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| ???org.dspace.app.webui.jsptag.ItemTag.dcfield??? | Value | Language |
|---|---|---|
| dc.contributor.advisor | 蔣本基(Pen-Chi Chiang) | |
| dc.contributor.author | Chen-Yao Hong | en |
| dc.contributor.author | 洪振耀 | zh_TW |
| dc.date.accessioned | 2022-11-23T09:09:52Z | - |
| dc.date.available | 2021-08-23 | |
| dc.date.available | 2022-11-23T09:09:52Z | - |
| dc.date.copyright | 2021-08-23 | |
| dc.date.issued | 2021 | |
| dc.date.submitted | 2021-08-20 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/79752 | - |
| dc.description.abstract | 自工業革命以來，科技與經濟活動蓬勃發展，大幅的改善與提高的人們的生活品質，然而伴隨著空氣污染物的排放，過去易被忽略的環境與生態問題也逐一浮現，其中，氮氧化物為指標性空氣污染物之一，對於環境與人體的傷害日益受到重視，政府部門所訂定的氮氧化物排放標準逐漸加嚴，也使科學家開始發展更有效率的氮氧化物去除技術。應用超重力旋轉床去除氮氧化物為相當具有潛力的空氣污染控制技術，透過離心力使反應器內產生高質傳的特性，可於一般常溫下操作，也大幅縮減傳統氧化吸收的濕式洗滌法所需要的設備體積。 本研究為利用超重力旋轉填充床進行化學氧化吸收程序去除氮氧化物，過程中包含測試各式氣相與液相藥劑、旋轉床操作條件與高中低濃度污染物負荷於氧化吸收程序中的去除效率。研究結果顯示以一氧化氮為主要成分 ((NO)⁄(NO_X≈0.9)) ，總濃度為200 ppm的氮氧化物，於氣液比20、超重力因子86、氣相氧化劑為二氧化氯與液相吸收劑為亞硫酸鈉的操作條件下，氮氧化物的總去除率達98.99 %；當污染物濃度提高至750 ppm時，以相同的操作條件，氮氧化物的總去除率仍可維持在98 %以上，且尾氣濃度也符合法規排放標準。此外，本研究中也對系統質傳係數進行因次分析，並建立相關的數學模式；另一方面，為了考量此技術於未來實務操作的可能性，對系統進行簡易的能耗評估與成本分析。期盼透過本研究的模組實驗、數學模式與能耗成本分析，提高此技術於實廠中應用的可行性。 | zh_TW |
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| dc.description.tableofcontents | 口試委員會審定書 I 致謝 II 中文摘要 IV Abstract V List of Content VII List of Figure X List of Table XV Comment for Oral Defense XVIII Nomenclature XXIII Chapter 1 Introduction 1–1 1.1 Background 1–1 1.2 Objectives 1–3 Chapter 2 Literature Review 2–1 2.1 Nitrogen Oxides 2–1 2.1.1 Formation and Emission Source about Nitrogen Oxides 2–2 2.1.2 Characteristics and Hazard of Nitrogen Oxides 2–5 2.2 Abatement Technology for Nitrogen Oxides Control 2–8 2.2.1 Technology about Removing Nitrogen Oxides 2–9 2.2.2 Oxidation-Absorption with Gas Phase Agents 2–15 2.2.3 Absorption-Oxidation (Reduction) with Liquid Phase Agents 2–17 2.3 Rotating Packed Bed: Principle and Practice 2–19 2.3.1 Principle: Characteristics and Mass Transfer 2–19 2.3.2 Practice: Application of RPB 2–26 2.4 Cost Benefit Analysis 2–27 Chapter 3 Materials and Methods 3–1 3.1 Research Framework 3–1 3.2 Materials 3–2 3.2.1 Reagents 3–2 3.2.2 Instruments and Equipment 3–4 3.2.3 Apparatus: Rotating Packed Bed 3–8 3.3 Methods 3–10 3.3.1 Experimental Design 3–10 3.3.2 Analytical Techniques 3–16 3.3.3 Cost Analysis 3–19 Chapter 4 Results and Discussion 4–1 4.1 Direct Oxidation Absorption 4–1 4.1.1 Liquid Phase Agents: Absorption-Oxidation (Reduction) 4–2 4.1.2 Gas Phase Agents: Oxidation-Absorption 4–7 4.2 Effects of Operating Parameters on NOX Removal 4–20 4.2.1 Gas-Liquid Ratio 4–20 4.2.2 High-Gravity Factor 4–28 4.3 Enhancement of NOX Removal 4–33 4.3.1 Combination of Gas/Liquid Agents in Process 4–33 4.4 Modeling NOX Removal 4–39 4.4.1 Dimensional Analysis in Mass Transfer 4–39 4.4.2 Applicable Concentration Loading in this System 4–44 4.4.3 Systematic Establishment of RPB Operation Model 4–50 4.5 Energy Consumption and Cost Analysis 4–54 4.5.1 Energy Consumption 4–56 4.5.2 Cost Analysis 4–61 Chapter 5 Conclusions and Recommendations 5–1 5.1 Conclusions 5–1 5.2 Recommendations 5–3 References R-1 Appendix A-1 | |
| dc.language.iso | en | |
| dc.subject | 超重力技術 | zh_TW |
| dc.subject | 氮氧化物控制技術 | zh_TW |
| dc.subject | 旋轉填充床 | zh_TW |
| dc.subject | 氧化吸收程序 | zh_TW |
| dc.subject | 質量傳輸 | zh_TW |
| dc.subject | 成本分析 | zh_TW |
| dc.subject | Rotating packed bed | en |
| dc.subject | Cost analysis | en |
| dc.subject | Oxidation-absorption process | en |
| dc.subject | NOX control technology | en |
| dc.subject | High-gravity technology (HiGee) | en |
| dc.subject | Mass transfer | en |
| dc.title | 利用旋轉填充床進行化學氧化吸收去除氮氧化物之性能評估 | zh_TW |
| dc.title | Performance Evaluation of Nitrogen Oxides Removal Using Chemical Oxidation and Absorption via a Rotating Packed Bed | en |
| dc.date.schoolyear | 109-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.coadvisor | 潘述元(Shu-Yuan Pan) | |
| dc.contributor.oralexamcommittee | 林逸彬(Hsin-Tsai Liu),顧洋(Chih-Yang Tseng),陳奕宏 | |
| dc.subject.keyword | 氮氧化物控制技術,超重力技術,旋轉填充床,氧化吸收程序,質量傳輸,成本分析, | zh_TW |
| dc.subject.keyword | NOX control technology,High-gravity technology (HiGee),Rotating packed bed,Oxidation-absorption process,Mass transfer,Cost analysis, | en |
| dc.relation.page | 139 | |
| dc.identifier.doi | 10.6342/NTU202102462 | |
| dc.rights.note | 同意授權(全球公開) | |
| dc.date.accepted | 2021-08-22 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| Appears in Collections: | 環境工程學研究所 | |
Files in This Item:
| File | Size | Format | |
|---|---|---|---|
| U0001-1808202111550000.pdf | 5.27 MB | Adobe PDF | View/Open |
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