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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 駱尚廉 | |
| dc.contributor.author | Tzu-Ning Kuo | en |
| dc.contributor.author | 郭子寧 | zh_TW |
| dc.date.accessioned | 2021-06-07T23:44:11Z | - |
| dc.date.copyright | 2014-07-15 | |
| dc.date.issued | 2014 | |
| dc.date.submitted | 2014-07-11 | |
| dc.identifier.citation | 1. 王根樹，蔡詩偉，陳家揚, 飲用水水源與水質中新興污染物對人體健康風險評估之研究計畫. 行政院環保署，國立臺灣大學環境衛生研究所, 2010.
2. Tan, C.Q., N.Y. Gao, Y. Deng, W.L. Rong, S.D. Zhou, and N.X. Lu, Degradation of antipyrine by heat activated persulfate. Separation and Purification Technology, 2013. 109, 122-128. 3. Le, C., J.H. Wu, P. Li, X.D. Wang, N.W. Zhu, P.X. Wu, and B. Yang, Decolorization of anthraquinone dye Reactive Blue 19 by the combination of persulfate and zero-valent iron. Water Science and Technology, 2011. 64(3), 754-759. 4. Lin, C.C., L.T. Lee, and L.J. Hsu, Performance of UV/S2O82- process in degrading polyvinyl alcohol in aqueous solutions. Journal of Photochemistry and Photobiology a-Chemistry, 2013. 252, 1-7. 5. Wofford, B.A., M.W. Jackson, C. Hartz, and J.W. Bevan, Surface wave plasma abatement of CHF3 and CF4 containing semiconductor process emissions. Environmental Science & Technology, 1999. 33(11), 1892-1897. 6. IPCC, IPCC Fourth Assessment Report:Climate Change 2007: Working Group I: The Physical Science Basis. 2007. 7. Lehmler, H.J., Synthesis of environmentally relevant fluorinated surfactants - a review. Chemosphere, 2005. 58(11), 1471-1496. 8. Lau, C., K. Anitole, C. Hodes, D. Lai, A. Pfahles-Hutchens, and J. Seed, Perfluoroalkyl acids: A review of monitoring and toxicological findings. Toxicological Sciences, 2007. 99(2), 366-394. 9. LoNostro, P., S.M. Choi, C.Y. Ku, and S.H. Chen, Fluorinated microemulsions: A study of the phase behavior and structure. Journal of Physical Chemistry B, 1999. 103(25), 5347-5352. 10. Gao, X.D. and J. Chorover, Adsorption of perfluorooctanoic acid and perfluorooctanesulfonic acid to iron oxide surfaces as studied by flow-through ATR-FTIR spectroscopy. Environmental Chemistry, 2012. 9(2), 148-157. 11. EPA, U.S., Emerging Contaminants –Perfluorooctane Sulfonate (PFOS) and Perfluorooctanoic Acid (PFOA). United States Environmental Protection Agency Solid Waste & Emergency Responseand (5106P) EPA 505-F-11-002 May 2012. 12. Vecitis, C.D., Y.J. Wang, J. Cheng, H. Park, B.T. Mader, and M.R. Hoffmann, Sonochemical Degradation of Perfluorooctanesulfonate in Aqueous Film-Forming Foams. Environmental Science & Technology, 2010. 44(1), 432-438. 13. Tseng, C.L., L.L. Liu, C.M. Chen, and W.H. Ding, Analysis of perfluorooctanesulfonate and related fluorochemicals in water and biological tissue samples by liquid chromatography-ion trap mass spectrometry. Journal of Chromatography A, 2006. 1105(1-2), 119-126. 14. Gustafsson, O., P.M. Gschwend, and K.O. Buesseler, Settling removal rates of PCBs into the Northwestern Atlantic derived from U-238-Th-234 disequilibria. Environmental Science & Technology, 1997. 31(12), 3544-3550. 15. Prevedouros, K., I.T. Cousins, R.C. Buck, and S.H. Korzeniowski, Sources, fate and transport of perfluorocarboxylates. Environmental Science & Technology, 2006. 40(1), 32-44. 16. Martin, J.W., S.A. Mabury, K.R. Solomon, and D.C.G. Muir, Bioconcentration and tissue distribution of perfluorinated acids in rainbow trout (Oncorhynchus mykiss). Environmental Toxicology and Chemistry, 2003. 22(1), 196-204. 17. Ahrens, L., S. Felizeter, R. Sturm, Z.Y. Xie, and R. Ebinghaus, Polyfluorinated compounds in waste water treatment plant effluents and surface waters along the River Elbe, Germany. Marine Pollution Bulletin, 2009. 58(9), 1326-1333. 18. Chen, H., C. Zhang, J.B. Han, Y.X. Yu, and P. Zhang, PFOS and PFOA in influents, effluents, and biosolids of Chinese wastewater treatment plants and effluent-receiving marine environments. Environmental Pollution, 2012. 