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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
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dc.contributor.advisor | 吳哲夫(Jeffrey D. Ward) | |
dc.contributor.author | Wei-hsuan Lin | en |
dc.contributor.author | 林瑋萱 | zh_TW |
dc.date.accessioned | 2021-06-17T07:15:06Z | - |
dc.date.available | 2020-07-17 | |
dc.date.copyright | 2019-07-17 | |
dc.date.issued | 2019 | |
dc.date.submitted | 2019-07-15 | |
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dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/73043 | - |
dc.description.abstract | 本篇利用MATLAB程式與常用化工程序模擬軟體Aspen Plus伺服器端進行自動化處理,並使用模擬退火法來進行變壓蒸餾系統的最適化設計,以尋找變壓蒸餾系統的最小年度總成本(TAC),並與其他分離方法比較,此方法可以降低尋找最適化設計的時間與人力,也能確保找尋到全域最佳解。變壓蒸餾系統總有九個變數(design variable),包含總板數(N1,N2)、進料板(N1FS,N2FS)、回流板(N1RS)、塔壓(P1,P2)以及與共沸物組成之距離(δ1,δ2),自動化過程可以同時考慮各變數對年度總成本之影響,並找出系統全域最佳解。為了計算年度總成本,還需考慮塔序列(sequence)、真空系統(vacuum system)以及兩塔間的熱整合(heat integration),針對此自動化處理程序,本篇會探討三種二成分共沸物系統-(1) 正己烷(N-hexane) /乙酸乙酯(ethyl acetate) (2) 丙酮(acetone)/氯仿(chloroform) (3) 苯(benzene)/ethanol(乙醇) ,利用模擬退火法找尋最小年度總成本,並與之常用的分離方法比較。三成分共沸物系統產生的共沸物可能不只一個,因此在最適化的過程會變得更加複雜,為了簡化問題,會針對一個共沸物的系統先進行探討。 | zh_TW |
dc.description.abstract | Pressure-swing distillation (PSD) is an attractive alternative for separation of azeotropic mixtures when the composition of the azeotrope changes significantly with pressure. Two columns are operated at significantly different pressures and can produce nearly pure products. Since there are a large number of design variables, it would be quite tedious and time-consuming to determine the optimal value of each variable manually, the process is modeled in Aspen Plus and the simulated annealing algorithm is implemented in MATLAB to search optimum values. MATLAB acts as a client calling Aspen Plus to run simulations and simulation results would be transferred back to MATLAB to calculate total annual cost (TAC). Combined with heat integration and vacuum system, three pressure-swing distillation cases are studied. Different initial input variables could get almost the same output variables and the results are reproducible. The optimization process executes about two hours to get the minimum total annual cost. | en |
dc.description.provenance | Made available in DSpace on 2021-06-17T07:15:06Z (GMT). No. of bitstreams: 1 ntu-108-R06524042-1.pdf: 2664918 bytes, checksum: c58554da55e51b66d9c8f9bb9df2c45c (MD5) Previous issue date: 2019 | en |
dc.description.tableofcontents | 誌謝 ii
摘要 iii Abstract iv Table of Contents v List of Figures viii List of Tables xi 1. Introduction 1 1.1. Overview 1 1.2. Literature survey 3 1.3. Motivation 8 1.4. Thesis organization 9 2. Method 10 2.1. Pressure-swing distillation (PSD) 10 2.2. Recycle stream of pressure-swing distillation 11 2.3. Vacuum system 13 2.4. Heat integration 15 2.5. Aspen Plus Active X automation server 16 2.6. Variable explorer to search cell paths 18 2.7. Detection of Aspen Plus error message and breakdown 19 2.8. Simulated annealing 20 2.8.1. Overview 20 2.8.2. Simulated annealing parameters 25 3. Application 28 3.1. Pressure-swing distillation – n-hexane/ethyl acetate case study 28 3.1.1. Design basis 28 3.1.2. Primary simulation 32 3.1.3. HP/LP PSD without heat integration 37 3.1.4. LP/HP PSD without heat integration 39 3.1.5. LP/HP PSD with partial heat integration 42 3.1.6. LP/HP PSD with/without partial heat integration 48 3.2. Pressure-swing distillation – acetone/chloroform case study 50 3.2.1. Design basis 50 3.2.2. Primary simulation 53 3.2.3. HP/LP PSD without heat integration 56 3.2.4. HP-LP PSD with partial heat integration 59 3.2.5. HP/LP PSD with/without partial heat integration 65 3.3. Pressure-swing distillation – benzene/ethanol 67 3.3.1. Design basis 67 3.3.2. Primary simulation 70 3.3.3. HP/LP PSD without heat integration 72 3.3.4. LP/HP PSD without heat integration 75 3.3.5. LP/HP PSD with partial heat integration 78 3.3.6. HP/LP PSD with/without partial heat integration 84 3.3.7. Discussions on initial guess and SA parameters 85 4. Triple column PSD – acetone/propanol/toluene case study 87 4.1.1. Design basis 87 4.1.2. Primary simulation 89 4.1.3. Without heat integration 91 5. Conclusions 94 Reference 96 Appendix A: MATLAB code 104 Appendix B: Total annual cost calculation 108 | |
dc.language.iso | en | |
dc.title | 利用程序模擬自動化伺服器設計熱整合變壓蒸餾系統 | zh_TW |
dc.title | Design of Heat-Integrated Pressure Swing Distillation Processes using a Process Simulation Automation Server | en |
dc.type | Thesis | |
dc.date.schoolyear | 107-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 陳誠亮(Cheng-Liang Chen),錢義隆(I-Lung Chien),李豪業(Hao-Yeh Lee),郭文生(Vincentius Surya Kurnia Adi) | |
dc.subject.keyword | 變壓蒸餾,模擬退火法,最適化,自動化伺服器, | zh_TW |
dc.subject.keyword | Pressure-swing distillation,simulated annealing,optimization,automation server, | en |
dc.relation.page | 110 | |
dc.identifier.doi | 10.6342/NTU201901488 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2019-07-16 | |
dc.contributor.author-college | 工學院 | zh_TW |
dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
顯示於系所單位: | 化學工程學系 |
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