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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 駱尚廉(Shang-Lien Lo) | |
| dc.contributor.author | Ting Fang | en |
| dc.contributor.author | 方婷 | zh_TW |
| dc.date.accessioned | 2022-11-25T05:34:47Z | - |
| dc.date.available | 2026-06-24 | |
| dc.date.copyright | 2021-08-18 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-06-24 | |
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International Journal of Refrigeration, 101, 117-124. 錢維億（2020）。以界面活性劑作為水中全氟辛酸之浮除收集劑。臺北醫學大學公共衛生學系暨研究所碩士論文，臺北市。 取自https://hdl.handle.net/11296/vr7qf4 | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/82050 | - |
| dc.description.abstract | "全氟辛酸（Perfluorooctanoic acid , PFOA）為全氟化合物（Perfluorinated chemicals , PFCs）的一種，在1950年代大量被使用，所以其不只在環境中存在，動植物體內、蔬菜水果甚至人體血漿內均存在，因其具有環境持久性及生物累積性而逐漸被重視。流行病學相關研究指出，暴露全氟辛酸可能會造成肝毒性、發育毒性、生殖毒性甚至癌症。 2017年歐盟將全氟辛酸、其鹽類及相關化合物列入REACH法規附17。 2019年舉辦第九屆斯德哥爾摩公約會議，將全氟辛酸、其鹽類及相關化合物列入關於持久性有機污染物的《斯德哥爾摩公約》附件A。 本研究使用電混凝浮除技術（ECF）為電混凝（EC）和電浮除（EF）之結合達到去除含全氟辛酸之廢水，並使用不同種類之界面活性劑為蒐集劑，探討不同條件對全氟辛酸之去除效率影響。研究結果表示，在單極鋁板條件下加入初始濃度為1 mM PFOA，使用癸基三甲基溴化銨（Decyltrimethylammonium Bromide , DTAB）僅需10分鐘反應時間PFOA可達98% 去除，加入加入ZnCl2後可達100%去除。將實驗最佳添加濃度使用於實廠廢水並與自製廢水結果相比較，結果顯示，最佳界面活性劑濃度之添加量及濃度適用於實廠廢水PFOA之去除。 為了解PFOA在電混凝浮除之去除機制，將浮除膠羽使用傅立葉轉換紅外光譜（FTIR）、場發射掃描電子顯微鏡（SEM）、化學分析影像能譜儀（XPS）及X光繞射儀（XRD）進行分析觀察膠羽特徵。從膠羽結果可看到具有Al-F鍵結及Al-O鍵結，推斷膠羽為氫氧化鋁之化合物。最後將探討電混凝浮除之能效（G50），加入DTAB之G50值為2882 g/kWh，其效能遠高於過去文獻的1000倍以上，具經濟可行性。" | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-25T05:34:47Z (GMT). No. of bitstreams: 1 U0001-2206202120541300.pdf: 15079669 bytes, checksum: cc7f836cd243e94234f188dd01f6b908 (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | 致謝 i 摘要 ii Abstract iii 目錄 v 圖目錄 ix 表目錄 xii 第一章 緒論 1 1.1 研究緣起 1 1.2 研究目的 4 1.3 研究內容 4 第二章 文獻回顧 5 2.1 全氟化合物 5 2.1.1 全氟化合物種類及特性 5 2.1.2 全氟辛酸之歷史 8 2.1.3 全氟辛酸相關法令及管制措施 9 2.1.4 全氟化合物毒性 11 2.2 我國全氟化合物現況 15 2.3全氟化合物之處理技術 19 2.3.1 吸附 19 2.2.4 聲化學降解 21 2.3.2 傳統混凝 22 2.3.3泡沫浮除法 24 2.3.4電混凝/電混凝浮除法 26 2.3.1 影響電混凝之參數 29 2.3.2 電混凝運用去除全氟化物 33 2.4界面活性劑 34 2.4.1 界面活性劑之添加對全氟化合物去除之影響 34 2.4.2 界面活性劑之種類及特性 37 第三章 材料與方法 39 3.1 實驗內容與架構 39 3.2 實驗材料與設備 40 3.3 分析方法 45 3.4 實驗步驟與方法 49 3.4.1 