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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 陳奕君(I-Chun Cheng) | |
| dc.contributor.author | Hong-Yi Hu | en |
| dc.contributor.author | 胡弘毅 | zh_TW |
| dc.date.accessioned | 2021-07-11T15:01:14Z | - |
| dc.date.available | 2022-08-23 | |
| dc.date.copyright | 2019-08-23 | |
| dc.date.issued | 2019 | |
| dc.date.submitted | 2019-08-19 | |
| dc.identifier.citation | [1] 沈輝 and 曾祖勤, '太陽能光電技術,' 五南圖書出版股份有限公司, 2008.
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/78512 | - |
| dc.description.abstract | 本研究以噴閥塗佈製備奈米銀線薄膜對電極並搭配低溫燒結之奈米顆粒TiO2電子傳輸層，成功於PEN / ITO基板上開發可撓性平面正規結構鈣鈦礦太陽能電池。接著以短時間紫外光臭氧處理奈米銀線對電極，以提升元件特性。最後，研究可撓性鈣鈦礦太陽能電池在多次彎曲後特性的變化。
研究中奈米銀線對電極以噴閥式塗佈法製備，藉由調控載流氣體(空氣)壓力、噴塗次數與基板加熱溫度對元件進行最佳化。接著，再對奈米銀線對電極面進行紫外光臭氧處理30、60、120與180 s。由電化學阻抗分析顯示，在短時間的紫外光臭氧處理後，奈米銀線/spiro-OMeTAD界面傳輸阻抗有所下降，於處理時間60 s時達到最佳效果，此時元件的能量轉換效率為12.13 %，開路電壓為1.04 V，短路電流密度為19.97 mA/cm2，填充因子為61.5 %；相較於未經紫外光臭氧處理之元件(能量轉換效率11.15 %，開路電壓1.031 V，短路電流密度19.2 mA/cm2與填充因子53.4 %)，效率顯著提升8 %。最後針對紫外光臭氧處理之元件進行彎曲穩定性測試，在經過100次和500次的彎曲後，元件效率仍保持在未彎曲前的94%和75%。 | zh_TW |
| dc.description.abstract | In this study, all-solution processed flexible n-i-p type planar perovskite solar cells were demonstrated by using low-temperature nanoparticle TiO2 electron transpart layers and solution-processed silver nanowires (AgNWs) counter electrodes. Next, an ultraviolet ozone (UVO) treatment was applied to the AgNWs counter electrode to improve the cell performance. Finally, the effect of cyclic bending on the performace of the flexible perovskite cells was investigated.
The deposition of AgNWs was carried out by spray coating with air as carrier gas. The optimization paramters include: the pressure of the carrier gas, the number of scans and the substrate temperature. Next, an UVO treatment was performed on the AgNWs counter electrode for 30, 60, 120 and 180 s. The electrochemical impedance spectroscopy analysis reveals that the short UVO treatment can reduce the charger transfer resistance at the spiro-OMeTAD/AgNWs interface. With an optimal UVO treatment duration of 60 s, the cell exhibits a photoelectric conversion efficiency (PCE) of 12.13 %, open circuit voltage (Voc) of 1.04 V, short circuit current density (Jsc) of 19.97 mA/cm2, and fill factor (F.F.) of 61.5 %. Compared with the counterpart without UVO treatment (PCE of 11.15 %, Voc of 1.031 V, Jsc of 19.2 mA/cm2 and F.F. of 53.4 %), the PCE is greatly improved 8 %. Finally, we perform the bending test on the UVO treated cell. After 100 and 500 bending cycles, the cell efficiency remaines at 94% and 75% of its initial value, respectively. | en |
