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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 于昌平(Chang-Ping Wu) | |
| dc.contributor.author | Chih-Huang Chou | en |
| dc.contributor.author | 周志璜 | zh_TW |
| dc.date.accessioned | 2021-06-17T07:03:38Z | - |
| dc.date.available | 2020-08-05 | |
| dc.date.copyright | 2019-08-05 | |
| dc.date.issued | 2019 | |
| dc.date.submitted | 2019-07-29 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/72687 | - |
| dc.description.abstract | 植物微生物燃料電池(Plant microbial fuel cell, PMFC)作為一種新興的綠色能源，具有透過植物將太陽能轉換為電力之能力，是具備環境友善、碳中和、成本低廉等新興科技，除此之外，植物微生物燃料電池尚具有去除汙染物之能力，不僅能有效降低廢水或是土壤中之化學需氧量，甚至能夠還原部分重金屬來達到去除水體或是土壤中之重金屬汙染的目的。
植物微生物燃料電池是經由微生物燃料電池衍伸而來，由埋在土壤的陽極、植物、放在水表面之陰極及外接電路組成，透過土壤取代一般微生物燃料電池內的離子交換膜，使植物微生物燃料電池可分為深層土壤中之厭氧陽極槽及與空氣接觸之耗氧陰極槽。本研究以植物微生物燃料電池去除土壤中之鎘(Cd)汙染作為研究目標， 以直徑15 cm、厚度0.4 cm之圓形碳氈作為電極，並使用香蒲(Typha orientalis)及野生稻(Oryza rufipo gon)作為PMFC系統之研究對象，同時也根據環保署所公布之土壤汙染管制標準(20 m g/k g)及土壤汙染監測標準(10 m g/k g)來配置不同濃度的鎘汙染土壤。結果顯示野生稻PMFC系統比起香蒲PMFC有更高之產電能力，野生稻組之PMFC產生之最高電壓來到0.64 V，而香蒲組之PMFC所能產生之最高電壓僅到0.43 V，平均之電壓產生也是野生稻組略勝一籌，可以得到野生稻是較適合用於PMFC系統產電之植物。在土壤中鎘的去除率研究中，香蒲組PMFC在高濃度(20 m g/k g)的鎘汙染土壤中達到了30 %的去除率，而在相同之條件下野生稻僅有14 %的去除率，若以處理土壤中鎘汙染為目標，香蒲PMFC可以達到較優良的去除效果。植物微生物燃料電池是近幾年來新興之研究，利用植生復育法結合微生物燃料電池去除土壤中重金屬，具有去除汙染物並同時產能之優勢，將來實際應用在汙染場址的重金屬去除上有良好的潛力。 | zh_TW |
| dc.description.abstract | Plant microbial fuel cell (PMFC), as an new green energy source, has the ability to convert solar energy into electricity through plants. PMFC have received increasing attention due to it’s many advantages,s such as eco-friendly, carbon neutrality, and low cost. In addition, PMFCs still have the ability to remove pollutants, not only can effectively reduce the COD, but also reduce some heavy metals at the cathode in wastewater or contaminated soil.
The PMFC consists of an anode buried in the soil, a plants and a cathode placed on the surface of the water. The soil replaces the ion exchange membrane in the general MFC which can help anode to stand anaerobic environment for the electrochemically active bacteria. In this study, the removal of cadmium (Cd) from soil by PMFCs was studied. Two of 15 cm diameter and a 0.4 cm thickness circular carbon felts were used as electrodes, and Typha orientalis and Oryza rufipogon were used as a research plants of the PMFCs, Different concentrations of Cd-contaminated soil were also configured according to the soil pollution control standards (20 mg/kg) and soil pollution monitoring standards (10 mg/kg) which were published by the Environmental Protection Administration in Taiwan. The results show that the highest voltage generated by the the Oryza rufipogon PMFC comes to 0.64 V, while the highest voltage that the Typha orientalis PMFC can produce is only 0.43 V., The average voltage generation from the Oryza rufipogon PMFC is also slightly better than that of the Oryza rufipogon PMFC. It shows that Typha orientalis is more suitable for electricity production in the PMFC. However, in the study