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DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 陳文章(Wen-Chang Chen) | |
dc.contributor.author | Mercedes Wu | en |
dc.contributor.author | 吳加恩 | zh_TW |
dc.date.accessioned | 2021-05-19T17:52:12Z | - |
dc.date.available | 2022-08-31 | |
dc.date.available | 2021-05-19T17:52:12Z | - |
dc.date.copyright | 2017-08-31 | |
dc.date.issued | 2017 | |
dc.date.submitted | 2017-07-31 | |
dc.identifier.citation | 1.4 References
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dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/7748 | - |
dc.description.abstract | Abstract
Biodegradable/biocompatible organic materials are a safe, non-toxic, renewable, and low-cost alternative to traditional inorganic and plastic options. In the world of electronic substrates, hydrogels are a viable “green” alternative to traditional stretchable electronic substrates but lack a direct integration pathway because of intrinsic properties like solvent evaporation, high water content, and poor mechanical characteristics. If these weaknesses were overcome, a suitable scaffold for fully stretchable, non-toxic, and biocompatible electronics could be recognized. In the first part of the thesis (chapter 2), a biocompatible, non-toxic, self-healing, mechanically tough, vapor absorbing and retaining, and recyclable PVA:PMAA pseudo-hydrogel is facilely fabricated. TGA, DSC, XRD, FTIR, and self-healing testing were used to confirm that the full blending of PVA and PMAA polymers as well as give insight on the strong hydrogen cross-link bonding between them. Stress-strain curves, relaxation times, loading and unloading mechanical testing revealed the high elongation, fast recovery, and tunable mechanical properties which helped confirm the 3D gel network of the pseudo-hydrogel structure. The pseudo-hydrogel interactions with water were especially important as the gel was able to absorb and retain water vapor which is a novel property. The gel was also able to dissolve fully in water which is important for recycling and biodegradable pathways. In the second part of the thesis (chapter 3), we built upon the stretchable, biocompatible, nontoxic, and water-soluble nature of the pseudo-hydrogel and fabricated a high performance resistive DNA memory device. Using St-DNA as a charge trapping and transporting layer, the memory device was fabricated using a structure of 1:1 pseudo-hydrogel/1:4 PEDOT:PU/St-DNA/1:4 PEDOT:PU to preserve the “green” properties of the pseudo-hydrogel. The device exhibited WORM memory characteristics similar to literature findings with a Vc,ON of 2V, a high ON/OFF current ratio of 104 and a long retention time of 104s. The device also retained these memory characteristics under 10, 30, and 50% strain as well as 1000 strain cycles at 30% strain. The device could be easily dissolved in DI water, which opens up recyclability, bioresorbability, and biodegradability potential. | en |
dc.description.provenance | Made available in DSpace on 2021-05-19T17:52:12Z (GMT). No. of bitstreams: 1 ntu-106-R04524100-1.pdf: 3317658 bytes, checksum: e08652e2b0b34f90762c2837b7f606ce (MD5) Previous issue date: 2017 | en |
dc.description.tableofcontents | Contents
Abstract……………………………………………………………………………....II Table Captions………………………………………………………………....…VIII Figure Captions……………………………………………………………......……IX Chapter 1. Introduction……………………………………………………………...1 1.1 Introduction to Biodegradable/Biocompatible Organic Electronics…….…...1 1.1.1 Hydrogels………………………………………………………………2 1.1.1.1 Tough Double-network Hydrogels……………………....…….2 1.1.1.2 Hybrid Hydrogels…………………………………...…………4 1.1.1.3 Self-healing Hydrogels…………………………………...……5 1.1.2 Organogels………………………………………………………...….6 1.1.3 Biodegradable “Green” Substrates……………………………………8 1.2 Introduction to Polymer Memory……………………………………..