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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 徐治平(Jyh-Ping Hsu) | |
| dc.contributor.author | Hou-Hsueh Wu | en |
| dc.contributor.author | 吳厚學 | zh_TW |
| dc.date.accessioned | 2021-06-15T13:01:38Z | - |
| dc.date.available | 2019-07-26 | |
| dc.date.copyright | 2016-07-26 | |
| dc.date.issued | 2016 | |
| dc.date.submitted | 2016-07-11 | |
| dc.identifier.citation | [1] X. Hou, W. Guo L. Jiang, Chem. Soc. Rev., 2011, 40, 2385-2401.
[2] W. Guo, Y. Tian L. Jiang, Acc. Chem. Res., 2013, 46, 2834-2846. [3] D. G. Haywood, A. Saha-Shah, L. A. Baker S. C. Jacobson, Anal. Chem., 2015, 87, 172-187. [4] Y. Fu, H. Tokuhisa L. A. Baker, Chem. Comm., 2009, DOI: 10.1039/b910511e, 4877-4879. [5] M. Ali, S. Nasir, P. Ramirez, J. Cervera, S. Mafe W. Ensinger, ACS Nano, 2012, 6, 9247-9257. [6] S. Umehara, M. Karhanek, R. W. Davis N. Pourmand, Proc. Natl. Acad. Sci. U.S.A., 2009, 106, 4611-4616. [7] C. A. Morris, A. K. Friedman L. A. Baker, Analyst, 2010, 135, 2190-2202. [8] S. R. German, L. Luo, H. S. White T. L. Mega, J. Phys. Chem. C, 2013, 117, 703-711. [9] W. J. Lan, C. Kubeil, J. W. Xiong, A. Bund H. S. White, J. Phys. Chem. C, 2014, 118, 2726-2734. [10] R. Vogel, G. Willmott, D. Kozak, G. S. Roberts, W. Anderson, L. Groenewegen, B. Glossop, A. Barnett, A. Turner M. Trau, Anal. Chem., 2011, 83, 3499-3506. [11] Y. L. Ying, J. Zhang, R. Gao Y. T. Long, Angew. Chem. Int. Ed., 2013, 52, 13154-13161. [12] J. Menestrina, C. 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U.S.A., 2009, 106, 4611-4616. [9] Y. L. Ying, J. Zhang, R. Gao Y. T. Long, Angew. Chem. Int. Ed., 2013, 52, 13154-13161. [10] B. Yameen, M. Ali, R. Neumann, W. Ensinger, W. Knoll O. Azzaroni, Nano Lett., 2009, 9, 2788-2793. [11] K. Xiao, G. Xie, P. Li, Q. Liu, G. Hou, Z. Zhang, J. Ma, Y. Tian, L. Wen L. Jiang, Adv. Mater., 2014, 26, 6560-6565. [12] H. Zhang, X. Hou, L. Zeng, F. Yang, L. Li, D. Yan, Y. Tian L. Jiang, J. Am. Chem. Soc., 2013, 135, 16102-16110. [13] M. Ali, P. Ramirez, S. Mafe, R. Neumann W. Ensinger, ACS Nano, 2009, 3, 603-608. [14] E. B. Kalman, I. Vlassiouk Z. S. Siwy, Adv. Mater., 2008, 20, 293-297. [15] I. Vlassiouk Z. S. Siwy, Nano Lett., 2007, 7, 552-556. [16] J. Gao, W. Guo, D. Feng, H. Wang, D. Zhao L. Jiang, J. Am. Chem. Soc., 2014, 136, 12265-12272. [17] A. Siria, P. Poncharal, A. L. Biance, R. Fulcrand, X. Blase, S. T. Purcell L. Bocquet, Nature, 2013, 494, 455-458. [18] S. Tseng, Y. M. Li, C. Y. Lin J. P. Hsu, Nanoscale, 2016, 8, 2350-2357. [19] S. J. Kim, S. H. Ko, K. H. Kang