of the removal rate of Cd in soil, the Typha orientalis PMFC achieved a Cd removal rate of 30% in the high Cd contaminated soil (20 mg/kg), while the removal rate of Oryza rufipogon PMFC was only 14% under the same conditions. If the target is treating Cd in contaminated soil, Typha orientalis PMFC can achieve better removal rate. PMFC is an emerging research in recent years. The use of phytoremediation combined with MFCs to remove heavy metals from soils has the advantage of removing pollutants and producing electricity simultaneously. In the future, maybe it will be a perfect way to recover heavy metals from the contaminated sites. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-17T07:03:38Z (GMT). No. of bitstreams: 1 ntu-108-R06541123-1.pdf: 4064280 bytes, checksum: 7b9e77408ec29d93ba9d2bd7e34ab74f (MD5) Previous issue date: 2019 | en |
| dc.description.tableofcontents | 論文口試委員審定書 i
致謝 ii 中文摘要 iii Abstract iv 目錄 v 圖目錄 viii 表目錄 x 第一章 緒論 1 1.1.研究背景 1 1.2.研究動機與目的 2 第二章 文獻回顧 3 2.1.微生物燃料電池之理論及發展 3 2.1.1.微生物燃料電池之沿革 3 2.1.2.微生物燃料電池的發電原理 4 2.1.3.電子傳遞機制 6 2.1.4.微生物燃料電池的各項單元分析 8 2.2.植物微生物燃料電池 12 2.2.1.PMFC原理 12 2.2.2.根際沉積物(Rhizodeposition) 13 2.2.3.PMFC應用 15 2.2.4.PMFC的發電潛力 16 2.3.鎘的汙染 17 2.3.1.鎘的來源及毒理 17 2.3.2.土壤中的鎘 18 2.3.3.MFC去除鎘 19 第三章 材料與方法 23 3.1.實驗藥品與設備 23 3.1.1.實驗藥品 23 3.1.2.實驗設備與儀器 24 3.2.實驗流程圖 25 3.3.實驗之土壤 26 3.3.1.來源與基本資料 26 3.3.2.有效性氮、磷、鉀檢測方法 27 3.4.PMFC結構與運行 29 3.4.1.植物的選擇 29 3.4.2.鎘汙染土壤配製 29 3.4.3.PMFC架設 30 3.5.PMFC土壤檢測 31 3.5.1.採樣及保存 31 3.5.2.土壤含水率 32 3.5.3.土壤酸鹼值 32 3.5.4.土壤導電度 32 3.5.5.土壤中之重金屬 33 3.5.6.鎘在土壤中之不同型態 35 3.5.7.生物有效性鎘 37 3.6.植物中之重金屬 38 3.6.1.採樣及保存 38 3.6.2.植物中重金屬濃度 38 3.7.孔隙水之重金屬 39 3.7.1.採樣及保存 39 3.7.2.水樣重金屬測定 39 3.8.電極之分析 40 3.8.1.掃描式電子顯微鏡 40 3.8.2.X-射線光電子光譜(XPS) 41 第四章 結果與討論. 43 4.1.酸鹼值 43 4.1.1.酸鹼值之變動 43 4.1.2.酸鹼值之分層 44 4.2.導電度 46 4.2.1.導電度之變動 46 4.2.2.導電度之分層 47 4.3.重金屬濃度 49 4.3.1.重金屬之變動 49 4.3.2.重金屬之分層 53 4.4.PMFC之產電 55 4.4.1.香蒲及野生稻之比較 55 4.4.2.香蒲之電壓 57 4.4.3.野生稻之電壓 60 4.5.植物中金屬濃度 63 4.5.1.植物累積之重金屬 63 4.5.2.重金屬植物濃縮係數 68 4.6.孔隙水重金屬濃度 69 4.7. Tessier法 70 4.8.電極之分析 71 4.8.1. XPS結果 71 4.8.2. SEM結果 72 第五章 結論與建議 73 5.1.結論 73 5.2.建議 75 第六章 參考文獻 77 | |
| dc.language.iso | zh-TW | |
| dc.subject | 植物微生物燃料電池；植生復育；綠色能源；鎘；永續發展 | zh_TW |
| dc.subject | plant microbial fuel cell；cadmium；green energy；phytoremediation | en |
| dc.title | 植物微生物燃料電池運行於鎘污染土壤之復育及產電效能之研究 | zh_TW |
| dc.title | Plant Microbial Fuel Cell for Remediation of Cadmium Contaminated Soil and Electricity Generation | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 107-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 郭獻文,林居慶 | |
| dc.subject.keyword | 植物微生物燃料電池；植生復育；綠色能源；鎘；永續發展, | zh_TW |
| dc.subject.keyword | plant microbial fuel cell；cadmium；green energy；phytoremediation, | en |
| dc.relation.page | 84 | |
| dc.identifier.doi | 10.6342/NTU201902177 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2019-07-30 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| 顯示於系所單位： | 環境工程學研究所 | |
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