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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 李君浩(Jiun-Haw Lee) | |
dc.contributor.author | Hung-Yi Lin | en |
dc.contributor.author | 林虹儀 | zh_TW |
dc.date.accessioned | 2021-06-17T01:09:16Z | - |
dc.date.available | 2025-01-01 | |
dc.date.copyright | 2021-02-20 | |
dc.date.issued | 2021 | |
dc.date.submitted | 2021-02-02 | |
dc.identifier.citation | [1] J. H. Lee, C. H. Chen, P. H. Lee, H. Y. Lin, M. K. Leung, T. L. Chiu, and C. F. Lin, J. Mater. Chem. C, 2019, 7, 5874-5888 [2] C. T. Chen, C. L. Chiang, Y. C. Lin, L. H. Chan, C. H. Huang, Z. W. Tsai, and C. T Chen, Org. Lett., 2003, 5, 8, 1261-1264 [3] K. Y. Kay, J. Kim, H. Cho, J. W. Park, Mol. Cryst. Liq. Cryst., 2004, 424, 167-172 [4] S. Kim, B. Kim, J. Lee, H. Shin, Y. Park, J. Park, Materials Science and Engineering R, 2016, 99, 1-22 [5] S. K. Kim, B. Yang, Y. Ma, J. H. Lee, and J. W. Park, J. Mater. Chem., 2008, 18, 3376-3384 [6] D. Yokoyama, Y. Park, B. Kim, S. Kim, Y. J. Pu, J. Kido, and J. Park, Appl. Phys. Lett., 2011, 99, 123303 [7] P. Y. Chou, H. H. Chou, Y. H. Chen, T. H. Su, C. Y. Liao, H. W. Lin, W. C. Lin, H. Y. Yen, I. C. Chena and C. H. Cheng, Chem. Commun., 2014, 50, 6869-6871 [8] Y. H. Chen, C. C. Lin, M. J. Huang, K. Hung, Y. C. Wu, W. C. Lin, R. W. C. Cheng, H. W. Lin and C. H. Cheng, Chem. Sci., 2016, 7, 4044-4051 [9] N. Hashimoto, K. Ogita, H. Nowatari, Y. Takita, H. Kido, T. Suzuki, and S. Seo, SID, 2016, Book 1, Session 24, OLED Devices I [10] N. A. Kukhta, T. Matulaitis, D. Volyniuk, K. Ivaniuk, P. Turyk, P. Stakhira, J. V. Grazulevicius, and A. P. Monkman, J. Phys. Chem. Lett., 2017, 8, 6199-6205 [11] S. Wang, M. Qiao, Z. Ye, D. Dou, M. Chen, Y. Peng, Y. Shi, X. Yang, L. Cui, J. Li, C. Li, B. Wei, and W. Y. Wong, iScience, 2018, 9, 532-541 [12] A. Salehi, C. Dong, D. H. Shin, L. Zhu, C. Papa, A. T. Bui, F. N. Castellano, and F. So, Nature Communications, 2019, 10, 2305 [13] C. J. Chiang, A. Kimyonok, M. K. Etherington, G. C. Griffiths, V. Jankus, F. Turksoy, and A. P. Monkman, Adv. Funct. Mater., 2013, 23, 739-746 [14] M. J. Sung, H. Chubachi, R. Sato, M. K. Shin, S. K. Kwon, Y. J. Pu, and Y. H. Kim, J. Mater. Chem. C, 2017, 5, 1090-1094 [15] H. Lim, H. J. Cheon, G. S. Lee, M. Kim, Y. H. Kim, and J. J. Kim, ACS Appl. Mater. Interfaces, 2019, 11, 48121-48127 [16] R. Ieuji, K. Goushi, and C. Adachi, Nature Communications, 2019, 10, 5283 [17] J. H. Jeon, S. J. Cha, Y. M. Jeon, J. H. Lee, M. C. Suh, Organic Electronics, 2014, 15, 2802-2809 [18] L. Hu, G. Zhang, Y. Liu, T. Guo, L. Shao, and L. Ying, J. Mater. Chem. C, 2020, 8, 2160-2170 [19] 林伯彥,白光有機電激發光元件外部量子效率及壽命之研究,國立臺灣大學光電工程學研究所碩士論文 (2012). [20] J. Rivnay, S. C. B. Mannsfeld, C. E. Miller, A. Salleo, and M. F. Toney, Chem. Rev., 2012, 112, 5488-5519 [21] Y. Watanabe, D. Yokoyama, T. Koganezawa, H. Katagiri, T. Ito, S. Ohisa, T. Chiba, H. Sasabe, and J. Kido, Adv. Mater., 2019, 31, 1808300 [22] A. Gujral, K. A. O’Hara, M. F. Toney, M. L. Chabinyc, and M.D. Ediger, Chem. Mater., 2015, 27, 3341-3348 [23] P. M. Buschbaum, Adv. Mater., 2014, 26, 7692-7709 [24] C. H. Chen, N. T. Tierce, M. K. Leung, T. L. Chiu, C. F. Lin, C. J. Bardeen, and