J. Han, Nat. Nanotechnol., 2010, 5, 297-301. [20] R. B. Schoch, J. Han P. Renaud, Rev. Mod. Phys., 2008, 80, 839-883. [21] L. H. Yeh, M. Zhang, N. Hu, S. W. Joo, S. Qian J. P. Hsu, Nanoscale, 2012, 4, 5169-5177. [22] M. Jia T. Kim, Anal. Chem., 2014, 86, 7360-7367. [23] L. H. Yeh, M. Zhang, S. Qian, J. P. Hsu S. Tseng, J. Phys. Chem. C, 2012, 116, 8672-8677. [24] Y. Ma, L. H. Yeh, C. Y. Lin, L. Mei S. Qian, Anal. Chem., 2015, 87, 4508-4514. [25] I. Vlassiouk, S. Smirnov Z. Siwy, Nano Lett., 2008, 8, 1978-1985. [26] L. H. Yeh, C. Hughes, Z. Zeng S. Qian, Anal. Chem., 2014, 86, 2681-2686. [27] Z. S. Siwy, Adv. Funct. Mater., 2006, 16, 735-746. [28] R. Karnik, C. Duan, K. Castelino, H. Daiguji A. Majumdar, Nano Lett., 2007, 7, 547-551. [29] D. Momotenko, F. Cortés-Salazar, J. Josserand, S. Liu, Y. Shao H. H. Girault, Phys. Chem. Chem. Phys., 2011, 13, 5430-5440. [30] Y. Kubo, T. J. Baldwin, Y. N. Jan L. Y. Jan, Nature, 1993, 362, 127-133. [31] I. Favre, E. 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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/50841 | - |
| dc.description.abstract | 圓錐奈米孔道因為擁有特殊的幾何形狀，它們能引起許多有趣的電動力學現象，像是離子濃度極化(ICP)以及離子電流整流效應(ICR)。我們考慮兩種圓錐奈米孔道：第一為僅將奈米孔道內之表面改質一層聚電解質層；第二為在奈米孔道內以及兩端出口外之表面全部改質一層聚電解質層。我們藉由一系列的數值模擬去探討電雙層厚度以及聚電解質層厚度對奈米孔道的離子電流整流效應的影響。我們發現第一種奈米孔道的離子濃度極化程度比第二種強。另外，當調控溶液離子濃度時，兩種奈米孔道的整流效應係數( )表現極不同。當溶液離子濃度很低時，可以在第一種奈米孔道發現其整流效應係數有翻轉的現象。
接著，我們討論表面上酸性官能基以及鹼性官能基都有並且電荷可調節的奈米孔道。並探討了奈米孔道形狀、溶液酸鹼值pH以及溶液鹽濃度對離子電流整流效應的影響。當溶液pH大於等電位點，我們發現當改變奈米孔道的曲率時，整流效應係數會出現區域最大值。相較之下，當溶液pH小於等電位點時，整流效應係數僅會隨著孔道曲率上升而單調遞增。 | zh_TW |
| dc.description.abstract | Due to their specific geometry, conical nanopores are capable of yielding several interesting electrokinetic phenomena, such as ion concentration polarization (ICP) and ion current rectification (ICR). Extending previous analyses, we consider two types of nanopore: only the inner surface of a nanopore is functionalized by a polyelectrolyte (PE) layer in type I nanopore, and both its outer and inner surfaces are functionalized in type II nanopore. Numerical simulation is conducted to examine the influences of the double layer thickness and the thickness of the PE layer of a nanopore on its ICR behavior. We show that the ICP in type I nanopore is more significant than that in type II nanopore. In addition, as the bulk salt concentration varies, the rectification factors ( ) for type I and II nanopore are different significantly. In particular, if the salt concentration is low, an inversion in is observed in type I nanopore.
