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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/80600完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 黃慶怡(Ching-I Huang) | |
| dc.contributor.author | Ming-Yang Chen | en |
| dc.contributor.author | 陳名揚 | zh_TW |
| dc.date.accessioned | 2022-11-24T03:10:25Z | - |
| dc.date.available | 2021-11-04 | |
| dc.date.available | 2022-11-24T03:10:25Z | - |
| dc.date.copyright | 2021-11-04 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-10-25 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/80600 | - |
| dc.description.abstract | 環氧樹脂以其優異的綜合性能在許多領域中得到廣泛應用，為了滿足各領域的應用標準，耐高溫環氧樹脂的開發儼然成為重要的問題。本研究導入電腦模擬技術對耐高溫環氧樹脂的胺類固化劑進行研發，選擇最具代表性的環氧單體DGEBA作為主要系統，尋找具備耐高溫特性的新型固化劑設計方案。我們收集了近二十年來以環氧單體DGEBA及胺類固化劑為主要材料的實驗文獻，透過定量結構性質關係(Quantitative structure-property relationships)技術來建立理論計算值與實驗數據的擬合式，並對其進行基因演算法的分析及材料使用的觀察，得出胺類固化劑分子結構影響環氧樹脂整體Tg值的關鍵因素為分子結構對稱性、分子量、固化劑中氮、氧、硫原子及芳香環數目。藉由這些關鍵因素來提出一系列可能具備耐高溫特性的基團並用於設計新型固化劑，其中觀察到在以蒽環(Anthracene)及萘環(naphthalene)進行結構改質時可以最顯著的提升Tg值；此外，碸基(Sulfone)及醯胺基(Amido)作為連接官能基時，對整體Tg提升也會有明顯的效果，約略提升5~10 K。後續對於所設計的新型固化劑用於環氧樹脂的理論計算Tg值代入擬合式來進行預測，值得注意的是，在新型設計的固化劑中，以非工業級固化劑PABP為參考對象時，可得到最高的預測實驗Tg值在含蒽環及不含蒽環的情況下分別為674 K及598 K，兩者皆遠遠超越我們在文獻收集中最高的530 K。透過本研究對於關鍵因素的探討並將其用於設計新型固化劑的設計策略，達到加速材料開發及降低開發成本的可能性，期許能作為實驗學者在未來研究上的參考依據，並且促進該領域的蓬勃發展。 | zh_TW |
| dc.description.provenance | Made available in DSpace on 2022-11-24T03:10:25Z (GMT). No. of bitstreams: 1 U0001-2210202118104600.pdf: 9771747 bytes, checksum: 49567d7cbef53b7bee6ca67f3e81ed8b (MD5) Previous issue date: 2021 | en |
| dc.description.tableofcontents | 摘要-i ABSTRACT-ii 目錄-iii 圖目錄-iv 表目錄-v 第1章 前言-1 第2章 模擬方法-7 2.1 數據收集-7 2.2 定量結構性質關係：QSPR(Quantitative Structure–Property Relationships)技術-7 2.3 基因演算法(Genetic Algorithm)-9 第3章 結果與討論-11 3.1 DGEBA系統的實驗文獻Tg值與理論計算關係-11 3.2 影響環氧樹脂玻璃轉移溫度之重要參數-18 3.3 設計耐高溫新型固化劑-21 第4章 結論-31 第5章 參考文獻-33 附件一 計算模組Synthia中Tg計算式之相關參數物理意義-38 附件二 各個重要參數與實驗Tg值之關係圖-41 附件三 不含蒽的新型固化劑分子結構及預測Tg值-43 附件四-含蒽的新型固化劑分子結構及預測Tg值-68 | |
| dc.language.iso | zh-TW | |
| dc.subject | 基因演算法 | zh_TW |
| dc.subject | 耐高溫環氧樹脂 | zh_TW |
| dc.subject | 定量結構性質關係 | zh_TW |
| dc.subject | 玻璃轉移溫度 | zh_TW |
| dc.subject | High-temperature resistant epoxy resin | en |
| dc.subject | Glass transition temperature | en |
| dc.subject | Quantitative structure-property relationships | en |
| dc.subject | Genetic algorithm | en |
| dc.title | 運用基因演算法設計應用於耐高溫環氧樹脂之新型固化劑 | zh_TW |
| dc.title | Design of Novel Curing Agents for High Temperature Resistant Epoxy Resins by Genetic Algorithm | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 童世煌(Hsin-Tsai Liu),韓錦鈴(Chih-Yang Tseng),陳錦文,蘭宜康 | |
| dc.subject.keyword | 耐高溫環氧樹脂,玻璃轉移溫度,基因演算法,定量結構性質關係, | zh_TW |
| dc.subject.keyword | High-temperature resistant epoxy resin,Glass transition temperature,Genetic algorithm,Quantitative structure-property relationships, | en |
| dc.relation.page | 72 | |
| dc.identifier.doi | 10.6342/NTU202104049 | |
| dc.rights.note | 同意授權(限校園內公開) | |
| dc.date.accepted | 2021-10-26 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 高分子科學與工程學研究所 | zh_TW |
| 顯示於系所單位： | 高分子科學與工程學研究所 | |
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