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| ???org.dspace.app.webui.jsptag.ItemTag.dcfield??? | Value | Language |
|---|---|---|
| dc.contributor.advisor | 丁育頡 | zh_TW |
| dc.contributor.advisor | Yu-Chieh Ting | en |
| dc.contributor.author | 朱昱銘 | zh_TW |
| dc.contributor.author | Yu-Ming Chu | en |
| dc.date.accessioned | 2023-10-03T16:19:48Z | - |
| dc.date.available | 2023-11-09 | - |
| dc.date.copyright | 2023-10-03 | - |
| dc.date.issued | 2023 | - |
| dc.date.submitted | 2023-08-04 | - |
| dc.identifier.citation | AL-WABEL, M. I., AL-OMRAN, A., EL-NAGGAR, A. H., NADEEM, M. & USMAN, A. R. A. 2013. Pyrolysis temperature induced changes in characteristics and chemical composition of biochar produced from conocarpus wastes. Bioresource Technology, 131, 374-379.
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/90492 | - |
| dc.description.abstract | 沼渣是厭氧消化的副產物，沼渣中剩餘未消化完全的豐富有機物含量使其具有資源再利用的價值。生物炭是一種具有豐富孔隙結構且富含碳的材料，利用生物質在隔絕氧氣的狀態下熱解製備而成，被視為經濟且環保的廢物處理和碳封存方案，可作為沼渣的去化管道。本研究分別利用豬糞尿沼渣以及豬糞尿與農業廢棄物共消化的沼渣作為作為生產生物炭的原料，經過高溫熱解後製備而成的生物炭，先進行甲苯吸附，再將吸附飽和的生物炭作為燃料使用。
在熱解之前對固體沼渣採用碳酸鉀浸漬的方法進行前處理，用以提升生物炭的表面性質，該方法旨在改善生物炭的孔隙特性和甲苯的吸附能力。生物炭通過慢熱解法在500至800°C的溫度下製備而成。結果表明，透過碳酸鉀浸漬後的沼渣做為原料製備而成的生物炭具有非常高的比表面積，最高達到1673 m2/g，並表現出優異的甲苯吸附能力，最高達到876 mg/g。 在熱解溫度800°C下製備的改質生物炭的淨熱值為8030 kcal/kg，在經過甲苯吸附後，吸附飽和的生物炭的淨熱值提高到9070 kcal/kg，提升了1040 kcal/kg。這一發現表明，生物炭孔隙內所吸附的甲苯可以在作為燃料利用時產生能量，進而增加生物炭整體的淨熱值。沼渣製備生物炭是一種有效的去化方式，不僅可以控制甲苯排放，還能進一步作為固體再生燃料，實現廢棄物再利用和延長生命週期，達成循環經濟的願景。 | zh_TW |
| dc.description.abstract | Digestate is a by-product of anaerobic digestion. The abundance of organic matter content in digestate has generated significant potential for its resource valorization. Biochar is a highly porous and carbon-rich material, which has been seen as an economical and environmentally friendly solution to waste disposal, carbon sequestration, and the treatment of digestate. This study utilized two different types of solid digestate: one derived from pig manure and the other derived from a mixture of pig manure with agricultural waste as the raw materials for producing biochar. Biochar prepared through high-temperature pyrolysis was first employed for the adsorption of toluene, and then the adsorbed saturated biochar was used as fuel.
