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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/23399完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 吳忠幟 | |
| dc.contributor.author | Chih-Hung Tsai | en |
| dc.contributor.author | 蔡志宏 | zh_TW |
| dc.date.accessioned | 2021-06-08T05:01:11Z | - |
| dc.date.copyright | 2011-02-09 | |
| dc.date.issued | 2011 | |
| dc.date.submitted | 2011-01-21 | |
| dc.identifier.citation | Chapter 1
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/23399 | - |
| dc.description.abstract | 由於染料敏化太陽能電池具有元件結構及製作相對簡易、材料成本低廉，且光電轉換效率良好等優點，目前已經成為太陽能電池研究課題中的重要方向之一。染料敏化太陽能電池基本結構包含了透明導電基板、奈米多孔性二氧化鈦薄膜工作電極、染料、電解質、以及白金對電極等五個部分，每個部分對元件整體效率皆有極重要的影響。本論文針對染料敏化太陽能電池中的透明導電基板、奈米多孔性二氧化鈦薄膜工作電極以及新型有機染料進行了有系統的研究與分析。
本論文首先探討了氟摻雜氧化錫透明導電基板的表面紋理結構對染料敏化太陽能電池元件效率的影響。我們對六種不同的透明導電基板進行了表面形貌與光電特性量測，將具有不同紋理結構與霧度的透明導電基板應用於染料敏化太陽能電池元件中，並對染料敏化太陽能電池元件，進行電流-電壓曲線、光譜響應曲線以及電化學阻抗頻譜量測，且比較不同紋理結構透明導電基板對元件效率的影響。 接著，本論文分析了不同結構的奈米多孔性二氧化鈦薄膜工作電極對染料敏化太陽能電池元件效率的影響。我們對五種不同顆粒大小的二氧化鈦奈米顆粒進行了表面形貌、光學穿透率與霧度等量測。並使用此五種不同大小的二氧化鈦奈米顆粒，搭配組合成二十種不同結構的奈米多孔性二氧化鈦電極，應用於染料敏化太陽能電池元件中。對各種染料敏化太陽能電池元件，進行了電流-電壓曲線、頻譜響應曲線以及電化學阻抗頻譜量測，且比較不同結構的奈米多孔性二氧化鈦薄膜電極對元件光電轉換效率的影響。 最後，我們研究了三類的新型有機染料，對此三類的新型有機染料進行了完整且系統性的光物理特性分析，並將這三類新型有機染料應用於染料敏化太陽能電池元件中，進而量測元件的電流-電壓曲線、頻譜響應曲線以及電化學阻抗頻譜，並探討此三類新型有機染料分子在染料敏化太陽能電池元件光電特性上的表現。 | zh_TW |
| dc.description.abstract | Dye-Sensitized Solar Cells (DSSCs) offer the advantages of simple structures, easy manufacturing, low cost, and high power conversion efficiencies. Therefore, DSSCs have become one important area of solar cell researches. Dye-Sensitized Solar Cells generally consist of transparent conductive substrates, nanoporous TiO2 working electrode, dye, electrolyte, and a platinum counter electrode. Each part of the cell has crucial effects on overall cell efficiency. This dissertation conducted a systematic investigation on the transparent conductive substrates, nanoporous TiO2 working electrode, and novel organic dyes for DSSCs.
First, we studied how the texture structures of various fluorine-doped tin oxide (FTO) transparent conductors influence the power conversion efficiency of DSSCs. Measurements of surface morphology and electro-optical properties were conducted for different kinds of FTO transparent conductors, each having a different texture structure and haze ratio. Effects of these transparent conductors on current density-voltage (J-V) curves, incident photo-to-current conversion efficiency (IPCE) spectra, and electrochemical impedance spectroscopy (EIS) analysis of DSSCs were analyzed. Device performance parameters based on these different textured FTO conductors were then compared. Next, the effects of various TiO2 nanoparticle working electrodes on DSSCs were studied. Measurements of surface morphology, optical transmittance, and haze ratio were conducted for TiO2 nanoparticles of different sizes. These TiO2 nanoparticles were combined in twenty different ways for DSSCs. The J-V curves, IPCE curves, and the EIS analysis of different DSSCs were analyzed to study how nanoporous TiO2 electrodes of different structures influence the DSSC efficiency. Finally, three types of novel organic dyes were investigated for DSSC. Comprehensive photophysical characterization of these dyes and their applications to DSSCs were conducted. The J-V curves, IPCE curves, and the EIS of device performance parameters of DSSCs based on these novel organic dyes were thoroughly analyzed to manifest their potential. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-08T05:01:11Z (GMT). No. of bitstreams: 1 ntu-100-D93941008-1.pdf: 7465011 bytes, checksum: c8297f4b48b892f1bfdf8ac30e033c5d (MD5) Previous issue date: 2011 | en |