170, 26-31. 19. Guo, R., W.J. Sim, E.S. Lee, J.H. Lee, and J.E. Oh, Evaluation of the fate of perfluoroalkyl compounds in wastewater treatment plants. Water Research, 2010. 44(11), 3476-3486. 20. Lin, A.Y., S.C. Panchangam, and P.S. Ciou, High levels of perfluorochemicals in Taiwan's wastewater treatment plants and downstream rivers pose great risk to local aquatic ecosystems. Chemosphere, 2010. 80(10), 1167-74. 21. Schultz, M.M., C.P. Higgins, C.A. Huset, R.G. Luthy, D.F. Barofsky, and J.A. Field, Fluorochemical mass flows in a municipal wastewater treatment facility. Environmental Science & Technology, 2006. 40(23), 7350-7357. 22. Murakami, M., H. Shinohara, and H. Takada, Evaluation of wastewater and street runoff as sources of perfluorinated surfactants (PFSs). Chemosphere, 2009. 74(4), 487-93. 23. Yu, J., J.Y. Hu, S. Tanaka, and S. Fujii, Perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA) in sewage treatment plants. Water Research, 2009. 43(9), 2399-2408. 24. Smithwick, M., D.C.G. Muir, S.A. Mabury, K.R. Solomon, J.W. Martin, C. Sonne, E.W. Born, R.J. Letcher, and R. Dietz, Perflouroalkyl contaminants in liver tissue from East Greenland polar bears (Ursus maritimus). Environmental Toxicology and Chemistry, 2005. 24(4), 981-986. 25. Hurley, M.D., M.P.S. Andersen, T.J. Wallington, D.A. Ellis, J.W. Martin, and S.A. Mabury, Atmospheric chemistry of perfluorinated carboxylic acids: Reaction with OH radicals and atmospheric lifetimes. Journal of Physical Chemistry A, 2004. 108(4), 615-620. 26. Murakami, M., K. Kuroda, N. Sato, T. Fukushi, S. Takizawa, and H. Takada, Groundwater Pollution by Perfluorinated Surfactants in Tokyo. Environmental Science & Technology, 2009. 43(10), 3480-3486. 27. Murakami, M., C. Morita, T. Morimoto, and H. Takada, Source analysis of perfluorocarboxylates in Tokyo Bay during dry weather and wet weather using sewage markers. Environmental Chemistry, 2011. 8(4), 355-362. 28. Vestergren, R. and I.T. Cousins, Tracking the Pathways of Human Exposure to Perfluorocarboxylates. Environmental Science & Technology, 2009. 43(15), 5565-5575. 29. Kennedy, G.L., J.L. Butenhoff, G.W. Olsen, J.C. O'Connor, A.M. Seacat, R.G. Perkins, L.B. Biegel, S.R. Murphy, and D.G. Farrar, The toxicology of perfluorooctanoate. Critical Reviews in Toxicology, 2004. 34(4), 351-384. 30. Post, G.B., J.B. Louis, K.R. Cooper, B.J. Boros-Russo, and R.L. Lippincott, Occurrence and Potential Significance of Perfluorooctanoic Acid (PFOA) Detected in New Jersey Public Drinking Water Systems. Environmental Science & Technology, 2009. 43(12), 4547-4554. 31. Ferrey, M.L., J.T. Wilson, C. Adair, C.M. Su, D.D. Fine, X.Y. Liu, and J.W. Washington, Behavior and Fate of PFOA and PFOS in Sandy Aquifer Sediment. Ground Water Monitoring and Remediation, 2012. 32(4), 63-71. 32. Giesy, J.P. and K. Kannan, Perfluorochemical surfactants in the environment. Environmental Science & Technology, 2002. 36(7), 146a-152a. 33. Boulanger, B., J.D. Vargo, J.L. Schnoor, and K.C. Hornbuckle, Evaluation of perfluorooctane surfactants in a wastewater treatment system and in a commercial surface protection product. Environmental Science & Technology, 2005. 39(15), 5524-5530. 34. Loganathan, B.G., K.S. Sajwan, E. Sinclair, K.S. Kumar, and K. Kannan, Perfluoroalkyl sulfonates and perfluorocarboxylates in two wastewater treatment facilities in Kentucky and Georgia. Water Research, 2007. 41(20), 4611-4620. 35. Yamada, T., P.H. Taylor, R.C. Buck, M.A. Kaiser, and R.J. Giraud, Thermal degradation of fluorotelomer treated articles and related materials. Chemosphere, 2005. 61(7), 974-84. 36. Ghafoori, S., M. Mehrvar, and P.K. Chan, Free-Radical-Induced Degradation of Aqueous Polyethylene Oxide by UV/H2O2: Experimental Design, Reaction Mechanisms, and Kinetic Modeling. Industrial & Engineering Chemistry Research, 2012. 