The modification method of potassium carbonate impregnation was employed on solid digestate prior to pyrolysis as a means to enhance the properties of the biochar. This approach aimed to improve the characteristics of biochar and the performance of adsorption toluene. The biochar was produced through slow pyrolysis at temperatures ranging from 500 to 800°C. The results showed that the biochar produced from digestate exhibited a remarkably high specific surface area, reaching up to 1673 m2/g, and demonstrated excellent toluene adsorption capacity, reaching 876 mg/g. The low heating value (LHV) of modified biochar produced at 800°C was 8030 kcal/kg. After the adsorption of toluene, the LHV of the biochar increased to 9070 kcal/kg, representing a 1040 kcal/kg enhancement. This finding demonstrates that the adsorption of toluene within the pores of biochar can increase LHV. The preparation of biochar from digestate is an effective management of waste treatment that is not only appropriate for the control of toluene emissions but also enables its utilization as a solid renewable fuel, thus facilitating waste reuse and extending its life cycle, thereby achieving the circular economy. | en |
| dc.description.provenance | Submitted by admin ntu (admin@lib.ntu.edu.tw) on 2023-10-03T16:19:48Z No. of bitstreams: 0 | en |
| dc.description.provenance | Made available in DSpace on 2023-10-03T16:19:48Z (GMT). No. of bitstreams: 0 | en |
| dc.description.tableofcontents | 口試委員會審定書 I
誌謝 II 中文摘要 III Abstract IV Content VI List of Figures IX List of Tables XI Chapter 1 Introduction 1 1.1 Background 1 1.2 Motivation 2 Chapter 2 Literature Review 4 2.1 Digestate 4 2.1.1 Sources 5 2.1.2 Restriction and regulations 8 2.2 Biochar 10 2.2.1 Production of biochar 11 2.2.2 Applications of biochar 12 2.2.3 Modification of biochar 13 2.3 Adsorption of toluene 15 2.3.1 Source of toluene 15 2.3.2 Adsorption mechanism 16 2.4 Fuel 18 Chapter 3 Materials and Methods 21 3.1 Research framework 21 3.2 Materials 22 3.2.1 Pretreatment of digestate 22 3.2.2 Preparation of biochar 23 3.3 Characterization 25 3.3.1 Specific Surface Area and Porosimetry Analyzer 25 3.3.2 Proximate analysis 26 3.3.3 Elemental analysis 27 3.3.4 Thermogravimetry – Infrared Spectroscopy (TG-FTIR) 29 3.3.5 Scanning Electron Microscope (SEM) 30 3.4 Adsorption test 30 3.4.1 Toluene generation system 31 3.4.2 Adsorption bed 32 3.4.3 Detector of toluene 33 3.5 Calorimeter 34 3.6 Data analysis 36 Chapter 4 Results and Discussion 37 4.1 Production of biochar 37 4.1.1 Yield and SSA of biochar 37 4.1.2 TG-FTIR analysis 40 4.2 Characterization of biochar 49 4.2.1 Proximate analysis 49 4.2.2 Elemental analysis 50 4.2.3 Pore structures 53 4.2.4 Morphology of biochar 58 4.3 Adsorption of toluene 63 4.4 Biochar as solid fuel 67 4.4.1 Heating value 67 4.4.2 Energy yield 69 Chapter 5 Conclusions and Recommendations 74 5.1 Conclusions 74 5.2 Recommendations 75 References 77 Supplementary Information 90 | - |
| dc.language.iso | en | - |
| dc.subject | 厭氧消化 | zh_TW |
| dc.subject | 生物質增值 | zh_TW |
| dc.subject | 緩慢熱解 | zh_TW |
| dc.subject | VOCs 控制 | zh_TW |
| dc.subject | 廢棄物處理 | zh_TW |
| dc.subject | slow pyrolysis | en |
| dc.subject | biomass valorization | en |
| dc.subject | VOCs control | en |
| dc.subject | anaerobic digestion | en |
| dc.subject | waste disposal | en |
| dc.title | 沼渣生物炭在甲苯吸附與固體再生燃料的應用 | zh_TW |
| dc.title | Toluene adsorption using biochar derived from solid digestate and the utilization for solid recovered fuel | en |
| dc.type | Thesis | - |
| dc.date.schoolyear | 111-2 | - |
| dc.description.degree | 碩士 | - |
| dc.contributor.oralexamcommittee | 張章堂;席行正;林亮毅 | zh_TW |
| dc.contributor.oralexamcommittee | Chang-Tang Chang;Hsing-Cheng Hsi;Liang-Yi Lin | en |
| dc.subject.keyword | 厭氧消化,緩慢熱解,生物質增值,VOCs 控制,廢棄物處理, | zh_TW |
| dc.subject.keyword | anaerobic digestion,slow pyrolysis,biomass valorization,VOCs control,waste disposal, | en |
| dc.relation.page | 90 | - |
| dc.identifier.doi | 10.6342/NTU202302154 | - |
| dc.rights.note | 同意授權(限校園內公開) | - |
| dc.date.accepted | 2023-08-07 | - |
| dc.contributor.author-college | 工學院 | - |
| dc.contributor.author-dept | 環境工程學研究所 | - |
| dc.date.embargo-lift | 2028-07-31 | - |
| Appears in Collections: | 環境工程學研究所 | |
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| ntu-111-2.pdf Restricted Access | 3.8 MB | Adobe PDF | View/Open |
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