Furthermore, we consider the case where the nanopore surface has both acidic and basic functional groups, and is pH-regulated. The influences of the nanopore shape, solution pH, and bulk salt concentration on the associated ICR behavior are examined. If the solution pH exceeds the isoelectric point, the rectification factor shows a local maximum as the curvature of the nanopore surface varies. In contrast, if it is lower than the isoelectric point, that factor increases monotonically with increasing surface curvature. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-15T13:01:38Z (GMT). No. of bitstreams: 1 ntu-105-R03524075-1.pdf: 5873868 bytes, checksum: 27d79d45747993cd37007ef01e4bcd72 (MD5) Previous issue date: 2016 | en |
| dc.description.tableofcontents | 中 文 摘 要 I
ABSTRACT II CONTENTS IV LIST OF FIGURES VI CHAPTER 1: Effect of Polyelectrolyte Modification 1 1-1. Introduction 2 1-2. Theory 5 1-3. Solution procedure 8 1-4. Results and discussion 8 1-4.1 Influence of applied voltage 9 1-4.2 Counterion enrichment inside nanopore 10 1-4.3 Effect of ion concentration polarization 12 1-4.4 Influence of bulk salt concentration 13 1-4.5 Influence of PE Layer Thickness on Ionic Current 16 1-5. Conclusions 17 References 20 CHAPTER 2: Effect of Nanopore Shape 34 2-1. Introduction 35 2-2. Theory 37 2-3. Solution Procedure 40 2-4. Results and Discussion 40 2-4.1. I-Vapp curves at pH 10 41 2-4.2. Electric field and ion conductivity at pH 10 42 2-4.3 I-V Curve and Cross Sectional Average Ion Concentration at pH 4 44 2-4.4 Electric field and ion conductivity at pH 4 45 2-4.5 Influence of pH on Rf 46 2-5. Conclusions 47 References 49 CHAPTER 3 Conclusions 64 APPENDIX A 67 A-1. Code Verification 67 A-2. Contours of the dimensionless counterions (cations) concentration near the base region of a nanopore 69 APPENDIX B 70 B-1. Code Verification 70 B-2. Axial distribution of cross sectional averaged total ion concentration at pH 10 72 B-3. Cross sectional averaged axial electric field at pH 10 75 B-4. Axial distribution of cross sectional averaged total ion concentration at pH 4 79 B-5. Axial distribution of cross sectional averaged electric field at pH 4 83 B-6. Axial distribution of cross sectional averaged H+ concentration and surface charge density ( ) 87 B-7. Axial distribution of ion conductivity and electric field in Figure 2-10 91 | |
| dc.language.iso | zh-TW | |
| dc.subject | 聚電解質層 | zh_TW |
| dc.subject | 圓錐奈米孔道 | zh_TW |
| dc.subject | 離子濃度極化 | zh_TW |
| dc.subject | 離子電流整流效應 | zh_TW |
| dc.subject | 電雙層 | zh_TW |
| dc.subject | 子彈形奈米孔道 | zh_TW |
| dc.subject | 圓錐奈米孔道 | zh_TW |
| dc.subject | 離子濃度極化 | zh_TW |
| dc.subject | 離子電流整流效應 | zh_TW |
| dc.subject | 聚電解質層 | zh_TW |
| dc.subject | 電雙層 | zh_TW |
| dc.subject | 子彈形奈米孔道 | zh_TW |
| dc.subject | bullet-shaped nanopore | en |
| dc.subject | polyelectrolyte layer | en |
| dc.subject | electric double layer | en |
| dc.subject | bullet-shaped nanopore | en |
| dc.subject | ion concentration polarization | en |
| dc.subject | ion current rectification | en |
| dc.subject | polyelectrolyte layer | en |
| dc.subject | electric double layer | en |
| dc.subject | conical nanopore | en |
| dc.subject | conical nanopore | en |
| dc.subject | ion concentration polarization | en |
| dc.subject | ion current rectification | en |
| dc.title | 圓錐奈米孔道內之離子電流整流效應:聚電解質層改質方式與孔道形狀之影響 | zh_TW |
| dc.title | Ionic Current Rectification in Conical Nanopores: Effect of Polyelectrolyte Modification and Nanopore Shape | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 104-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 曾琇瑱(Shio-Jenn Tseng),張有義(Yu-Yi Chang),郭勇志(Yung-Chih Kuo),葉禮賢(Li-Hsien Yeh) | |
| dc.subject.keyword | 圓錐奈米孔道,離子濃度極化,離子電流整流效應,聚電解質層,電雙層,子彈形奈米孔道, | zh_TW |
| dc.subject.keyword | conical nanopore,ion concentration polarization,ion current rectification,polyelectrolyte layer,electric double layer,bullet-shaped nanopore, | en |
| dc.relation.page | 92 | |
| dc.identifier.doi | 10.6342/NTU201600801 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2016-07-11 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
| 顯示於系所單位： | 化學工程學系 | |
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