51(46), 14980-14993. 37. Crittenden, J.C., S.M. Hu, D.W. Hand, and S.A. Green, A kinetic model for H2O2/UV process in a completely mixed batch reactor. Water Research, 1999. 33(10), 2315-2328. 38. Buxton, G.V., C.L. Greenstock, W.P. Helman, and A.B. Ross, Critical-Review of Rate Constants for Reactions of Hydrated Electrons, Hydrogen-Atoms and Hydroxyl Radicals (.Oh/.O-) in Aqueous-Solution. Journal of Physical and Chemical Reference Data, 1988. 17(2), 513-886. 39. Christensen, H., K. Sehested, and H. Corfitzen, Reactions of Hydroxyl Radicals with Hydrogen-Peroxide at Ambient and Elevated-Temperatures. Journal of Physical Chemistry, 1982. 86(9), 1588-1590. 40. Koppenol, W.H., The Haber-Weiss cycle - 70 years later. Redox Report, 2001. 6(4), 229-234. 41. Weinstein, J. and B.H.J. Bielski, Kinetics of the Interaction of Ho2 and O2-Radicals with Hydrogen-Peroxide - Haber-Weiss Reaction. Journal of the American Chemical Society, 1979. 101(1), 58-62. 42. Bielski, B.H.J., D.E. Cabelli, R.L. Arudi, and A.B. Ross, Reactivity of Ho2/O-2 Radicals in Aqueous-Solution. Journal of Physical and Chemical Reference Data, 1985. 14(4), 1041-1100. 43. Elliot, A.J. and G.V. Buxton, Temperature-Dependence of the Reactions Oh + O-2- and Oh + Ho2 in Water up to 200-Degrees-C. Journal of the Chemical Society-Faraday Transactions, 1992. 88(17), 2465-2470. 44. Linden, K.G.S., C. M.; Andrews, S.; Atasi, K.; and V.S. Korategere, M.; Suffet, I. H. M., Innovative UV Technologies to Oxidize Organic and Organoleptic Chemicals. IWA Publishing: London, 2005. 45. Vecitis, C.D., H. Park, J. Cheng, B.T. Mader, and M.R. Hoffmann, Treatment technologies for aqueous perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA). Frontiers of Environmental Science & Engineering in China, 2009. 3(2), 129-151. 46. Tang, H., Q. Xiang, M. Lei, J. Yan, L. Zhu, and J. Zou, Efficient degradation of perfluorooctanoic acid by UV–Fenton process. Chemical Engineering Journal, 2012. 184, 156-162. 47. 江佳玲，張鎮南，黃科倫‡, 探討臭氧結合紫外光反應去除腐植酸之降解情形. 東海科學, 2007. 9, 15-28. 48. Hori, H., E. Hayakawa, H. Einaga, S. Kutsuna, K. Koike, T. Ibusuki, H. Kiatagawa, and R. Arakawa, Decomposition of environmentally persistent perfluorooctanoic acid in water by photochemical approaches. Environmental Science & Technology, 2004. 38(22), 6118-6124. 49. Chen, J., P.-y. Zhang, and J. Liu, Photodegradation of perfluorooctanoic acid by 185 nm vacuum ultraviolet light. Journal of Environmental Sciences, 2007. 19(4), 387-390. 50. Petrier, C., M.F. Lamy, A. Francony, A. Benahcene, B. David, V. Renaudin, and N. Gondrexon, Sonochemical Degradation of Phenol in Dilute Aqueous-Solutions - Comparison of the Reaction-Rates at 20-Khz and 487-Khz. Journal of Physical Chemistry, 1994. 98(41), 10514-10520. 51. Destaillats, H., H.M. Hung, and M.R. Hoffmann, Degradation of alkylphenol ethoxylate surfactants in water with ultrasonic irradiation. Environmental Science & Technology, 2000. 34(2), 311-317. 52. Kotronarou, A., G. Mills, and M.R. Hoffmann, Ultrasonic Irradiation of Para-Nitrophenol in Aqueous-Solution. Journal of Physical Chemistry, 1991. 95(9), 3630-3638. 53. Manousaki, E., E. Psillakis, N. Kalogerakis, and D. Mantzavinos, Degradation of sodium dodecylbenzene sulfonate in water by ultrasonic irradiation. Water Research, 2004. 38(17), 3751-3759. 54. Vinodgopal, K., M. Ashokkumar, and F. Grieser, Sonochemical degradation of a polydisperse nonylphenol ethoxylate in aqueous solution. Journal of Physical Chemistry B, 2001. 105(16), 3338-3342. 55. W-F Fan, C.-W.H., C-S Chen, and W-S Chen, Ablation Effect of High Intensity Focal Ultrasound with Bubbles. The 33rd National Conference on Theoretical and Applied Mechanics., 2009. 56. Didenko, Y.T., W.B. McNamara, and K.S. Suslick, Hot spot conditions during cavitation in water. Journal of the American Chemical Society, 1999. 