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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 柳中明(Chung-Ming Liu) | |
dc.contributor.author | Chong-En Peng | en |
dc.contributor.author | 彭眾恩 | zh_TW |
dc.date.accessioned | 2021-05-20T20:12:57Z | - |
dc.date.available | 2009-07-28 | |
dc.date.available | 2021-05-20T20:12:57Z | - |
dc.date.copyright | 2009-07-28 | |
dc.date.issued | 2009 | |
dc.date.submitted | 2009-07-23 | |
dc.identifier.citation | 王作台、胡志文、林松錦、柳中明,1994:氣象環流對背影氣成份傳送影響:第一部分:軌跡方法之建立及個案分析結果。大氣科學,22,57-76。
吳承翰,2002:亞洲沙塵暴之模擬,國立中央大學,大氣物理研究所碩士論文。 柳中明,1992:台灣背景大氣研究:(1)中美合作「氣候與空氣品質台灣站(CATS)研究發展與西太平洋地區觀測(PEM-west)研究計劃及背景大氣中甲烷(CH4)測量分析」。NSC810421M0023224z。 柳中明,張修武,劉紹臣,1999:蘭嶼背景大氣監測初析。大氣科學,27,99-130。 柳中明,葉銘德,彭立新,吳俊傑,劉紹臣,2004: 冬夏季長程傳送影響台灣海 域背景臭氧之模擬探討。大氣科學,32,1-21。 柳中明,商俊盛,陳瑋蘭,葉銘德,2005:1995-2004 年蘭嶼背景臭氧濃度分析。 氣候變遷與永續發展研討會。 陳進煌,1995:氣流軌跡模式在大氣污染物長程輸送上之運用,國立中央大學,大氣物理研究所碩士論文。 劉紹臣,2005:亞洲沙塵及污染物對台灣空氣品質之影響。中央研究院週報,1041,11-14。 鄭福田、張時禹、黃賀春、張艮輝、劉遵賢,2000:台灣空氣品質模式(Taiwan Air Quality Model)操作使用手冊。 Abdalmogith , S.S., and R.M. Harrison, 2005: The use of trajectory cluster analysis to examine the long-range transport of secondary inorganic aerosol in the UK, Atmospheric Environment 39, pp. 6686–6695. Akimoto, H., 2003: Global Air Quality and Pollution, Science, 302, 1716-1719. Anthes, R. A., and T.T. Warner, 1978:Development of hydro-dynamical models suitable for air pollution and other mesometeorological studies. Mon. Wea. Rev., 106, 1045-1078 Anderberg, M.R., 1973: Cluster Analysis for Applications, Academic Press, p. 48–52. Avila, A., and M. Alarcón., 1999: Relationship between precipitation chemistry and meteorological situations at a rural site in NE Spain. Atmospheric Environment 33, pp. 1663–1677. Blake, J., G. W. Sachse, J. E. Collins, Jr., B. G. Heikes, J. T. Merrill, G. L. Gregory, B. E. Anderson, H. B. Singh, D. C. Thornton, A. R. Brady, and R. F. Pueschel, 1997: Chemical characteristics of continental outflow from Asia to the troposphere over the western Pacific Ocean during February-March, 1994:Results from PEM-West B. J. Geophys. Res., 102, 28,255-28,274. Cape, J.N., J. Methven, L.E. Hudson, , 2000: The use of trajectory cluster analysis to interpret trace gas measurements at Mace Head, Ireland. Atmospheric Environment 34, 3651–3663. Chameides, W. L., and D. H. Stedman, 1977: Tropospheric ozone: Coupling transport and chemistry, J. Geophys. Res., 82, 1787–1794. Chan, C.Y., Chan, L.Y., Lam, K.S., Li, Y.S., Harris, J.M. and Oltmans, S.J., 2002: Effects of Asian air pollution transport and photochemistry on carbon monoxide variability and ozone production in coastal South China at Hong Kong, J. Geophys. Res., 107(0), 4746. Clatworthy, J., Buick, D., Hankins, M., Weinman, J., & Horne, R. (2005). The use and reporting of cluster analysis in health psychology: A review. British Journal of Health Psychology, 10(3), 329–358. Crum, F. X. and D. E. Stevens, 1988: A case study of atmospheric blocking using isentropic analysis. Mon. Wea. Rev., 116, 223-241. Crutzen, P. J., 2003: A discussion of the chemistry of some minor constituents in the stratosphere and troposphere, Pure Appl. Geophys., 106–108, 1385–1394. Danielsen, E. F., and V. Mohnen, 1977: Project Duststorm: Ozone transport in situ measurements and meteorological analysis of