請用此 Handle URI 來引用此文件:
http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/29698完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 吳志毅(Chih-I Wu) | |
| dc.contributor.author | Chao-Wei Chen | en |
| dc.contributor.author | 陳晁偉 | zh_TW |
| dc.date.accessioned | 2021-06-13T01:15:19Z | - |
| dc.date.available | 2007-07-23 | |
| dc.date.copyright | 2007-07-23 | |
| dc.date.issued | 2007 | |
| dc.date.submitted | 2007-07-17 | |
| dc.identifier.citation | [1] M. Pope and C.E. Swenberg. Electronic processes in organic crystals and polymers. Oxford University Press, 1999.
[2] CW Tang and SA VanSlyke. Organic electroluminescent diodes. Applied Physics Letters, 51:913, 1987. [3] W. BrÄutting, S. Berleb, and A.G. MÄuckl. Device physics of organic light-emitting diodes based on molecular materials. Organic Electronics, 2(1):1{36, 2001. [4] MA Baldo and SR Forrest. Interface-limited injection in amorphous organic semiconductors. Physical Review B, 64(8):85201, 2001. [5] T. YASUDA, Y. YAMAGUCHI, D.C. ZOU, and T. TSUTSUI. Carrier mobilities in organic electron transport materials determined from space charge limited current. Japanese journal of applied physics, 41(9):5626~5629, 2002. [6] AJ Campbell, DDC Bradley, and DG Lidzey. Space-charge limited conduction with traps in poly (phenylene vinylene) light emitting diodes. Journal of Applied Physics, 82:6326, 1997. [7] PS Davids, IH Campbell, and DL Smith. Device model for single carrier organic diodes. Journal of Applied Physics, 82:6319, 1997. [8] C. Shen, I.G. Hill, and A. Kahn. Role of Electrode Contamination in Electron Injection at Mg: Ag/Alq. Adv. Mater, 11:18, 1999. [9] C. H. Chen. Organic Electroluminescent Materials & Devices. Wu-Nan Book Inc., 1 edition, 2005. [10] WILKINSON DL MULLER G KUMBERGER O SCHMIDBAUR H, LETTENBAUER J. Model systems for gallium extraction .1. structure and molecular-dynamics of aluminum and gallium tris(oxinates). Z. Naturforsch., Teil B, 46:901~911. [11] C. GANZORIG and M. FUJIHIRA. A lithium carboxylate ultrathin film on an aluminum cathode for enhanced electron injection in organic electroluminescent devices. Japanese journal of applied physics. Pt. 2, Letters, 38(11B):L1348{L1350, 1999. [12] M. Brinkmann, G. Gadret, M. Muccini, C. Taliani, N. Masciocchi, and A. Sironi. Correlation Between Molecular Packing and Optical Properties in Different Crystalline Polymorphs and Amorphous Thin Films of mer-Tris (8-hydroxyquinoline) aluminum (III). J. Am. Chem. Soc, 122(21):5147{5157, 2000. [13] PE Burrows et al. Relationship between electroluminescence and current transport in organic heterojunction light-emitting devices. Journal of Applied Physics, 79(10):7991, 1996. [14] Forrest S.R. Bulovic, V. and M.E. Thompson. Color-tunable organic light emitting devices, 2001. US Patent 6287712. [15] T. YOKOYAMA, D. YOSHIMURA, E. ITO, H. ISHII, Y. OUCHI, and K. SEKI. Energy level alignment at Alq3/LiF/Al interfaces studied by electron spectroscopies: Island growth of LiF and size-dependence of the electronic structures. Japanese journal of applied physics, 42(6A):3666-3675, 2003. [16] JD Anderson, EM McDonald, PA Lee, ML Anderson, EL Ritchie, HK Hall, T. Hopkins, EA Mash, J. Wang, A. Padias, et al. Electrochemistry and electrogenerated chemiluminescence processes of the components of aluminum quinolate/triarylamine, and related organic