121(24), 5817-5818. 57. Adewuyi, Y.G., Sonochemistry: Environmental science and engineering applications. Industrial & Engineering Chemistry Research, 2001. 40(22), 4681-4715. 58. Moriwaki, H., Y. Takagi, M. Tanaka, K. Tsuruho, K. Okitsu, and Y. Maeda, Sonochemical decomposition of perfluorooctane sulfonate and perfluorooctanoic acid. Environmental Science & Technology, 2005. 39(9), 3388-3392. 59. Ochoa-Herrera, V. and R. Sierra-Alvarez, Removal of perfluorinated surfactants by sorption onto granular activated carbon, zeolite and sludge. Chemosphere, 2008. 72(10), 1588-1593. 60. Karoyo, A.H. and L.D. Wilson, Tunable macromolecular-based materials for the adsorption of perfluorooctanoic and octanoic acid anions. Journal of Colloid and Interface Science, 2013. 402, 196-203. 61. Zhao, D.M., J. Cheng, C.D. Vecitis, and M.R. Hoffmann, Sorption of Perfluorochemicals to Granular Activated Carbon in the Presence of Ultrasound. Journal of Physical Chemistry A, 2011. 115(11), 2250-2257. 62. Yu, Q., R.Q. Zhang, S.B. Deng, J. Huang, and G. Yu, Sorption of perfluorooctane sulfonate and perfluorooctanoate on activated carbons and resin: Kinetic and isotherm study. Water Research, 2009. 43(4), 1150-1158. 63. Qu, Y., C.J. Zhang, F. Li, X.W. Bo, G.F. Liu, and Q. Zhou, Equilibrium and kinetics study on the adsorption of perfluorooctanoic acid from aqueous solution onto powdered activated carbon. Journal of Hazardous Materials, 2009. 169(1-3), 146-152. 64. Deng, S.B., Q. Zhou, G. Yu, J. Huang, and Q. Fan, Removal of perfluorooctanoate from surface water by polyaluminium chloride coagulation. Water Research, 2011. 45(4), 1774-1780. 65. Yu, J. and J. Hu, Adsorption of Perfluorinated Compounds onto Activated Carbon and Activated Sludge. Journal of Environmental Engineering, 2011. 137(10), 945-951. 66. House, D.A., Kinetics and Mechanism of Oxidations by Peroxydisulfate. Chemical Reviews, 1962. 62(3), 185-203. 67. Vorsina, I.A. and Y.I. Mikhailov, Kinetics of thermal decomposition of ammonium persulfate. Russian Chemical Bulletin, 1996. 45(3), 539-542. 68. Behrman, E.J. and D.H. Dean, Sodium peroxydisulfate is a stable and cheap substitute for ammonium peroxydisulfate (persulfate) in polyacrylamide gel electrophoresis. Journal of Chromatography B, 1999. 723(1-2), 325-326. 69. Lemaire, J., V. Croze, J. Maier, and M.O. Simonnot, Is it possible to remediate a BTEX contaminated chalky aquifer by in situ chemical oxidation? Chemosphere, 2011. 84(9), 1181-1187. 70. Krembs, F.J., R.L. Siegrist, M.L. Crimi, R.F. Furrer, and B.G. Petri, ISCO for Groundwater Remediation: Analysis of Field Applications and Performance. Ground Water Monitoring and Remediation, 2010. 30(4), 42-53. 71. Crimi, M.L. and J. Taylor, Experimental evaluation of catalyzed hydrogen peroxide and sodium persulfate for destruction of BTEX contaminants. Soil & Sediment Contamination, 2007. 16(1), 29-45. 72. Kolthoff, I.M. and I.K. Miller, The Chemistry of Persulfate .1. The Kinetics and Mechanism of the Decomposition of the Persulfate Ion in Aqueous Medium. Journal of the American Chemical Society, 1951. 73(7), 3055-3059. 73. Lee, Y., S.L. Lo, J. Kuo, and C.H. Hsieh, Decomposition of perfluorooctanoic acid by microwaveactivated persulfate: Effects of temperature, pH, and chloride ions. Frontiers of Environmental Science & Engineering, 2012. 6(1), 17-25. 74. Yan, J.C., M. Lei, L.H. Zhu, M.N. Anjum, J. Zou, and H.Q. Tang, Degradation of sulfamonomethoxine with Fe3O4 magnetic nanoparticles as heterogeneous activator of persulfate. Journal of Hazardous Materials, 2011. 186(2-3), 1398-1404. 75. Liu, C.S., K. Shih, C.X. Sun, and F. Wang, Oxidative degradation of propachlor by ferrous and copper ion activated persulfate. Science of the Total Environment, 2012. 416, 507-512. 