tropopause folding, J. Geophys. Res., 82, 5867–5877. Draxler, R.R., and G. D. Hess, 1998: An overview of the HYSPLITp4 modelling system for trajectories, dispersion, and deposition. Aust.Meteor. Mag., 47, 295–308. Draxler, R.R., and G. D. Rolph, cited 2003: NOAA ARL HYSPLIT Model. NOAA Air Resources Laboratory. (Available online at http://www.arl.noaa.gov/ ready/hysplit4.html.) Draxler, R.R., Hess, G.D., 2004: Description of the Hysplit_4 Modeling System. NOAA Technical Memorandum ERL ARL-224, 25pp. Dudhia, J., 1993: A nonhydrostatic version of the Penn State-NCAR meso-scale model: Validation tests and simulation of an Atlantic cyclone and the cold front. Mon. Wea. Rev., 121, 1493-1513. Eisen, M., Spellman, P.T., Brown, P.O. & Botstein, D. 1998: Cluster analysis and display of genome-wide expression patterns. Proc. Natl Acad. Sci. USA 95, 14863–14868. Everitt BL. 1980: Ecology of saltcedar: a plea for research. Environmental Geology 3(2): 77–84. Fabian, P., and P. G. Pruchniewicz, 1977: Meridional distribution of ozone in the troposphere and its seasonal variations, J. Geophys. Res., 82, 2063–2073. Fiore, A., D.J. Jacob, H. Liu, R.M. Yantosca, T.D. Fairlie, Q. Li, 2003: Variability in surface ozone background over the United States: Implications for air quality policy. J. Geophys. Res., 108, 4787. Fishman, J., and P. J. Crutzen, 1977: The origin of ozone in the troposphere, Nature, 274, 855-858. Fishman, J., S. Solomon, and P. J. Crutzen, 1979: Observational and theoretical evidence in support of a significant in-situ photochemical source of tropospheric ozone, Tellus, 31,432– 446. Fuglestvedt, J. S., and J. E. Johnson, 1994: Effects of reductions in stratospheric ozone on tropospheric chemistry through changes in photolysis rates, Tellus, Ser. B, 46, 172–192. Gong, X. and M.B. Richman, 1995: On the application of cluster analysis to growing season precipitation data in North America east of the Rockies. J. Climate, 8: 891-931. Gregory, G. L., J. T. Merrill, M. C. Shipham, D. R. Blake, G. W. Sachse, and H. B. Singh, 1997: Chemical characteristics of tropospheric air over the Pacific Ocean as measured during PEM-west B: Relationship to Asian outflow and trajectory history. J. Geophys. Res., 102,28,275-28,286. Hafner, W.D., N.N. Solorzano, D.A. Jaffe, 2007:Analysis of rainfall and fine aerosol data using clustered analysis for National Park sites in the Western US. Atmospheric Environment, 41, 3071~3081. Harris, J. M. and Kahl, J. D. (1990) A descriptive atmospheric transport climatology for the Mauna Loa Observatory,using clustered trajectories. Journal of Geophysical Research 95, 13,651-13,667. Heald, C.L., Jacob, D.J., Fiore, A.M., Emmons, L.K., Gille, J.C., Deeter, M.N., Warner, J., Edwards, D.P., Crawford, J.H., Hamlin, A.J., Sachse, G.W., Browell, E.V., Avery, M.A., Vay, S.A., Westberg, D.J., Blake, D.R., Singh, H.B., Sandholm, S.T., Talbot, R.W., Fuelberg, H.E., 2003: Asian outflow and transpacific transport of carbon monoxide and ozone pollution: an integrated satellite, aircraft and model perspective. J. Geophys. Res. 108 (D24), 4804. Hoell, J. M., D. D. Davis, S. C. Liu, R. E. Newell, M. Shipham, H. Akimoto, R. J. McNeal, R. J. Bendura, and J. W. Drewry, 1996: The Pacific Exploratory Mission-West Phase A:September –October 