| dc.description.tableofcontents | 致謝 i
摘要 ii Abstract iv Table of Contents vi List of Figures ix List of Tables xiv Chapter 1 Introduction 1 1.1 Renewable Energy and Solar Cells 1 1.1.1 Renewable Energy 1 1.1.2 Solar Cells 3 1.2 Overview of Dye-Sensitized Solar Cells 6 1.2.1 History of Dye-Sensitized Solar Cells 6 1.2.2 Principles of Dye-Sensitized Solar Cells 7 1.2.3 Characterization of Dye-Sensitized Solar Cells 8 1.2.4 Optimization of Dye-Sensitized Solar Cells 11 1.2.5 Recent Milestones 13 1.3 Motivation and Dissertation Organization 14 References 16 Figures 23 Chapter 2 Effects of Textures in FTO on Dye-Sensitized Solar Cells 30 2.1 Introduction 30 2.2 Experimental 32 2.2.1 Materials 32 2.2.2 Characterization of Textured FTO 32 2.2.3 Device Fabrication and Characterization 33 2.3 Results and Discussions 37 2.3.1 Properties of Textured FTO 37 2.3.2 Device Characteristics 38 2.3.3 Electrochemical Impedance Spectroscopy of Devices 39 2.4 Conclusions 42 References 43 Tables and Figures 46 Chapter 3 Dye-sensitized Solar Cells Using Combinations of Different TiO2 Nanoparticles 61 3.1 Introduction 61 3.2 Experimental 63 3.2.1 Materials 63 3.2.2 Characterization of TiO2 Nanoparticle Thin Films 63 3.2.3 Device Fabrication and Characterization 64 3.3 Results and Discussions 68 3.3.1 Properties of TiO2 Nanoparticle Thin Films 68 3.3.2 Device Characteristics 69 3.3.3 Electrochemical Impedance Spectroscopy of Devices 72 3.4 Conclusions 74 References 75 Tables and Figures 78 Chapter 4 Dye-Sensitized Solar Cells Using Novel Organic Dyes 95 4.1 Introduction 95 4.2 Organic Dyes Containing Coplanar Diphenyl-Substituted Dithienosilole Core for Efficient Dye-Sensitized Solar Cells 99 4.2.1 Introduction 99 4.2.2 Experimental 101 4.2.3 Results and Discussions 104 4.3 Novel Organic Dyes Bearing Electron-Deficient Pyrimidine as π-Spacer for Efficient Dye-Sensitized Solar Cells 109 4.3.1 Introduction 109 4.3.2 Experimental 111 4.3.3 Results and Discussions 114 4.4 Dye-Sensitized Solar Cells Using Organic Dyes Containing Coplanar Diindenothiophene Moiety 120 4.4.1 Introduction 120 4.4.2 Experimental 121 4.4.3 Results and Discussions 124 4.5 Conclusions 130 References 132 Tables and Figures 138 Chapter 5 Summary and Future Directions 160 5.1 Summary 160 5.2 Future Directions 162 References 164 | |
| dc.language.iso | en | |
| dc.subject | 二氧化鈦奈米顆粒 | zh_TW |
| dc.subject | 奈米多孔性 | zh_TW |
| dc.subject | 氟摻雜氧化錫 | zh_TW |
| dc.subject | 染料敏化太陽能電池 | zh_TW |
| dc.subject | 紋理結構 | zh_TW |
| dc.subject | 有機染料 | zh_TW |
| dc.subject | texture structure | en |
| dc.subject | organic dyes | en |
| dc.subject | titanium dioxide nanoparticles | en |
| dc.subject | nanoporous | en |
| dc.subject | fluorine-doped tin oxide | en |
| dc.subject | dye-sensitized solar cell | en |
| dc.title | 染料敏化太陽能電池元件結構及新型有機染料之研究 | zh_TW |
| dc.title | Investigation of Device Structures and Novel Organic Dyes for Dye-Sensitized Solar Cells | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 99-1 | |
| dc.description.degree | 博士 | |
| dc.contributor.oralexamcommittee | 汪根欉,陳介偉,李重君,蘇海清,陳俐吟 | |
| dc.subject.keyword | 染料敏化太陽能電池,紋理結構,氟摻雜氧化錫,奈米多孔性,二氧化鈦奈米顆粒,有機染料, | zh_TW |
| dc.subject.keyword | dye-sensitized solar cell,texture structure,fluorine-doped tin oxide,nanoporous,titanium dioxide nanoparticles,organic dyes, | en |
| dc.relation.page | 165 | |
| dc.rights.note | 未授權 | |
| dc.date.accepted | 2011-01-21 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| 顯示於系所單位： | 光電工程學研究所 | |
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