76. Bagal, M.V. and P.R. Gogate, Degradation of 2,4-dinitrophenol using a combination of hydrodynamic cavitation, chemical and advanced oxidation processes. Ultrasonics Sonochemistry, 2013. 20(5), 1226-1235. 77. Chen, K.F., C.M. Kao, L.C. Wu, R.Y. Surampalli, and S.H. Liang, Methyl Tert-Butyl Ether (MTBE) Degradation by Ferrous Ion-Activated Persulfate Oxidation: Feasibility and Kinetics Studies. Water Environment Research, 2009. 81(7), 687-694. 78. Jiang, X.X., Y.L. Wu, P. Wang, H.J. Li, and W.B. Dong, Degradation of bisphenol A in aqueous solution by persulfate activated with ferrous ion. Environmental Science and Pollution Research, 2013. 20(7), 4947-4953. 79. Kusic, H., I. Peternel, N. Koprivanac, and A.L. Bozic, Iron-Activated Persulfate Oxidation of an Azo Dye in Model Wastewater: Influence of Iron Activator Type on Process Optimization. Journal of Environmental Engineering-Asce, 2011. 137(6), 454-463. 80. Liang, C.J. and Y.Y. Guo, Mass Transfer and Chemical Oxidation of Naphthalene Particles with Zerovalent Iron Activated Persulfate. Environmental Science & Technology, 2010. 44(21), 8203-8208. 81. Oh, S.Y. and D.S. Shin, Degradation of spent caustic by Fenton and persulfate oxidation with zero-valent iron. Journal of Chemical Technology and Biotechnology, 2013. 88(1), 145-152. 82. Gu, X.G., S.G. Lu, Z.F. Qiu, Q. Su, C.J. Banks, T. Imai, K.F. Lin, and Q.S. Luo, Photodegradation performance of 1,1,1-trichloroethane in aqueous solution: In the presence and absence of persulfate. Chemical Engineering Journal, 2013. 215, 29-35. 83. Xie, X.F., Y.Q. Zhang, W.L. Huang, and S.B. Huang, Degradation kinetics and mechanism of aniline by heat-assisted persulfate oxidation. Journal of Environmental Sciences-China, 2012. 24(5), 821-826. 84. Liang, C.J., Y.Y. Guo, Y.C. Chien, and Y.J. Wu, Oxidative Degradation of MTBE by Pyrite-Activated Persulfate: Proposed Reaction Pathways. Industrial & Engineering Chemistry Research, 2010. 49(18), 8858-8864. 85. Khan, J.A., X.X. He, H.M. Khan, N.S. Shah, and D.D. Dionysiou, Oxidative degradation of atrazine in aqueous solution by UV/H2O2/Fe2+, UV/S2O82-/Fe2+ and UV/HSO5-/Fe2+ processes: A comparative study. Chemical Engineering Journal, 2013. 218, 376-383. 86. Lee, Y.C., S.L. Lo, J. Kuo, and Y.L. Lin, Persulfate oxidation of perfluorooctanoic acid under the temperatures of 20-40 degrees C. Chemical Engineering Journal, 2012. 198, 27-32. 87. Wu, F.C., R.L. Tseng, and R.S. Juang, Initial behavior of intraparticle diffusion model used in the description of adsorption kinetics. Chemical Engineering Journal, 2009. 153(1-3), 1-8. 88. Chowdhury, S. and P. Saha, Adsorption Kinetic Modeling of Safranin onto Rice Husk Biomatrix Using Pseudo-first- and Pseudo-second-order Kinetic Models: Comparison of Linear and Non-linear Methods. Clean-Soil Air Water, 2011. 39(3), 274-282. 89. Wang, Z.L., T.L. Yue, Y.H. Yuan, R. Cai, C. Niu, and C.X. Guo, Kinetics of adsorption of bovine serum albumin on magnetic carboxymethyl chitosan nanoparticles. International Journal of Biological Macromolecules, 2013. 58, 57-65. 90. Liu, W.F., J.A. Zhang, C.L. Zhang, Y.F. Wang, and Y. Li, Adsorptive removal of Cr (VI) by Fe-modified activated carbon prepared from Trapa natans husk. Chemical Engineering Journal, 2010. 162(2), 677-684. 91. Chen, W.F., R. Parette, J.Y. Zou, F.S. Cannon, and B.A. Dempsey, Arsenic removal by iron-modified activated carbon. Water Research, 2007. 41(9), 1851-1858. 92. Vitela-Rodriguez, A.V. and J.R. Rangel-Mendez, Arsenic removal by modified activated carbons with iron hydro(oxide) nanoparticles. Journal of Environmental Management, 2013. 114, 225-231. 93. Tuna, A.O.A., E. Ozdemir, E.B. Simsek, and U. Beker, Removal of As(V) from aqueous solution by activated carbon-based hybrid adsorbents: Impact of experimental conditions. Chemical Engineering Journal, 2013. 223, 116-128. 