J. H. Lee, Adv. Mater., 2018, 30, 1804850 [25] A. Gujral, K. A. O’Hara, M. F. Toney, M. L. Chabinyc, and M.D. Ediger, Chem. Mater., 2015, 27, 3341-3348 [26] J. Rivnay, S. C. B. Mannsfeld, C. E. Miller, A. Salleo, and M. F. Toney, Chem. Rev., 2012, 112, 5488-5519 [27] K. Y. Kay, J. Kim, H. Cho and J. W. Park, Molecular Crystals and Liquid Crystals, 2004, 424, 167-172 [28] A. Salehi, Y. Chen, X. Fu, C. Peng, and Franky So, ACS Appl. Mater. Interfaces, 2018, 10, 9595-9601 [29] Y. Hu, L. Song, S. Zhang, Y. Lv, J. Lin, X. Guo, and X. Liu, Adv. Mater. Interfaces, 2020, 2000657 [30] H. W. Lin, C. W. Lu, L. Y. Lin, Y. H. Chen, W. C. Lin, K. T. Wong, and F. Lin, J. Mater. Chem. A, 2013, 1, 1770-1777 [31] L. Xiao, Z. Chen, B. Qu, J. Luo, S. Kong, Q. Gong, and J. Kido, Adv. Mater., 2011, 23, 926-952 [32] L. Liu, S. Li, Y. M. Zhou, L. Y. Liu, X. A. Cao, Microelectronics Reliability, 2017, 71, 106-110 [33] M. Mahboub, H. Maghsoudiganjeh, A. M. Pham, Z. Huang, and M. L. Tang, Adv. Funct. Mater., 2016, 26, 6091-6097 [34] R. Chen, Y. Tang, Y. Wan, T. Chen, C. Zheng, Y. Qi, Y. Cheng, W. Huang, Scientific Reports, 2017, 7, 6225 [35] J. H. Jeon, S. J. Cha, Y. M. Jeon, J. H. Lee, M. C. Suh, Organic Electronics, 2014, 15, 2802-2809 [36] L. Hu, G. Zhang, Y. Liu, T. Guo, L. Shao, and L. Ying, J. Mater. Chem. C, 2020, 8, 2160-2170 [37] P. Y. Chou, H. H. Chou, Y. H. Chen, T. H. Su, C. Y. Liao, H. W. Lin, W. C. Lin, H. Y. Yen, I. C. Chen and C. H. Cheng, Chem. Commun., 2014, 50, 6869-6871 [38] Y. H. Chen, C. C. Lin, M. J. Huang, K. Hung, Y. C. Wu, W. C. Lin, R. W. C. Cheng, H. W. Lin and C. H. Cheng, Chem. Sci., 2016, 7, 4044-4051 [39] Y. Hu, L. Song, S. Zhang, Y. Lv, J. Lin, X. Guo, and X. Liu, Adv. Mater. Interfaces, 2020, 2000657 [40] L. Xiao, Z. Chen, B. Qu, J. Luo, S. Kong, Q. Gong, and J. Kido, Adv. Mater., 2011, 23, 926-952 [41] R. A. K. Yadav, D. K. Dubey, S. Z. Chen, T. W. Liang, J. H. Jou, Scientific Reports, 2020, 10, 9915 [42] H. Lee, M. J. Maeng, J. A. Hong, R. Najnin, J. Moon, H. Cho, J. Lee, B. G. Yu, Y. Park, and N. S. Cho, J. Mater. Chem. C, 2017, 5, 9911-9919 [43] Y. H. Chen, C. C. Lin, M. J. Huang, K. Hung, Y. C. Wu, W. C. Lin, R. W. C. Cheng, H. W. Lin and C. H. Cheng, Chem. Sci., 2016, 7, 4044-4051 [44] K. C. Wu, P. J. Ku, C. S. Lin, H. T. Shih, F. I. Wu, M. J. Huang, J. J. Lin, I. C. Chen, and C. H. Cheng, Adv. Funct. Mater., 2008, 18, 67-75 [45] C. Zhao, L. Duan, J. Mater. Chem. C, 2020, 8, 803-820 [46] M. Y. Chang, Y. K. Han, C. C. Wu, S. C. Lin, and W. Y. Huanga, Journal of The Electrochemical Society, 2008, 155, 12, J345-J349 [47] P. Y. Chou, H. H. Chou, Y. H. Chen, T. H. Su, C. Y. Liao, H. W. Lin, W. C. Lin, H. Y. Yen, I. C. Chen and C. H. Cheng, Chem. Commun., 2014, 50, 6869-6871 [48] C. Hosokawa, H. Higashi, H. Nakamura, and T. Kusumoto, Appl. Phys. Lett., 1995, 67, 25 [49] L. Hu, G. Zhang, Y. Liu, T. Guo, L. Shao, and L. Ying, J. Mater. Chem. C, 2020, 8, 2160-2170 [50] S. Oyama, H. Sakai, and H. Murata, Jpn. J. Appl. Phys., 2016, 55, 03DD13 | |
dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/66838 | - |