1991. J. Geophys. Res., 101, 1641-1653. Hoell, J. M., D. D. Davis, S. C. Liu, R. E. Newell, H. Akimoto, R. J. McNeal and R. J. Bendura, 1997: The Pacific Exploratory Mission-West Phase B:February-March, 1994. J. Geophys Res., 102, 28,223-28,239. Holton, J. R., P. H. Haynes, M. E. McIntyre, A. R. Douglass, R. R. Rood, and L. Pfister, 1995: Stratosphere-troposphere exchange, Rev. Geophys., 33,403–439. Johnson, R.A. and Wichern, D.W., 2002: Applied Mulitivariate Statistical Analysis, Prentice Hall. Jorba, O., C. Perez, F. Rocandenbosch, and J.M. Baldasano, 2004: Cluster Analysis of 4-day Back-Trajectories Arriving into Barcelona Area (Spain) from 1997 to 2002. J. Appl, Meteor., 43, 887–901. Junge, C. E., 1962: Global ozone budget and exchange between stratosphere and troposphere, Tellus, 14, 363- 377. Kappos A. D., and G. Koss, 1990: Health effects of ozone as component of summer smog. Offentl Gesundheitswes, 53, 16-22. Liu C. M., M. P. Buhr, J.-G. Lo, T.-L. Tso, K. J. Hsu, J.-T. Wang, J. T. Merrill and S. C. Liu, 1995: A study of Taiwan background atmosphere. J. Terrestrial Atmos. and Oceanic Sci. (TAO), 6, 419-442. Lin, C.-Y. Lin, S.C. Liu, C. C.-K. Chou, T.H. Liu, C.-T. Lee, C.-S. Yuan, C.-J. Shiu, and C.-Y. Young, 2004: Long-Range Transport of Asian Dust and Air Pollutants to Taiwan. Terrestrail, Atmosphericand Oceanic Sciences, 15 , 759-784. Lin, C.-Y., Z. Wang, W-N. Chen, S-Y. Chang, C.C.K. Chou, N.Sugimoto and Z. Zhao, 2007: Long-range transport of Asian dust and air pollutants to Taiwan: Observed evidence and model simulation, Atmos. Chem. Phys. 7, 423-434. MacQueen, J., 1967: Some methods for classification and analysis of multivariate observations, Proceedings of the Fifth Berkeley Symposium on Mathematical Statistics and Probability. Volume I: Statistics, pages 281-297. Madronich, S., and C. Granier, 1994: Tropospheric chemistry changes due to increased UV-B radiation, in Stratospheric Ozone Depletion/UV-B Radiation in the Biosphere, NATO ASI Ser., Ser. I, 18, edited by R.H. Biggs and M. E. B. Joyne, pp. 3–10. McConnell R, Berhane K, Gilliland F, 2002. Asthma in exercising children exposed to ozone: a cohort study. Lancet 2002; 359: 386–91. Moody, J. L., 1986: The influence of meteorology on precipitation chemistry at selected sites in the Eastern United States. Ph.D. dissertation, University of Michigan, 176 pp. Moody, and J. N. Galloway, 1988: Quantifying the relationship between atmospheric transport and the chemical composition of precipitation on Bermuda. Tellus, 40, 463–479. Punj G., and David W. Stewart, 1983: Cluster analysis in marketing research: review and suggestions for application, Journal of Marketing Research, 20, No. 2, pp.134-148. Rolph, G, D., 2003: Real-time Environmental Applications and Display sYstem(READY) Website (http://www.arl.noaa.gov/ready/HYSPLIT4.html). Sillman, S., and P. J. Samson, 1995: Impact of temperature on oxidant photochemistry in urban, polluted rural and remote environments, J. Geophys. Res., 100, 11,497–11,508. Stockwell, W.R.., Middleton, P., Chang, J.S., 1990: The second generation regional acid deposition model chemical mechanism for regional air quality modeling. J. Geophys. Res. 95 (D10), 16343-16367. Stohl, A. and Wotawa, G. 1995: A method for computing single trajectories representing boundary layer transport. Atmospheric Environment, 29, 3235~3239. Stohl, A., 1998: Computation, accuracy and applications of trajectories—A review and bibliography. Atmos. Environ., 32, 947–966. Streets, D.G., Bond, T.C., Carmichael, G.R., Fernandes, S.D., Fu, Q., He, D., Klimont, Z., Nelson, S.M., Tsai, N.Y., Wang, M.Q., Woo, J.