94. Georgi, A. and F.D. Kopinke, Interaction of adsorption and catalytic reactions in water decontamination processes Part I. Oxidation of organic contaminants with hydrogen peroxide catalyzed by activated carbon. Applied Catalysis B-Environmental, 2005. 58(1-2), 9-18. 95. Santos, V.P., M.F.R. Pereira, P.C.C. Faria, and J.J.M. Orfao, Decolourisation of dye solutions by oxidation with H2O2 in the presence of modified activated carbons. Journal of Hazardous Materials, 2009. 162(2-3), 736-742. 96. Aguinaco, A., J.P. Pocostales, J.F. Garcia-Araya, and F.J. Beltran, Decomposition of hydrogen peroxide in the presence of activated carbons with different characteristics. Journal of Chemical Technology and Biotechnology, 2011. 86(4), 595-600. 97. Wang, G.P., T. Wu, Y.J. Li, D.J. Sun, Y. Wang, X.H. Huang, G.C. Zhang, and R.H. Liu, Removal of ampicillin sodium in solution using activated carbon adsorption integrated with H2O2 oxidation. Journal of Chemical Technology and Biotechnology, 2012. 87(5), 623-628. 98. Chen, C.C., W.C. Chen, M.R. Chiou, S.W. Chen, Y.Y. Chen, and H.J. Fan, Degradation of crystal violet by an FeGAC/H2O2 process. Journal of Hazardous Materials, 2011. 196, 420-425. 99. Yang, S.Y., X. Yang, X.T. Shao, R. Niu, and L.L. Wang, Activated carbon catalyzed persulfate oxidation of Azo dye acid orange 7 at ambient temperature. Journal of Hazardous Materials, 2011. 186(1), 659-666. 100. Yang, S.Y., P. Wang, X. Yang, G. Wei, W.Y. Zhang, and L. Shan, A novel advanced oxidation process to degrade organic pollutants in wastewater: Microwave-activated persulfate oxidation. Journal of Environmental Sciences-China, 2009. 21(9), 1175-1180. 101. Lien, H.L., Y.S. Jhuo, and L.H. Chen, Effect of heavy metals on dechlorination of carbon tetrachloride by iron nanoparticles. Environmental Engineering Science, 2007. 24(1), 21-30. 102. Liang, C.J. and M.C. Lai, Trichloroethylene degradation by zero valent iron activated persulfate oxidation. Environmental Engineering Science, 2008. 25(7), 1071-1077. 103. Lv, X.S., J. Xu, G.M. Jiang, and X.H. Xu, Removal of chromium(VI) from wastewater by nanoscale zero-valent iron particles supported on multiwalled carbon nanotubes. Chemosphere, 2011. 85(7), 1204-1209. 104. Chen, F., Y. Li, W.D. Cai, and J.L. Zhang, Preparation and sono-Fenton performance of 4A-zeolite supported alpha-Fe2O3. Journal of Hazardous Materials, 2010. 177(1-3), 743-749. 105. Maiti, A., J.K. Basu, and S. De, Development of a Treated Laterite for Arsenic Adsorption: Effects of Treatment Parameters. Industrial & Engineering Chemistry Research, 2010. 49(10), 4873-4886. 106. Chen, A.H., H.Q. Wang, and X.Y. Li, Influence of concentration of FeCl3 solution on properties of polypyrrole-Fe3O4 composites prepared by common ion absorption effect. Synthetic Metals, 2004. 145(2-3), 153-157. 107. 林宗龍, 利用活性碳催化過硫酸鹽在室溫下氧化全氟辛酸之研究. 國立台灣大學環境工程學研究所, 2012. 108. Liang, C., Y.Y. Guo, and Y.R. Pan, A study of the applicability of various activated persulfate processes for the treatment of 2,4-dichlorophenoxyacetic acid. International Journal of Environmental Science and Technology, 2014. 11(2), 483-492. 109. Lee, Y.C., S.L. Lo, P.T. Chiueh, and D.G. Chang, Efficient decomposition of perfluorocarboxylic acids in aqueous solution using microwave-induced persulfate. Water Research, 2009. 43(11), 2811-2816. 110. Hao, F.F., L.L. Guo, A.Q. Wang, Y.Q. Leng, and H.L. Li, Intensification of sonochemical degradation of ammonium perfluorooctanoate by persulfate oxidant. Ultrasonics Sonochemistry, 2014. 21(2), 554-558. 111. Yang, S.W., J.H. Cheng, J. Sun, Y.Y. Hu, and X.Y. Liang, Defluorination of Aqueous Perfluorooctanesulfonate by Activated Persulfate Oxidation. Plos One, 2013. 8(10). 112. Liang, C.J., C.J. Bruell, M.C. Marley, and K.L. Sperry, Persulfate oxidation for in situ remediation of TCE. I. Activated by ferrous ion with and without a persulfate-thiosulfate redox couple. Chemosphere, 2004. 55(9), 1213-1223. 