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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 于昌平(Chang-Ping yu) | |
| dc.contributor.author | I-Chi Hing | en |
| dc.contributor.author | 洪意琦 | zh_TW |
| dc.date.accessioned | 2022-11-25T03:05:19Z | - |
| dc.date.available | 2023-06-30 | |
| dc.date.copyright | 2021-08-18 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-06-25 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/81863 | - |
| dc.description.abstract | 隨著人口急速增加，使科技與經濟發展的追求造成了許多環境問題，水資源與能源議題逐漸受到關注與重視。由於能源需求的增加與化石燃料的減少，人們開始追求低成本且可持續供應的能源，以及如何將能源更為有效地儲存並利用。電極材料在電能儲存系統中的效能佔有重要影響，透過電極之改良能大幅提升產電與儲能的效率。然而，傳統之電池廢棄物導致嚴重的環境問題，為此生物衍生材料其較為安全、經濟和環境友好的特性，被認為是可進一步研究之電極材料。 真菌可在嚴峻環境下生長，具有極高的適應性，因此被認為應用於生物處理是新穎且有潛力的方法之一。本研究透過兩種真菌分離株，分別是Fusarium solani 與 Clonostachys rosea，將其暴露於高濃度重金屬進行一系列誘導耐受性培訓，以確定通過持續暴露可培養出更大的耐受性，並觀察活真菌細胞對水中重金屬與硝酸鹽氮去除情形以及製備由真菌菌絲衍生的熱碳化電極。在培養過程中添加重金屬，於生物吸附的機制過程中摻雜金屬發揮真菌生物模板的特性，此外真菌還具有碳、氮、磷與氧等元素組成也可作為雜原子摻雜並有效地增強及改善生物質衍生電極的電化學性能。結果顯示：(1) 在經過誘導性耐受度訓練後，F. solani與C. rosea分別對鎳與鈷表現出更高的耐受性。(2) F. solani與C. rosea對於初始濃度50 mg/L的銅分別有80.33%與80.81%之去除效率。(3) F. solani與C. rosea皆可利用反硝化作用，硝酸根去除效率分別達到99.9%與98.7%。(4) 真菌生物質生長時添加選定重金屬改性真菌碳質電極，在0.1 A/g下比電容值(106.4 F/g)最高提升了2.3倍且具有良好的實驗穩定性。本研究結果證實：真菌的生物質除了可作為一種去除重金屬與硝酸鹽氮的一項多功能水處理技術，擁有良好之處理效果與永續發展的可能性，也可作為真菌熱碳化電極，並以生物模板的特性於生長過程中提升電化學效能，增加生物性衍生材料電極其運用於其他電化學處理程序之應用潛力。 | zh_TW |
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| dc.description.tableofcontents | 口試委員會審定書 I 致謝 III 摘要 V Abstract VI 目錄 IX 圖目錄 XI 表目錄 XIII 第一章 緒論 1 1.1. 研究背景 1 1.2. 研究動機 2 1.3. 研究目的 3 第二章 文獻回顧 4 2.1. 重金屬的危害與處理技術 4 2.1.1. 重金屬之危害 4 2.1.2. 廢水中重金屬之常見處理技術 6 2.1.3. 廢水中重金屬去除的生物處理 7 2.3. 真菌與金屬間之相互作用 8 2.3.1. 微生物與金屬之間的相互作用 8 2.3.2. 真菌對金屬之耐受性 10 2.4. 真菌應用於廢水處理技術 13 2.4.1. 去除水中重金屬 13 2.4.2. 去除水中硝酸鹽 15 2.4.3. 其他常見廢水處理 17 2.5. 生物衍生材料 18 2.5.1. 生物衍生材料之沿革 18 2.5.2. 真菌衍生電極材料 19 第三章 材料與方法 21 3.1. 實驗藥品與設備 21 3.1.1. 實驗用藥品 21 3.1.2. 實驗設備與儀器 22 3.2. 真菌對金屬之耐受性訓練 23 3.2.1. 真菌菌種來源 23 3.2.2. 馴養與生長條件 24 3.2.3. 耐受性訓練試驗 25 3.3. 真菌去除水中重金屬與硝酸根試驗 27 3.3.1. 活真菌細胞馴養與篩取 27 3.3.2. 活真菌細胞之金屬生物累積能力試驗 28 3.3.3. 真菌去除水中硝酸鹽實驗 30 3.3.4. 感應耦合電漿原子發射光譜儀 31 3.3.5. 離子層析法 31 3.4. 真菌衍生電極材料製備 32 3.5. 電極特性分析 33 3.5.1. 循環伏安法實驗 35 3.5.2. 定電流充放電測試 37 3.5.3. 電化學阻抗分析 39 3.6. 電極之表面特性分析 41 3.6.1. 掃描式電子顯微鏡 41 3.6.2. 能量散射X射線譜 42 3.6.3. 熱重分析 42 3.6.4. 比表面積分析儀 43 第四章 結果與討論 44 4.1. 真菌對於金屬耐受性試驗 44 4.1.1. 耐受性過程真菌菌株表現 44 4.1.2. 金屬存在下真菌於各生長階段之耐受性指數 47 4.1.3. 金屬濃度對真菌之耐受性發展的影響 53 4.2. 金屬之生物累積性試驗 55 4.2.1. 真菌對於各目標金屬濃度之去除效率 55 4.2.2. 金屬吸附量或生物累積量之探討與比較 60 4.2.3. 硝酸根去除 62 4.3. 真菌生物碳電極表面分析 65 4.3.1. 電極之表面形態分析 65 4.3.2. 元素與比表面積分析 68 4.3.3. 熱重分析 70 4.4. 真菌生物碳之電化學特性分析 71 4.4.1. 電化學之定電流充放電分析 71 4.4.2. 電化學分析之循環伏安法 76 4.4.3. 交流阻抗分析 81 第五章 結論與建議 83 5.1. 結論 83 5.2. 建議 85 參考資料 86 | |
| dc.language.iso | zh-TW | |
| dc.subject | 真菌 | zh_TW |
| dc.subject | 電化學 | zh_TW |
| dc.subject | 電極改性 | zh_TW |
| dc.subject | 生物碳材料 | zh_TW |
| dc.subject | 硝酸鹽 | zh_TW |
| dc.subject | 耐受性 | zh_TW |
| dc.subject | electrode modification | en |
| dc.subject | fungi | en |
| dc.subject | bio-carbon materials | en |
| dc.subject | nitrate | en |
| dc.subject | tolerance | en |
| dc.subject | electrochemistry | en |
| dc.title | 利用真菌吸附重金屬以製備生物衍生性電極材料 | zh_TW |
| dc.title | Heavy Metal Adsorbed Fungi for Bio-derived Electrode Materials | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 羅南德(Hsin-Tsai Liu),陳翰儀(Chih-Yang Tseng) | |
| dc.subject.keyword | 真菌,生物碳材料,硝酸鹽,耐受性,電化學,電極改性, | zh_TW |
| dc.subject.keyword | fungi,bio-carbon materials,nitrate,tolerance,electrochemistry,electrode modification, | en |
| dc.relation.page | 94 | |
| dc.identifier.doi | 10.6342/NTU202101123 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2021-06-25 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| dc.date.embargo-lift | 2023-06-30 | - |
| 顯示於系所單位： | 環境工程學研究所 | |
文件中的檔案：
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| U0001-2406202116062200.pdf | 5.25 MB | Adobe PDF | 檢視/開啟 |
系統中的文件，除了特別指名其著作權條款之外，均受到著作權保護，並且保留所有的權利。