背景試驗 49 3.4.2 電混凝浮除試驗 50 3.4.3 PFOA去除率計算 51 3.4.4 半去除率能效(G50)之計算 51 3.4.5 品保品管 52 第四章 結果與討論 53 4.1 背景實驗 53 4.2 添加不同種類之界面活性劑對PFOA去除率之影響 54 4.3 極板數量之影響 56 4.3.1 添加OTAB在單極板和雙極板系統之影響 56 4.3.2 添加DTAB在單極板和雙極板系統之影響 57 4.3.3 添加CTAB在單極板和雙極板系統之影響 58 4.3.4 添加TBAB在單極板和雙極板系統之影響 59 4.4 初始PFOA濃度之影響 61 4.4.1 添加OTAB於不同初始PFOA濃度之影響 61 4.4.2 添加DTAB於不同初始PFOA濃度之影響 62 4.4.3 添加CTAB於不同初始PFOA濃度之影響 63 4.4.4 添加TBAB於不同初始PFOA濃度之影響 64 4.5 電流及鋅鹽之影響 65 4.5.1 在不同電流下添加OTAB及鋅鹽之影響 65 4.5.2 在不同電流下添加DTAB及鋅鹽之影響 66 4.5.3 在不同電流下添加CTAB及鋅鹽之影響 67 4.5.4 在不同電流下添加TBAB及鋅鹽之影響 68 4.6 界面活性劑濃度與濁度和PH之關係 69 4.7 界面活性劑最佳添加濃度 73 4.8 實廠廢水去除效果 74 4.8.1 在實廠廢水加入OTAB對去除率之影響 75 4.8.2 在實廠廢水加入DTAB對去除率之影響 76 4.8.3 在實廠廢水加入CTAB對去除率之影響 77 4.8.4 在實廠廢水加入TBAB對去除率之影響 78 4.9 電混凝浮除後之膠羽分析 79 4.9.1 場發射電子顯微鏡/能量色散X射線光譜儀 80 4.9.2 傅立葉紅外光譜儀分析儀 83 4.9.3 X射線光電子能譜儀分析儀 88 4.9.4 X光繞射儀分析儀 93 4.10 添加不同種類之界面活性劑能效比較 95 4.11 各PFOA降解方法之能效(G50)比較 97 第五章 結論與建議 98 5.1 結論 98 5.2 建議 100 參考文獻 101 附錄 111 | |
| dc.language.iso | zh-TW | |
| dc.subject | 氫氧化物膠羽 | zh_TW |
| dc.subject | 全氟辛酸（PFOA） | zh_TW |
| dc.subject | 界面活性劑 | zh_TW |
| dc.subject | 電混凝浮除法 | zh_TW |
| dc.subject | 半去除率能效（G50） | zh_TW |
| dc.subject | perfluorooctanoic acid (PFOA) | en |
| dc.subject | Hydroxide flocs | en |
| dc.subject | energy yield for 50% removal (G50) | en |
| dc.subject | electrocoagulation-flotation method (ECF) | en |
| dc.subject | surfactant | en |
| dc.title | 以電混凝浮除法去除水中之全氟辛酸（PFOA） | zh_TW |
| dc.title | Removal of Perfluorooctanoic Acid（PFOA）by Electrocoagulation-flotation from Water | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 郭繼汾(Hsin-Tsai Liu),胡景堯(Chih-Yang Tseng) | |
| dc.subject.keyword | 全氟辛酸（PFOA）,界面活性劑,電混凝浮除法,半去除率能效（G50）,氫氧化物膠羽, | zh_TW |
| dc.subject.keyword | perfluorooctanoic acid (PFOA),surfactant,electrocoagulation-flotation method (ECF),energy yield for 50% removal (G50),Hydroxide flocs, | en |
| dc.relation.page | 127 | |
| dc.identifier.doi | 10.6342/NTU202101099 | |
| dc.rights.note | 同意授權(限校園內公開) | |
| dc.date.accepted | 2021-06-25 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| dc.date.embargo-lift | 2026-06-25 | - |
| 顯示於系所單位： | 環境工程學研究所 | |
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