-H., Yarber, K.F., 2003: An inventory of gaseous and primary aerosol emissions in Asia in the year 2000: J. Geophys. Res. 108 (D21), 8809. Talbot, R. W., J. E. Dibb, K. I. Klemm, J. D. Bradshaw, S. T. Sandholm, D. R. Blake, G. W. Sachse, J. Collins, B. G. Heikes, G. L. Gregory, B. E. Anderson, H. B. Singh, D. C. Thornton, and J. T. Merrill, 1996: Chemical characteristics of continental outflow from Asia to the troposphere over the western Pacific Ocean during September-October 1991: Results from PEM-West A. J. Geophys Res., 101, 1713-1726. Unal, Y., Kındap, T. and Karaca, M., 2003: 'Redefining Climate Zones for Turkey Using Cluster Analysis', International Journal of Climatology, 23, 1045 - 1055. Vukovich, F. M., W. D. Bach, B. W. Crissman, and W. J. King, 1977: On the relationship between high ozone in the rural surface layer and high pressure systems, Atmos. Environ., 11, 967-983. Woo, J.-M., Streets, D., Carmichael, G.R., Tang, Y., Yoo, B.-I., Lee, W.-C., Thongboonchoo,N., Pinnock, S., Kurata, G., Uno, I., Fu, Q., Vay, S., Sachse, G.W., Blake, D.R., Fried, A., Thornton, D.C., 2003: The contribution of biomass and biofuel emissions to trace gas distributions in Asia during the TRACE-P experiment. J. Geophys. Res. 108 (D21), 8812. Harvard Atmospheric Chemistry Modeling Group http://acmg.seas.harvard.edu/ NOAA ERL: Physical Sciences Division:Daily Mean Composite http://www.cdc.noaa.gov/data/composites/day | |
dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/9206 | - |
dc.description.abstract | 蘭嶼背景大氣測站(22°02‘N,121°33’E,324公尺高)自1995年開始進行臭氧之監測。柳(1999)曾指出,臭氧為最能反應季節性氣團變動之大氣化學物質:冬季乾冷北風攜帶高濃度臭氧,而夏季海洋暖濕南風伴隨低濃度臭氧。為了延續先前之議題,進一步了解臭氧和空氣來源的關係,本研究利用群集分析,配合蘭嶼臭氧夜間觀測資料,期求客觀量化分析台灣地區空氣來源分布及隨時間之變化,尋找1995-2007年間變化特徵,並觀察與臭氧濃度間之關聯性。
群集分析(Cluster analysis)為多變數分析方法,其目的是希望利用客觀計量,將事物根據某些屬性歸在各群體中,使同一集群內的事物都具有高度同質性(Homogeneity)。我們利用群集分析中K-means法進行改良來進行分群,最終得到六主要族群:A:從西北方來之族群 (佔全部來源之15%),B:從北方來之族群 (17%),C:從北北東方來之族群 (13%),D:從東北方來之族群 (6%),E:從東方來之族群 (23%),F:從西南方來之族群 (21%)。 時間分佈上,依季節區分,冬季主要以大陸性族群A、B為主,夏季則以海洋性族群E、F為主,族群C、D則在秋季較盛行。比對空氣胞族群和蘭嶼臭氧含量,發現族群A、B臭氧含量較高,平均超過45ppbv,族群C、D略低,平均達為43及36ppbv;族群E、F之臭氧含量則明顯較低,平均分別僅22、23ppbv。 在臭氧值年際變化上,大陸性族群臭氧含量以2002為分界,前半段為上升,後半段為下降;海洋性族群則呈逐年上升趨勢。若依臭氧值高低將各族群再分成三類次族群,可發現高臭氧次族群其路徑較偏向排放源。藉由冬季兩個案模擬,也可發現偏向陸路到達台灣之個案,由於其路徑後期亦受排放源影響,因此抵達蘭嶼時之臭氧值較經由海路路徑的個案高。 | zh_TW |
dc.description.abstract | Lanyu background station (22°02 N, 121°33 E, height:324m) has monitored ozone since 1995. Liu et al.(1999) observed 4-year Lanyu data, indicated that ozone was the best gas to response to seasonal air masses change. In order to continue his research about air sources and ozone background concentration of Taiwan, we used cluster analysis to separate all air parcel trajectories from 1995 to 2007 into groups, to find out the spatial and temporal characteristics of air parcels of Taiwan. We also compared back trajectories groups with background ozone concentration in Lanyu to find out ozone characteristics and long-term change trends of groups.
