, J.; Park, I. S.; Jeon, S.; Lee, J.; Kim, J. M., Recent functional material based approaches to prevent and detect counterfeiting. J. Mater. Chem. C 2013, 1, 2388-2403.
(18) You, M. L.; Zhong, J. J.; Hong, Y.; Duan, Z. F.; Lin, M.; Xu, F., Inkjet printing of upconversion nanoparticles for anti-counterfeit applications. Nanoscale 2015, 7, 4423-4431.
(19) Liao, Y. M.; Liao, W. C.; Chang, S. W.; Hou, C. F.; Tai, C. T.; Su, C. Y.; Hsu, Y. T.; Wu, M. H.; Chou, R. J.; Lee, Y. H.; Lin, S. Y.; Lin, W. J.; Chang, C. H.; Haider, G.; Kataria, M.; Roy, P. K.; Bera, K. P.; Paullnbaraj, C. R.; Hu, H. W.; Lin, T. Y.; Chen, Y. F., Inkjet-Printed Random Lasers. Adv. Mater. Technol. 2018, 3, 1800214.
(20) Dubois, J.; La Rochelle, S. Active cooperative tuned identification friend or foe (ACTIFF). U.S. Patent 5966227, October 12, 1999.
(21) Letokhov, V. S., Generation of Light by a Scattering Medium with Negative Resonance Absorption. Sov. Phys. Jetp-Ussr 1968, 26, 835.
(22) Liu, X. Y.; Shan, C. X.; Wang, S. P.; Zhang, Z. Z.; Shen, D. Z., Electrically pumped random lasers fabricated from ZnO nanowire arrays. Nanoscale 2012, 4, 2843-2846.
(23) Solis, D. M.; Taboada, J. M.; Landesa, L.; Rodriguez, J. L.; Obelleiro, F., SQUEEZING MAXWELL'S EQUATIONS INTO THE NANOSCALE (Invited Paper). Progress In Electromagnetics Research 2015, 154, 35-50.
(24) Amendola, V.; Bakr, O. M.; Stellacci, F., A Study of the Surface Plasmon Resonance of Silver Nanoparticles by the Discrete Dipole Approximation Method: Effect of Shape, Size, Structure, and Assembly. Plasmonics 2010, 5, 85-97.
(25) Meng, X. G.; Fujita, K.; Zong, Y. H.; Murai, S.; Tanaka, K., Random lasers with coherent feedback from highly transparent polymer films embedded with silver nanoparticles. Appl. Phys. Lett. 2008, 92, 201112.
(26) Porel, S.; Singh, S.; Harsha, S. S.; Rao, D. N.; Radhakrishnan, T. P., Nanoparticle-embedded polymer: In situ synthesis, free-standing films with highly monodisperse silver nanoparticles and optical limiting. Chem. Mater. 2005, 17, 9-12.
(27) Chiad, B. T.; Latif, K. H.; Kadhim, F. J.; Hammed, M. A., Random laser of R6G dye and TiO2 nanoparticles doped in PMMA polymer. Adv. Mater. Phys. Chem. 2011, 1, 20.
(28) Garcia, M. A., Surface plasmons in metallic nanoparticles: fundamentals and applications. J. Phys. D. Appl. Phys. 2011, 44, 283001.
(29) Dominguez, C. T.; Maltez, R. L.; dos Reis, R. M. S.; de Melo, L. S. A.; de Araujo, C. B.; Gomes, A. S. L., Dependence of random laser emission on silver nanoparticle density in PMMA films containing rhodamine 6G. J. Opt. Soc. Am. B 2011, 28, 1118-1123.
(30) Meng, X. G.; Fujita, K.; Murai, S.; Tanaka, K., Coherent random lasers in weakly scattering polymer films containing silver nanoparticles. Phys. Rev. A 2009, 79, 053817
(31) Dice, G. D.; Mujumdar, S.; Elezzabi, A. Y., Plasmonically enhanced diffusive and subdiffusive metal nanoparticle-dye random laser. Appl. Phys. Lett. 2005, 86, 131105
(32) Ismail, W. Z. W.; Vo, T. P.; Goldys, E. M.; Dawes, J. M., Plasmonic enhancement of Rhodamine dye random lasers. Laser Phys. 2015, 25, 085001.
(33) Kitur, J.; Zhu, G.; Bahoura, M.; Noginov, M. A., Dependence of the random laser behavior on the concentrations of dye and scatterers. J. Opt. 2010, 12, 024009.
(34) Sen, T.; Sadhu, S.; Patra, A., Surface energy transfer from rhodamine 6G to gold nanoparticles: A spectroscopic ruler. Appl. Phys. Lett. 2007, 91, 043104.
(35) Kalele, S.; Deshpande, A. C.; Singh, S. B.; Kulkarni, S. K., Tuning luminescence intensity of RHO6G dye using silver nanoparticles. Bull. Mater. Sci. 2008, 31, 541-544.
(36) Fu, Y.; Lakowicz, J. R., Modification of single molecule fluorescence near metallic nanostructures. Laser Photonics Rev. 2009, 3, 221-232.