light-emitting diodes. J. Am. Chem. Soc, 120(37):9646, 1998. [17] BN Limketkai and MA Baldo. Charge injection into cathode-doped amorphous organic semiconductors. Physical Review B, 71(8):85207,2005. [18] H. Ishii, K. Sugiyama, E. Ito, and K. Seki. Energy Level Alignment and Interfacial Electronic Structures at Organic/Metal and Organic/Organic Interfaces. Advanced Materials, 11(8):605{625, 1999. [19] A. Rajagopal and A. Kahn. Photoemission spectroscopy investigation of magnesium-Alq3 interfaces. Journal of Applied Physics, 84(1):355~358, 1998. [20] ST Lee. Energy level alignment at Alq/metal interfaces. Applied Physics Letters, 72(13):1593, 1998. [21] IG Hill, A. Kahn, ZG Soos, and RA Pascal Jr. Charge Separation Energy in Films of pi-Conjugated Organic Molecules. Chem. Phys. Lett, 327:181~188, 2000. [22] PE Burrows and SR Forrest. Electroluminescence from trap-limited current transport in vacuum deposited organic light emitting devices. Applied Physics Letters, 64:2285, 1994. [23] M. Kiy. Observation of the Mott-Gurney law in tris(8-hydroxyquinoline) aluminum films. Applied Physics Letters, 80(7):1198, 2002. [24] VG Kozlov. Temperature independent performance of organic semiconductor lasers. Applied Physics Letters, 71(18):2575, 1997. [25] RG Kepler, PM Beeson, SJ Jacobs, RA Anderson, MB Sinclair, VS Valencia, and PA Cahill. Electron and hole mobility in tris (8-hydroxyquinolinolato-N1, O8) aluminum. Applied Physics Letters, 66:3618, 1995. [26] W. BruµEtting, S. Berleb, and AG MuµEckl. Space-charge limited conduction with a ‾eld and temperature dependent mobility in Alq light-emitting devices. Synthetic Metals, 122(99):104, 2001. [27] Murray A. Lampert and Peter Mark. Current injection in solids. New York : Academic Press, 1970. [28] M.A. Lampert. Simplified Theory of Space-Charge-Limited Currents in an Insulator with Traps. Physical Review, 103(6):1648~1656, 1956. [29] Z.H. Kafafi. Organic light-emitting materials and devices II; Proceedings of the Meeting, San Diego, CA, July 21-23, 1998. Bellingham, WA, Society of Photo-Optical Instrumentation Engineers(SPIE Proceedings., 3476, 1998. [30] D. Natali and M. Sampietro. Field-dependent mobility from space-charge-limited current{voltage curves. Journal of Applied Physics,92:5310, 2002. [31] PN Murgatroyd. Theory of space-charge-limited current enhanced by Frenkel effect. Journal of Physics D Applied Physics, 3(2):151~156, 1970. [32] J. Frenkel. On Pre-Breakdown Phenomena in Insulators and Electronic Semi-Conductors. Physical Review, 54(8):647~648, 1938. [33] W. Y. Hung. Study of Charge Transport in Amorphous Organic Semiconductors and OLED Materials. National Taiwan University, 2005. section 3.3. [34] DF Barbe. Space-charge-limited current enhanced by Frenkel effect. Journal of Physics D Applied Physics, 4(11):1812~1815, 1971. [35] RH YOUNG. Trap-free space-charge-limited current: analytical solution for an arbitrary mobility law. Philosophical magazine letters, 70(5):331~333, 1994. [36] WD Gill. Drift mobilities in amorphous charge-transfer complexes of trinitrofluorenone and poly-n-vinylcarbazole. Journal of Applied Physics, 43:5033, 2003. | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/29698 | - |
