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| ???org.dspace.app.webui.jsptag.ItemTag.dcfield??? | Value | Language |
|---|---|---|
| dc.contributor.advisor | 韋文誠(Wen-Cheng Wei) | |
| dc.contributor.author | Yi-Wun Bai | en |
| dc.contributor.author | 白逸紋 | zh_TW |
| dc.date.accessioned | 2021-06-17T04:52:25Z | - |
| dc.date.available | 2023-08-01 | |
| dc.date.copyright | 2018-08-01 | |
| dc.date.issued | 2018 | |
| dc.date.submitted | 2018-07-30 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/71089 | - |
| dc.description.abstract | 本研究對中國清涼寺汝瓷破片(083006-b-2)進行微結構、成分、光學性質的分析，根據鈣鋁矽氧化物三元相圖(主成分之間比例)與破片成分分析(主成分/助熔劑=92.33/8.27)設計出三種玻璃(CAS-F)進行釉藥之模擬，其中氧化矽與氧化鈣固定比例(86/14)，並對氧化鋁進行調整。以可見光反射光譜探討微結構對於持溫時間(5小時、50小時)及反應氣氛之影響。利用空氣、5%氫氮混合氣以及三種碳材(木屑、煤炭、中間相碳素微球)經由高溫氣化所提供之還原氣氛進行比較。三種配方(CAS-F)皆可在1275 oC下熔融，模擬的汝釉經由長時間熱處理後具有汝瓷特徵，包含鈣長石、玻璃相分解、氣泡等，並採用一氧化碳/二氧化碳氣氛， 1250 oC/5 h處理後，其中之一樣品可顯示近似汝瓷破片之反射光譜。 | zh_TW |
| dc.description.abstract | One piece of Ru-shard (083006-b-2) from Qingliangsi (清涼寺) at Henan province in China has been investigated on microstructure, composition, and optical properties. Three glaze compositions (CAS-F series) are selected based on the CAS/F ratio of 92.33/8.27 based on the glaze composition of Ru-shard. Parent melts (CAS) is selecting from the CaO-Al2O3-SiO2 (CAS) ternary diagram with a constant SiO2/CaO ratio of 86/14, and adjusted Al2O3 contents. Visible reflective spectrometry is used to investigate the effects of dwell time (5 hr or 50 hr) and reducing atmosphere on the microstructure. Air, 5%H2-N2, and gasses from gasification three kinds of carbon materials (wood-chips (WC), Indonesia subbituminous coal (IS), meso carbon micro beads (MCMB)) are also used for comparison. Melting points of CAS-F series are all below 1275 oC. The imitated Ru-glasses by strong reduction show the characteristics of typical Ru-glaze, such as anorthite grain in glass, dual phase by decomposition, bubbles after long heating treatment. Also, one glaze formulation appears the spectrum similar to that of Ru-shard if treated by a CO/CO2 reducing atmosphere at 1250 oC for 5 h. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-17T04:52:25Z (GMT). No. of bitstreams: 1 ntu-107-R05527018-1.pdf: 8954843 bytes, checksum: 4c73d8e897cf3e690f2777ede27c8fd2 (MD5) Previous issue date: 2018 | en |
| dc.description.tableofcontents | 摘要 IV
Abstract V List of Figures X List of Tables XX Chapter 1 Introduction 1 1.1 Motivation 1 1.2 Research Objectives 2 Chapter 2 Literature Review 4 2.1 Formation of Glass Materials in China History 4 2.1.1 Provenance of Glass in China 4 2.1.2 History of Ru-wares 5 2.2 Glasses Formulation 10 2.2.1 Parent Melts 10 2.2.2 Flux (Minor Compounds) 12 2.3 Optical Properties of Glasses 18 2.3.1 Color Agent of Glasses 18 2.3.2 Random Network Theory of Glasses 26 Chapter 3 Experimental Procedure 34 3.1 Materials 34 3.2 Synthesis of Anorthite Substrate 34 3.3 Synthesis of CAS Glasses 35 3.3.1 Formulation of CAS Glasses 35 3.3.2 Composition Analysis of Ru Shard 36 3.3.3 Formulation of CAS-F Glasses 37 3.4 Annealing of Glasses on Substrate 38 3.5 Property Characterization 39 3.5.1 Microstructural (SEM) and Composition Analysis 39 3.5.2 Spinodal Decomposition Analysis (TEM) 40 3.5.3 X-ray Diffraction Analysis 40 3.5.4 Oxygen Partial Pressure 41 3.5.5 Gas Chromatography 41 3.5.6 Wetting Test 42 3.5.7 Optical Analysis 42 Chapter 4 Results and Discussion 65 4.1 Characterization of Shard from Qingliangsi Temple 65 4.1.1 Crystal Phases Analysis 65 4.1.2 Microstructure and Composition Analysis of Ru-shard 67 4.1.3 Structure Characteristics of Spinodal 83 4.1.4 Optical Properties of Ru-shard 88 4.2 Characterizations of CAS-F Glasses 92 4.2.1 Microstructure and Crystal Phases 92 4.2.2 Wetting Behavior 104 4.2.3 Optical Properties of CAS-F Glasses 109 4.3 Effects of Atmosphere 117 4.3.1 Annealing/Atmosphere Control 117 4.3.2 Optical Properties of CAS-F 127 Chapter 5 Conclusions 135 Appendix 138 Appendix I Characterization of Local Minerals from Henan 138 Appendix II Characterization of Plant Ashes from Henan and NTU Campus 156 Appendix III Practice of the Ru-Formulation from Local Resources 162 Appendix III.1 Powder Sources 162 Appendix III.2 Formulation of C1F 166 Appendix IV Energy Dispersive X-ray Analysis of The Ru-Shard 171 References 173 | |
| dc.language.iso | en | |
| dc.subject | 相分離 | zh_TW |
| dc.subject | 反射光譜 | zh_TW |
| dc.subject | 還原 | zh_TW |
| dc.subject | 氣泡 | zh_TW |
| dc.subject | 鈣鋁矽玻璃 | zh_TW |
| dc.subject | 汝瓷 | zh_TW |
| dc.subject | 鈣長石 | zh_TW |
| dc.subject | reflective spectrum | en |
| dc.subject | CaO-Al2O3-SiO2 glass | en |
| dc.subject | bubble | en |
| dc.subject | phase decomposition | en |
| dc.subject | anorthite | en |
| dc.subject | reduction | en |
| dc.subject | Ru-porcelain | en |
| dc.title | 汝瓷之科學驗證 | zh_TW |
| dc.title | Scientific Forensics of Ru-porcelain | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 106-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 魏國彥(Kuo-Yen Wei),方冠榮(Kuan-Zong Fung),李慶樹(Ching-Su Lee) | |
| dc.subject.keyword | 汝瓷,鈣鋁矽玻璃,氣泡,相分離,鈣長石,還原,反射光譜, | zh_TW |
| dc.subject.keyword | Ru-porcelain,CaO-Al2O3-SiO2 glass,bubble,phase decomposition,anorthite,reduction,reflective spectrum, | en |
| dc.relation.page | 181 | |
| dc.identifier.doi | 10.6342/NTU201800768 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2018-07-31 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 材料科學與工程學研究所 | zh_TW |
| Appears in Collections: | 材料科學與工程學系 | |
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