113. Long, A.H., Y. Lei, and H. Zhang, Degradation of Toluene by a Selective Ferrous Ion Activated Persulfate Oxidation Process. Industrial & Engineering Chemistry Research, 2014. 53(3), 1033-1039. 114. Zhou, L., W. Zheng, Y.F. Ji, J.F. Zhang, C. Zeng, Y. Zhang, Q. Wang, and X. Yang, Ferrous-activated persulfate oxidation of arsenic(III) and diuron in aquatic system. Journal of Hazardous Materials, 2013. 263, 422-430. 115. Hussain, I., Y.Q. Zhang, and S.B. Huang, Degradation of aniline with zero-valent iron as an activator of persulfate in aqueous solution. Rsc Advances, 2014. 4(7), 3502-3511. 116. Ji, Y.F., C. Ferronato, A. Salvador, X. Yang, and J.M. Chovelon, Degradation of ciprofloxacin and sulfamethoxazole by ferrous-activated persulfate: Implications for remediation of groundwater contaminated by antibiotics. Science of the Total Environment, 2014. 472, 800-808. 117. Hussain, I., Y.Q. Zhang, S.B. Huang, and X.Z. Du, Degradation of p-chloroaniline by persulfate activated with zero-valent iron. Chemical Engineering Journal, 2012. 203, 269-276. 118. Xu, X.R. and X.Z. Li, Degradation of azo dye Orange G in aqueous solutions by persulfate with ferrous ion. Separation and Purification Technology, 2010. 72(1), 105-111. 119. Tan, C.Q., N.Y. Gao, Y. Deng, N. An, and J. Deng, Heat-activated persulfate oxidation of diuron in water. Chemical Engineering Journal, 2012. 203, 294-300. 120. Furukawa, Y., J.W. Kim, J. Watkins, and R.T. Wilkin, Formation of ferrihydrite and associated iron corrosion products in permeable reactive barriers of zero-valent iron. Environmental Science & Technology, 2002. 36(24), 5469-5475. 121. Ahmad, M., A.L. Teel, O.S. Furman, J.I. Reed, and R.J. Watts, Oxidative and Reductive Pathways in Iron-Ethylenediaminetetraacetic Acid-Activated Persulfate Systems. Journal of Environmental Engineering-Asce, 2012. 138(4), 411-418. 122. Patil, S.F., A.G. Bedekar, and R.M. Patil, Gamma-Radiolysis of Isobutanol and Nitrate in Aqueous-Solution. Journal of Radioanalytical and Nuclear Chemistry-Articles, 1992. 158(1), 107-114. 123. Vicente, F., A. Santos, A. Romero, and S. Rodriguez, Kinetic study of diuron oxidation and mineralization by persulphate: Effects of temperature, oxidant concentration and iron dosage method. Chemical Engineering Journal, 2011. 170(1), 127-135. 124. Mark, G., M.N. Schuchmann, H.P. Schuchmann, and C. Vonsonntag, The Photolysis of Potassium Peroxodisulfate in Aqueous-Solution in the Presence of Tert-Butanol - a Simple Actinometer for 254 Nm Radiation. Journal of Photochemistry and Photobiology a-Chemistry, 1990. 55(2), 157-168. 125. Lin, H., J.F. Niu, S.Y. Ding, and L.L. Zhang, Electrochemical degradation of perfluorooctanoic acid (PFOA) by Ti/SnO2-Sb, Ti/SnO2-Sb/PbO2 and Ti/SnO2-Sb/MnO2 anodes. Water Research, 2012. 46(7), 2281-2289. 126. Kusic, H., I. Peternel, S. Ukic, N. Koprivanac, T. Bolanca, S. Papic, and A.L. Bozic, Modeling of iron activated persulfate oxidation treating reactive azo dye in water matrix. Chemical Engineering Journal, 2011. 172(1), 109-121. 127. Al-Shamsi, M.A. and N.R. Thomson, Treatment of Organic Compounds by Activated Persulfate Using Nanoscale Zerovalent Iron. Industrial & Engineering Chemistry Research, 2013. 52(38), 13564-13571. | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/16711 | - |
| dc.description.abstract | This study was focused on PFOA decomposition in persulfate solution catalyzed iron-modified activated carbon. to by Fe/AC to decompose PFOA. With the process impregnation and calcination, the redox state Fe covered on AC can promote the generation of sulfate radicals and the elevation of decomposition of PFOA. In order to explore the different factors influence the performance, experiments were designed for the effect of pesulfate dosage, Fe/AC dose, Fe covered ratio, pH, temperature, ferrous ion and the radical inhibitors.