| dc.description.provenance | Made available in DSpace on 2021-07-11T15:01:14Z (GMT). No. of bitstreams: 1 ntu-108-R06941002-1.pdf: 6014716 bytes, checksum: d9c545b989f6482fd292ca8ae9b673d2 (MD5) Previous issue date: 2019 | en |
| dc.description.tableofcontents | 致謝ii
中文摘要 iii Abstractiv 目錄v 圖目錄viii 表目錄xiv 第1章 緒論16 1.1 前言16 1.2 太陽能電池發展16 1.3 研究動機18 1.4 論文架構18 第2章 文獻回顧20 2.1 太陽能電池20 2.1.1 太陽能電池原理20 2.1.2 太陽能電池特性參數21 2.2 鈣鈦礦太陽能電池24 2.2.1 鈣鈦礦材料24 2.2.2 鈣鈦礦太陽能電池發展25 2.2.3 鈣鈦礦太陽能電池溶液製程26 2.2.4 溶液式奈米銀線電極製程26 2.2.5 奈米銀線電極於正結構鈣鈦礦太陽能電池之應用33 2.2.6 奈米銀線電極於反結構鈣鈦礦太陽能電池之應用38 2.2.7 可撓式鈣鈦礦太陽能電池44 第3章 研究方法49 3.1 製程儀器49 3.1.1 氮氣手套箱49 3.1.2 旋轉塗佈機50 3.1.3 噴閥式塗佈機50 3.1.4 離心機51 3.1.5 紫外光臭氧系統52 3.2 量測系統53 3.2.1 太陽光模擬器53 3.2.2 掃描式電子顯微鏡54 3.2.3 原子力顯微鏡55 3.2.4 X光子繞射儀55 3.2.5 紫外光-可見光光譜儀56 3.2.6 電化學阻抗58 3.3 實驗材料介紹59 3.3.1 銦錫氧化物 (ITO)59 3.3.2 軟性基版59 3.3.3 電子傳輸層材料60 3.3.4 主動層材料60 3.3.5 電洞傳輸層材料61 3.3.6 對電極材料61 3.4 可撓性鈣鈦礦太陽能電池製程62 3.4.1 基材清洗62 3.4.2 電子傳輸層製備63 3.4.3 鈣鈦礦調配、塗佈及燒結64 3.4.4 電洞傳輸層調配、塗佈65 3.4.5 奈米銀線對電極置備及後處理65 第4章 實驗結果與討論67 4.1 不同TiO2電子傳輸層製備方式對鈣鈦礦太陽能電池效能之影響67 4.2 不同基板對鈣鈦礦太陽能電池效能之影響70 4.2.1 基板比較70 4.2.2 不同基板對低溫TiO2電子傳輸層特性的影響71 4.2.3 不同基板對Perovskite吸收層的影響73 4.2.4 不同基板對鈣鈦礦太陽能電池特性的影響79 4.3 奈米銀線對電極應用於可撓性鈣鈦礦太陽能電池81 4.3.1 噴閥式塗佈(次數)81 4.3.2 噴閥式塗佈(壓力)84 4.3.3 噴閥式塗佈(溫度)85 4.3.4 可撓性鈣鈦礦太陽能電池87 4.4 紫外光臭氧處理奈米銀對電極對可撓性鈣鈦礦太陽能電池特性之影響 92 4.4.1 紫外光臭氧處理之可撓性鈣鈦礦太陽能電池92 4.4.2 電化學阻抗分析96 4.4.3 奈米銀線及Spiro-OMeTAD之XPS分析98 4.4.4 紫外光臭氧處理之可撓性鈣鈦礦太陽能電池的彎曲測試103 第5章 結論與未來展望107 附錄A UV-Vis分析108 附錄B 薄膜分析110 附錄C111 參考文獻 112 | |
| dc.language.iso | zh-TW | |
| dc.title | 以溶液製程製備之可撓性鈣鈦礦太陽能電池 | zh_TW |
| dc.title | Solution-Processed Flexible Perovskite Solar Cells | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 107-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 陳建彰,徐振哲,吳肇欣,吳育任 | |
| dc.subject.keyword | 可撓性鈣鈦礦太陽能電池,奈米銀線,噴閥式塗佈,紫外光臭氧處理,彎曲測試, | zh_TW |
| dc.subject.keyword | flexible perovskite solar cell,silver nanowires,spray coating,ultraviolet ozone,bending test, | en |
| dc.relation.page | 119 | |
| dc.identifier.doi | 10.6342/NTU201903991 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2019-08-20 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| 顯示於系所單位： | 光電工程學研究所 | |
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