| dc.description.abstract | 本論文著重載子傳導反應在電流電壓特性上的研究。我們回顧與發展了兩種常見的空間電荷限制電流(SCLC)理論。第一個理論是SCLC搭配指數分佈陷阱的模型,我們發展了正確的解析解,與傳統的近似解相較,我們指出近似解低估了電流的大小,並低估了電流電壓曲線的參數l。第二個理論是SCLC搭配Poole-Frenkel的效應,修改後的電性曲線指出高壓下的電流將正比於溫度。對這兩者理論而言,未來研究電流-電壓-溫度(J-V-T)將有助於澄清這兩種模型的可行性。我們利用前者的模型配合我們實驗的數據,結論熱致電子濃度(n0)與移動率(u0)的乘積約在6.5×10^4 ~ 8×10^5 (/ V s cm)之間。 | zh_TW |
| dc.description.abstract | This thesis focuses on the current-voltage characteristic of carrier transport. Two common SCLC theories are overviewed and developed. For the case of space charge limited current (SCLC) with exponential trap distribution, we develop the analytical solution, indicating that the traditional approximation underestimates the current magnitude and underestimates the parameter l in the model. For the case of SCLC coupled with Poole-Frenkel effect, the refined solution at high bias indicates the current depends on the temperature directly. For both cases, studying J-V-T will justify the validity of these models. We use the former model to ‾t our experiment data, and conclude that the product of thermal generated electron concentration and the mobility to be around 6.5x10^4 ~ 8x10^5(/cm V s). | en |
| dc.description.provenance | Made available in DSpace on 2021-06-13T01:15:19Z (GMT). No. of bitstreams: 1 ntu-96-R94941011-1.pdf: 1663384 bytes, checksum: 52d0cc8ee3f8bcea663afaedd091aec0 (MD5) Previous issue date: 2007 | en |
| dc.description.tableofcontents | 1 Introduction 6
2 Devices, experimental methods, and materials 10 2.1 Devices:Al/Alq3/Al 11 2.2 Experimental methods: thermal evaporation 13 2.3 Materials 18 2.3.1 Aluminum 18 2.3.2 Alq3 19 3 Carrier transport 22 3.1 Trap free SCLC theory 25 3.1.1 Ohm's Law 31 3.1.2 Mott-Gurney Law 32 3.2 A transformation and the scaling law 35 3.2.1 the slope of J-V 40 3.3 TCLC theory 41 3.3.1 J-V of TCLC with exponential trap distribution 44 3.3.2 Arguments for TCLC with exponential trap distribution 58 3.4 Field-dependent SCLC theory 60 3.4.1 J-V of SCLC with Poole-Frenkel type mobility 62 3.4.2 Arguments for SCLC with PF type mobility 67 3.5 Simulation strategy: tricks and the philosophy 69 3.6 Conclusion 71 4 Result and discussion 73 4.1 Fitting to experiment data and discussion 73 4.2 Conclusion and future work 82 | |
| dc.language.iso | en | |
| dc.subject | 熱蒸鍍 | zh_TW |
| dc.subject | 空間電荷限制電流 | zh_TW |
| dc.subject | 比例法則 | zh_TW |
| dc.subject | 指數分佈陷阱 | zh_TW |
| dc.subject | Poole-Frenkel效應 | zh_TW |
| dc.subject | Poole-Frenkel effect | en |
| dc.subject | exponential trap distribution | en |
| dc.subject | The Scaling Law | en |
| dc.subject | SCLC | en |
| dc.subject | thermal evaporation | en |
| dc.title | 有機發光二極體載子傳導的電流電壓特徵曲線 | zh_TW |
| dc.title | Current-Voltage Characteristics of Carrier Transport in Organic Light-Emitting Devices | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 95-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.coadvisor | 吳忠幟(Chung- Chih Wu) | |
| dc.contributor.oralexamcommittee | 汪根欉(Ken-Tsung Wong) | |
| dc.subject.keyword | 熱蒸鍍,空間電荷限制電流,比例法則,指數分佈陷阱,Poole-Frenkel效應, | zh_TW |
| dc.subject.keyword | thermal evaporation,SCLC,The Scaling Law,exponential trap distribution,Poole-Frenkel effect, | en |
| dc.relation.page | 88 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2007-07-20 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| 顯示於系所單位: | 光電工程學研究所 | |
文件中的檔案:
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| ntu-96-1.pdf 未授權公開取用 | 1.62 MB | Adobe PDF |
系統中的文件,除了特別指名其著作權條款之外,均受到著作權保護,並且保留所有的權利。