The decomposition and defluorination efficiency of PFOA were higher in Fe/AC-PS system than that of PS system. Moreover, the PFOA removals increased with the increasing PS dosage. For the experiments of Fe/AC dose and Fe covered ratio, results indicated that the decomposition and defluorination efficiency of PFOA improved with the promotion of Fe/AC dose and Fe ratio but decreased if the amounts were excess. Under neutral condition, PFOA decomposition efficiency was better than that in acidic condition because too much sulfate radicals produced would hinder the oxidation, and the worst in base conditions due to the suppression by OH-. Compared the efficiency of catalysis by Fe2+ and Fe/AC, experiments results illustrated that Fe/AC is more effective based on the function of catalysis as well as adsorption. The tert-Butanol served as the radical inhibitor that result in the decline of the decomposition and defluorination efficiency of PFOA. It proved that tert-Butanol can scavenge the sulfate radicals. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-07T23:44:11Z (GMT). No. of bitstreams: 1 ntu-103-R01541113-1.pdf: 3464308 bytes, checksum: 595e8c52763a9ff86f0e951c1c581900 (MD5) Previous issue date: 2014 | en |
| dc.description.tableofcontents | 口試委員審定書 i
誌謝 ii 摘要 iii Abstract iv 目錄 v 圖目錄 ix 表目錄 xi 第一章 緒論 1 1.1前言 1 1.2研究目的 2 1.3研究內容 4 第二章 文獻回顧 5 2.1 PFCs危害性與污染特性 5 2.1.1 PFCs之基本性質 5 2.1.2 PFOA之化合物特性 6 2.1.3 PFOA之產源及環境宿命 8 2.1.4 PFOA對人體和生物體影響 10 2.1.5 國內PFOA與PFOS管制狀況 11 2.2 PFCs之處理技術 12 2.2.1高溫燃燒法 12 2.2.2高級氧化法 12 2.2.3光化學氧化法 14 2.2.4超音波化學氧化法 15 2.2.5活性碳吸附法 16 2.3過硫酸鹽氧化劑 18 2.3.1過硫酸鹽種類與ISCO使用 19 2.3.2過硫酸鹽溶解於水中反應 20 2.3.3其它催化過硫酸鹽之方法 22 2.3.4過硫酸鹽實際應用 23 2.4活性碳吸附理論及催化氧化劑機制和應用 26 2.4.1活性碳吸附理論 26 2.4.2活性碳等溫吸附模式 26 2.4.3活性碳吸附動力模式 27 2.4.4活性碳改質 29 2.4.5活性碳催化氧化劑機制及實際應用 30 第三章 實驗方法與材料 33 3.1研究架構 33 3.2實驗試劑 35 3.3鐵改質活性碳製備 36 3.4實驗分析方法 36 3.4.1高效液相層析儀 36 3.4.2離子層析儀 38 3.4.3場發射掃描式電子顯微鏡 39 3.4.4比表面積與孔徑分析儀 39 3.4.5 XRD粉末繞射分析儀 41 3.5 PFOA降解實驗步驟 41 3.6 PFOA降解實驗操作參數 42 3.6.1過硫酸鹽濃度影響試驗 42 3.6.2鐵改質活性碳劑量影響試驗 42 3.6.3鐵披覆活性碳比例影響試驗 42 3.6.4 pH值影響試驗 43 3.6.5溫度影響試驗 43 3.6.6亞鐵離子催化與Fe/AC催化影響比較 43 3.6.7自由基抑制劑影響試驗 43 第四章 結果與討論 44 4.1背景實驗 44 4.2鐵改質活性碳特性分析 46 4.2.1掃描式電子顯微鏡分析 46 4.2.2 XRD粉末繞射、BET與界達電位探討 52 4.3過硫酸鹽濃度效應 54 4.3.1過硫酸鹽系統 54 4.3.2鐵改質活性碳結合過硫酸鹽系統 55 4.4鐵改質活性碳添加劑量效應 63 4.5鐵披覆活性碳比例效應 70 4.6 pH及溫度效應 73 4.6.1 pH效應 73 4.6.2溫度效應 76 4.7亞鐵離子催化結合系統降解效應比較 78 4.8自由基抑制劑對PFOA降解影響 80 4.9 結合系統機制探討 83 4.9.1 PFOA礦化機制 83 4.9.2降解系統機制 84 第五章 結論與建議 85 5.1結論 85 5.2建議 86 參考文獻 87 附錄 98 | |
| dc.language.iso | zh-TW | |
| dc.subject | 鐵改質活性碳 | zh_TW |
| dc.subject | 全氟辛酸 | zh_TW |
| dc.subject | 過硫酸鹽 | zh_TW |
| dc.subject | 催化 | zh_TW |
| dc.subject | 亞鐵離子 | zh_TW |
| dc.subject | PFOA | en |
| dc.subject | ferrous ion | en |
| dc.subject | catalysis | en |
| dc.subject | iron-modified activated carbon | en |
| dc.subject | persulfate | en |
| dc.title | 以鐵改質活性碳結合過硫酸鹽系統降解全氟辛酸之研究 | zh_TW |
| dc.title | Decompositions of PFOA in Persulfate solution catalyzed by Iron-Modified Activated Carbon | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 102-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 林郁真,胡景堯 | |
| dc.subject.keyword | 全氟辛酸,過硫酸鹽,鐵改質活性碳,催化,亞鐵離子, | zh_TW |
| dc.subject.keyword | PFOA,persulfate,iron-modified activated carbon,catalysis,ferrous ion, | en |
| dc.relation.page | 102 | |
| dc.rights.note | 未授權 | |
| dc.date.accepted | 2014-07-11 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| 顯示於系所單位： | 環境工程學研究所 | |
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