Cluster Analysis is a multivariate analysis technique that seeks to organize information about variables so that relatively homogeneous groups can be formed. In all methods of clustering, we used K-means method for clustering air parcels to Taiwan, and finally got 6 groups: group A from northwest (accounting for 15% of all trajectories), group B from north (17%), group C from north-northeast (13%), group D from northeast (6%), group E from east (23%), and group F from southwest (21%). From the analysis of seasonal ozone distribution, groups from continental (A、B) prevailed in winter, group from ocean(E、F) prevail in summer, and group C and D prevailed in autumn. Comparing air parcel group with Lanyu ozone, we found that group A and B had larger mean ozone concentration, which was higher than 45 ppbv; the mean ozone concentration of group C and group D was 43ppbv and 36ppbv, respectively; group E and F was evidently lower mean ozone concentration than other groups, only 22 ppbv and 23 ppbv. In terms of ozone yearly trend, there were two phases of continental group: before 2002, ozone concentration increased; after 2002, ozone concentration decreased. Oceanic group had lasting increase trend. According to ozone concentration, we separated each group into three sub-groups. The mean trajectory of high ozone sub-group was closer to emission zone than other two sub-groups. Using case study, we found because the ozone values of trajectories whose routes were near to emission zone still affected by emission when parcels approached Lanyu, ozone concentration of near emission air parcels was higher than air parcels whose routes far from emission zone. | en |
dc.description.provenance | Made available in DSpace on 2021-05-20T20:12:57Z (GMT). No. of bitstreams: 1 ntu-98-R96229003-1.pdf: 4505666 bytes, checksum: 54e85f11241748e2a89e90634a921e36 (MD5) Previous issue date: 2009 | en |
dc.description.tableofcontents | 目錄
第一章:前言: 1 第二章:資料來源 6 2.1 臭氧資料來源 6 2.1.1蘭嶼背景站簡介 6 2.1.2 臭氧資料 7 2.2軌跡線模式HYSPLIT: 7 2.3數值模式 9 2.3.1 中尺度氣象模式MM5 10 2.3.2 台灣空氣品質模式TAQM: 11 第三章:研究方法 14 3.1群集分析簡介及其在空氣胞逆軌跡線上之應用 14 3.2 方法簡介 16 第四章:結果分析 19 4.1 分群結果與空氣胞的時空分佈特性探討 19 4.1.1 空氣胞空間分布特性 19 4.1.2 六類空氣胞典型個案 20 4.1.3 空氣胞來源月份分布特性 21 4.1.4 季節盛行族群特性 22 4.2 各族群所攜帶之臭氧值討論 23 4.3 空氣胞來源與臭氧值的年際變化與相關性探討 25 4.3.1 空氣胞來源與臭氧值年際變化分佈特性 25 4.3.2 空氣胞來源與臭氧值分段年際變化特性 26 4.4 臭氧值分佈與路徑之相關性探討 27 4.5 個案模擬分析 29 4.5.1 071206個案模擬討論 30 4.5.2 050118個案模擬討論 32 4.5.3 討論 34 第五章:結論與展望 35 參考文獻: 37 附表 附圖 | |
dc.language.iso | zh-TW | |
dc.title | 大氣長程傳送對台灣背景臭氧之影響:空氣胞逆軌跡線之群集分析 | zh_TW |
dc.title | Effects of Air Long-range Transport on Background Ozone Concentration in Taiwan: The Cluster Analysis of Air Parcel Back Trajectories | en |
dc.type | Thesis | |
dc.date.schoolyear | 97-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 吳明進(Ming-Chin Wu),龍世俊(Shih-Chun Candice Lung),林沛練(Pay-Liam Lin),程萬里(Wan-Li Cheng) | |
dc.subject.keyword | 長程傳送,背景臭氧,群集分析, | zh_TW |
dc.subject.keyword | long-range transport,background ozone,cluster analysis, | en |
dc.relation.page | 88 | |
dc.rights.note | 同意授權(全球公開) | |
dc.date.accepted | 2009-07-24 | |
dc.contributor.author-college | 理學院 | zh_TW |
dc.contributor.author-dept | 大氣科學研究所 | zh_TW |
顯示於系所單位: | 大氣科學系 |
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