dc.description.abstract | 本篇論文中包含兩個主題。第一個主題,我們介紹由中研院化學所陳錦地教授團隊所合成的以蒽衍生物為發光層的有機發光二極體。其中,以9,10-bis(3',4',5'-triphenyl-[1,1':2',1''-terphenyl]-4-yl)anthracene (TpbPhAth)為主的無摻雜有機發光二極體,具有最大電流效率為3.6 cd/A,最大功率效率為3.8 lm/W,最大外部量子效率為5.3%,並且伴隨CIE座標(0.153, 0.077)的深藍色放光。透過在TpbPhAth中摻雜天藍色客體材料4,4’-Bis[4-(di-p-tolylamino)styryl]biphenyl (DPAVBi),有機發光二極體達到最大電流效率為8.5 cd/A,最大功率效率為8.9 lm/W,最大外部量子效率為6.9%。 第二個研究主題中,我們著重在以雙層發光層的結構達到高效率的三重態-三重態融合(TTF)之有機發光二極體,該結構以1,1'-(2,5-Dimethyl-1,4-phenylene)dipyrene (DMPPP) 和 9-(1-naphthalenyl)-10-(4-(2-naphthalenyl)phenyl)anthracene (NPAN)為主體,以7,7,13,13-tetramethyl-N5,N5,N11,N11-tetraphenyl-7,13-dihydrobenzo-[g]indeno[1,2-b]fluorene-5,11-diamine (DPaNIF)為客體。與以DMPPP和NPAN為單層發光層的有機發光二極體相比,雙層發光層的架構因為更有效率的TTF而具有更高的效率表現。經過優化,雙層發光層的有機發光二極體達到最高外部量子效率15.4%,是目前我們已知所有的藍光TTF有機發光二極體中最高的記錄。 | zh_TW |
dc.description.abstract | There are two topics in this thesis. In the first topic, we demonstrated organic light-emitting diode (OLED) with four anthracene-derivative materials as the emitting layer (EML) which were synthesized by Prof. Chin-Ti Chen’s group, Institute of Chemistry in Academia Sinica. Among them, non-doped OLED based on 9,10-bis(3',4',5'-triphenyl-[1,1':2',1''-terphenyl]-4-yl)anthracene (TpbPhAth) exhibited the maximum current efficiency of 3.6 cd/A, the maximum power efficiency of 3.8 lm/W, and the maximum external quantum efficiency (EQE) of 5.3% with CIE of (0.153, 0.077) at deep-blue emission. With the incorporation of sky-blue dopant, 4,4’-Bis[4-(di-p-tolylamino)styryl]biphenyl (DPAVBi) into the TpbPhAth, the OLED achieved maximum current efficiency of 8.5 cd/A, maximum power efficiency of 8.9 lm/W, and maximum EQE of 6.9%. In the second topic, we focused on achieving high efficiency triplet-triplet fusion (TTF) OLED based on double-EML structure, which was composed of 1,1'-(2,5-Dimethyl-1,4-phenylene)dipyrene (DMPPP) and 9-(1-naphthalenyl)-10-(4-(2-naphthalenyl)phenyl)anthracene (NPAN) as the host and 7,7,13,13-tetramethyl-N5,N5,N11,N11-tetraphenyl-7,13-dihydrobenzo-[g]indeno[1,2-b]fluorene-5,11-diamine (DPaNIF) as the dopant. Compared with the DMPPP- and NPAN-based OLEDs, the double-EML structure exhibited the higher efficiency because of efficient TTF. After optimization, the double-EML OLED with the maximum EQE of 15.4% was obtained which is the highest record among all blue TTF-OLEDs to our best knowledge. | en |
dc.description.provenance | Made available in DSpace on 2021-06-17T01:09:16Z (GMT). No. of bitstreams: 1 U0001-0202202100280800.pdf: 10790444 bytes, checksum: 94a0a63f6d86a847e578698bb6dc182f (MD5) Previous issue date: 2021 | en |
dc.description.tableofcontents | 致謝 i 摘要 ii Abstract iii Content iv Figure content viii Table content xvii Chapter 1 Introduction 1 1.1 Overview 1 1.2 Introduction of OLED 1 1.3 Review of OLEDs with bulky side groups 2 1.3.1 Motivation 6 1.4 Review of TTF OLEDs 7 1.4.1 High efficiency blue TTF-/ F- OLEDs 7 1.4.2 OLEDs with high delayed emission ratio measured from TrEL 14 1.4.3 Motivation 18 1.5 References 20 Chapter 2 Experiments 22 2.1 OLED fabrication process 22 2.2 Measurement systems 22 2.2.1 J-L-V, EQE, and operation lifetime measurements 22 2.2.2 