(37) Zehentbauer, F. M.; Moretto, C.; Stephen, R.; Thevar, T.; Gilchrist, J. R.; Pokrajac, D.; Richard, K. L.; Kiefer, J., Fluorescence spectroscopy of Rhodamine 6G: Concentration and solvent effects. Spectrochim. Acta A 2014, 121, 147-151.
dc.identifier.urihttp://tdr.lib.ntu.edu.tw/jspui/handle/123456789/56561-
dc.description.abstract由於具備雷射等級光強、狹窄光譜帶寬及廣發光角度,隨機雷射已經吸引無數研究者投入心力,探索與其相關的各種潛在應用。在本文章中,我們將研究焦點投射在隨機雷射跟光學加密科技有關的應用,包含防偽列印技術、軍用敵我辨識系統,以及文件和資料的加密及防盜;為整合這些應用,我們提出多功能隨機雷射墨水的概念。為驗證此一概念,我們首先利用自發輻射和隨機雷射光譜的差異,來定義本系統的加密方式,並展示隱型簽名的應用。緊接者,我們藉由深入討論此隨機雷射系統的可調性,提出多位元加密的可行性。不僅如此,此隨機雷射墨水具有可製成暫態元件的特性,並且可以適用於不同材料的表面。考慮到此隨機雷射墨水的多功能性及簡便製作程序,我們相信它將很快能被實作於各種應用,並可幫助光學加密及防偽科技的創新與發展。zh_TW
dc.description.abstractWith the superiority of laser-level intensity, narrow spectral line-width, and broad-angular emission, random lasers (RLs) have drawn considerable research interests for their potential to carry out a variety of applications. In this work, the applications associated with optical encoded technologies, including security printing, military friend or foe identification (FFI) and anti-counterfeiting of documents are highlighted, and the concept of a transient RL “smart ink” has been proposed. The proof-of-concept was first demonstrated as invisible signatures, which encoded the messages through the spectral difference of spontaneous emission and RL under specified optical pumping. Next, the possibility for encoding the data with multi-bit signals was further confirmed by exploiting the threshold tunability of RLs. Moreover, the transient characteristic of this smart ink and its capability to be attached on freeform surfaces of different materials were also shown. With the advantages of facile manufacturing process and multiple purpose, it is expected that this ink can soon be carried out in a variety of practical utilities.en
dc.description.provenanceMade available in DSpace on 2021-06-16T05:34:56Z (GMT). No. of bitstreams: 1
U0001-2507202016552400.pdf: 6192715 bytes, checksum: 89c0176f8b8c0a3ab03973383e4a9b6d (MD5)
Previous issue date: 2020
en
dc.description.tableofcontents口試委員會審定書 2
誌謝 3
中文摘要 5
Abstract 6
Contents 7
List of Figures 9
Chapter 1 Introduction 12
Chapter 2 Theoretical Background 16
2.1 Photoluminescence (PL) 16
2.1.1 Introduction 16
2.1.2 Mechanism 17
2.2 Random Laser (RL) 20
2.2.1 Laser 20
2.2.2 Mechanism 23
2.2.3 Categories and Emission properties 24
2.2.4 Applications 27
2.3 Localized Surface Plasmon Resonance (LSPR) 30
2.4 Fluorescence Energy Transfer 36
2.4.1 Dipole Interaction 36
2.4.2 Förster Resonance Energy Transfer (FRET) 38
Chapter 3 Experimental Details 39
3.1 The List of Materials 39
3.2 Fabrication of Materials and Samples 39
3.3 The List of Instruments 44
3.4 Random Laser Measurement 44
3.5 Absorption Spectroscopy and Spectrophotometer 47
Chapter 4 Results and Discussion 49
4.1 Highlight of Major Contributions 49
4.2 Spontaneous Emission versus Random Laser – The 0/1 50
4.3 Tunability and Multi-bit Signals 53
4.4 Random Laser Characteristics on Different Substrates 58
4.5 The Transient Characteristic 61
Conclusion 63
Reference 64
dc.language.isoen
dc.subject隨機雷射zh_TW
dc.subject光學加密zh_TW
dc.subject防偽zh_TW
dc.subjectoptical encodingen
dc.subjectrandom laseren
dc.subjectsecurity inken
dc.title多功能隨機雷射墨水—光學加密系統及防偽技術方面的應用zh_TW
dc.titleMultifunctional Random Laser Smart Inksen
dc.typeThesis
dc.date.schoolyear108-2
dc.description.degree碩士
dc.contributor.author-orcid0000-0002-9051-4835
dc.contributor.oralexamcommittee謝雅萍(Ya-Ping Hsieh),許芳琪(Fang-Chi Hsu)
dc.subject.keyword隨機雷射,防偽,光學加密,zh_TW
dc.subject.keywordrandom laser,security ink,optical encoding,en
dc.relation.page69
dc.identifier.doi10.6342/NTU202001850
dc.rights.note有償授權
dc.date.accepted2020-08-12
dc.contributor.author-college理學院zh_TW
dc.contributor.author-dept物理學研究所zh_TW
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