…….10 1.2.1 Resistor-type Polymer Memory Device Structure and Fabrication…11 1.2.2 Resistor-type Memory Classifications………………………...…….12 1.2.3 Operating Mechanism of Polymer Resistor-type Memory………….13 1.2.3.1 Filamentary Conduction Mechanism………………….…..…13 1.2.3.2 Charge Transfer (CT) Mechanism……………………...……14 1.2.3.3 Charge Trapping-Detrapping Mechanism……………………15 1.2.3.4 Conformational Change……………………………...………16 1.2.4 Polymer Materials for Resistor-type Memory……………………….17 1.2.4.1 Polyimides………………………………………………...….18 1.2.4.2 π-Conjugated Polymers………………………………………19 1.2.4.3 “Green” and Biocompatible Polymers………………...……..20 1.2.4.4 Polymer Composites…………………………………………21 1.3 Research Objectives…………………………………………………...……24 1.4 References…………………………………………………..………………26 Chapter 2. Fabrication and Characterization of PVA:PMAA Pseudo-Hydrogels for Biocompatible and Stretchable Electronic Substrates………………………..46 2.1 Introduction to PVA:PMAA Pseudo-Hydrogel……………………...……..46 2.2 Experimental………………………………………………………………..47 2.2.1 Materials……………………………………………………………..47 2.2.2 Characterization………………………………………………...……47 2.2.3 Fabrication of Pseudo-Hydrogels……………………………………48 2.3 Results and Discussion…………………………………………………..….49 2.3.1 Pseudo-hydrogel Analysis…………………………………………...49 2.3.1.1 Thermogravimetric Analysis (TGA)……………...………….49 2.3.1.2 Differential Scanning Calorimetry (DSC)……………………50 2.3.1.3 X-ray Diffraction (XRD)……………………………………..52 2.3.1.4 Infrared Spectroscopy (FTIR)………………………………..53 2.3.1.5 Self-healing Properties……………………………………….55 2.3.2 Water and Pseudo-hydrogel interactions…………………………….56 2.3.2.1 Water Vapor Absorption and Equilibrium…………….……..57 2.3.2.2 Recycling and Biodegradable Potential………………..…….60 2.3.2.3 Effect of Vapor Content on Mechanical Properties……...…..61 2.3.3 Mechanical Properties……………………………………………….62 2.3.3.1 Stress-Strain Curves and Relaxation Times of Pseudo-hydrogel Blends …………………………….…………………………………………….……62 2.3.3.2 Relaxation Times and Load-Unload Cycles……….…………64 2.3.3.3 Effect of Different Cross-linking Times and Temperatures.…65 2.4 Conclusion………………………………………………………….……….66 2.5 References…………………………………………………………….…….68 Chapter 3. Biocompatible and Stretchable DNA Memory fabricated on a PVA:PMAA Pseudo Hydrogel……………………………………………..………90 3.1 Introduction to Biocompatible Memory Devices…………………...………90 3.2 Experimental………………………………………………………..………93 3.2.1 Materials………………………………………………………….….93 3.2.2 Characterization………………………………………………...……93 3.3.3 Fabrication and Measurement of Memory Devices…………….…...94 3.3 Results and Discussion……………………………………………….…..…96 3.3.1 Pseudo-hydrogel Surface Morphology………………………………97 3.3.2 Memory Device Characterization………………………………...…99 3.3.2.1 Memory Device Performance Under Strain…………...……100 3.3.2.2 DNA Memory Mechanism…………………………….……100 3.3.3 Memory Device Dissolution in Water………………...……………102 3.3.4 Conclusions………………………………………………………...103 3.4 References……………………………………………………………....…104 Chapter 4. Conclusion and Future Work………………………………..………112 | |
dc.language.iso | en | |
dc.title | 具拉伸及生物可相容性之水膠:製備、特性分析及於電阻式記憶體應用 | zh_TW |
dc.title | Fabrication and Characterization of a Stretchable and Biocompatible Pseudo-Hydrogel for Resistor Memory Device Applications | en |
dc.type | Thesis | |
dc.date.schoolyear | 105-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 郭霽慶(Chi-Ching Guo),李文亞(Wen-Ya Lee),邱昱誠(Yu-Cheng Chiu) | |
dc.subject.keyword | 拉伸性,水膠,電阻式記憶體,生物相容性,可分解性, | zh_TW |
dc.subject.keyword | stretchable,hydrogel,resistor memory,biocompatible,disintegratable, | en |
dc.relation.page | 114 | |
dc.identifier.doi | 10.6342/NTU201702068 | |
dc.rights.note | 同意授權(全球公開) | |
dc.date.accepted | 2017-08-01 | |
dc.contributor.author-college | 工學院 | zh_TW |
dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
顯示於系所單位: | 化學工程學系 |
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