TrEL measurement 23 2.2.3 TrPL measurement 24 2.2.4 Absorption and PL spectra 25 2.2.5 Photoelectron spectroscopy 26 2.2.6 Grazing-incidence wide-angle X-ray diffraction (GIWAXD) 26 2.3 References 30 Chapter 3 31 3.1 Introduction 31 3.2 Photophysical properties and device performances of anthracene-derivatives 32 3.2.1 Photophysical properties of four anthracene-derivative materials 32 3.2.2 Device performances of four anthracene-derivatives as the EML of non-doped OLEDs 36 3.2.3 Anthracene-derivatives as hosts for blue OLEDs 41 3.3 Device performances of TpbAth-based OLED 44 3.3.1 Selection of different ETL materials 45 3.3.2 Selection of HIL/HTL materials 51 3.4 Device performances of TpbPhAth-based OLED 53 3.4.1 EML thickness optimization 54 3.4.2 ETL thickness Optimization 57 3.4.3 DPAVBi concentration optimization 61 3.4.4 Ni808 concentration optimization 67 3.4.5 DPaNIF concentration optimization 70 3.5 Device performance of CzPhAthTpb-based OLEDs 74 3.5.1 EML thickness optimization 75 3.5.2 ETL thickness optimization 78 3.5.3 DPAVBi concentration optimization 81 3.6 Device performances of CzPhAthTze-based OLEDs 85 3.7 TTF process in four anthracene derivatives 89 3.8 Light outcoupling of TpbPhAth 96 3.9 References 98 Chapter 4 99 4.1 Introduction 99 4.2 High EQE blue TTF-OLEDs with double-EML structure 100 4.3 Photophysical properties of EML thin films 105 4.3 NPAN-based single EML devices optimization 108 4.3.1 Selection of different ETL for single EML devices 109 4.3.2 DPaNIF concentration optimization 113 4.3.3 EML thickness optimization 117 4.3.4 ETL thickness optimization 120 4.3.5 Change different HTL 123 4.4 Double-EML devices optimization 126 4.4.1 Replacement of TTF host and change different ETL 127 4.4.2 Selection of different HTL materials 133 4.4.3 DPaNIF concentration in DMPPP optimization 136 4.4.4 DPaNIF concentration in NPAN optimization 140 4.4.5 DMPPP thickness optimization 143 4.4.6 NPAN thickness optimization 146 4.4.7 TmPyPb thickness optimization 149 4.5 References 153 Chapter 5 Summary 154 Appendix 155 A. Lifetime improvement 155 B. Use the DMPPP/ ADN double-EML structure to select a potential dopant 159 C. Use hole only and electron only devices to prove triplet-polaron quench in double-EML structure 168 D. References 172 | |
dc.language.iso | en | |
dc.title | 高效率藍色螢光有機發光二極體之研究 | zh_TW |
dc.title | Study on High Efficiency Blue Fluorescent Organic Light-emitting Diodes | en |
dc.type | Thesis | |
dc.date.schoolyear | 109-1 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 邱天隆(Tien-Lung Chiu),梁文傑(Man-kit Leung),陳錦地(Chin-Ti Chen),蔡永誠(Yung-Cheng Tsai) | |
dc.subject.keyword | 有機發光二極體,深藍色,高效率,三重態-三重態融合,雙層發光層, | zh_TW |
dc.subject.keyword | organic light-emitting diode,deep-blue,high efficiency,triplet-triplet fusion,double-emitting layer, | en |
dc.relation.page | 172 | |
dc.identifier.doi | 10.6342/NTU202100354 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2021-02-03 | |
dc.contributor.author-college | 電機資訊學院 | zh_TW |
dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
顯示於系所單位: | 光電工程學研究所 |
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