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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 王珮玲(Pei-Ling Wang) | |
| dc.contributor.author | Zhe-Wei Hsu | en |
| dc.contributor.author | 許哲維 | zh_TW |
| dc.date.accessioned | 2021-06-16T17:13:49Z | - |
| dc.date.available | 2012-08-20 | |
| dc.date.copyright | 2012-08-20 | |
| dc.date.issued | 2012 | |
| dc.date.submitted | 2012-08-20 | |
| dc.identifier.citation | 張永欣 (2011)。臺灣東部雷公火泥火山之微生物甲烷循環。國立臺灣大學地質科學研究所碩士論文，共111頁
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/63547 | - |
| dc.description.abstract | 本研究旨在瞭解陸域泥火山系統中含鐵礦物的變化與 AOM 作用的關係。研究區域為台灣東部雷公火泥火山，前人研究已初步證實AOM 作用與鐵還原作用的關聯。本研究於不同的噴發泥池邊採取6根岩芯，長度自30 cm ~ 60 cm不等，萃取沈積物中3種不同型式的鐵含量，分別為可反應總鐵、碳酸鐵與易還原氧化鐵，並進行沈積物中總碳、有機碳與無機碳的含量分析。對比沈積物孔隙水中甲烷、鐵離子和溶解無機碳濃度，發現各岩芯分別在不同深度都有AOM的存在，並且鐵還原菌消耗的氧化鐵主要為易還原的氧化鐵。在岩芯中各深度的碳酸鐵含量大部分都較噴泥中的含量高，顯示在沈積物累積由淺層深埋至底層的過程中，曾經發生或正在進行鐵還原作用，總還原態鐵含量的證據也支持了岩芯中碳酸鐵的含量是經由長時間累積的結果，不過 AOM 與鐵還原作用合作或是鐵還原菌代謝有機碳的產物，均可促進碳酸鐵的沈澱。影響有機碳與無機碳含量的生地化作用很多，與鐵還原作用合作的AOM作用可能增加有機碳含量，但代謝有機碳鐵還原作用則會消耗有機碳，岩芯中有機碳與無機碳含量變化與AOM或其他生地化反應的關係仍有待進一步釐清。 | zh_TW |
| dc.description.abstract | Anaerobic oxidation of methane (AOM) is widely performed by the cooperation between anaerobic methanotrophic archaea (ANME) and sulfate-reducing bacteria in marine sediments. Due to the lack of sulfate, AOM may carry out by ANMEs and iron reducers (IRs) in terrestrial mud volcanoes. Both mechanisms could enhance carbonate precipitates and also regulate iron cycling.
The objective of this study is to understand the relationship between AOM and the iron-bearing minerals in the Lei-Gong-Huo mud volcano in eastern Taiwan. Six cores were retrieved beside different eruptive pools. The content of three different types of iron (total reactive iron, easily reducible iron and carbonate iron), total organic carbon (TOC) and total inorganic carbon (TIC) were analyzed. The iron-methane transition zone (IMTZ) can be reconginzed in all cores, inferring the cooperation between ANMEs and IRs. Iron carbonate contents and/or fractions in the IMTZ are generally higher than that of adjacent bubbling fluids. Apparently, iron-dependent AOM is channeled into siderite (FeCO3) precipitates. Siderite was widely accumulated in whole cores, suggesting iron reduction does not only perform in certain depth recently. However, both iron-dependent AOM and organotrophic iron reduction could enhance siderite precipitatation. Many biogeochemical processes could change the TOC and TIC contents. It seems that iron-dependent AOM could increase the TOC concent, but organotrophic iron reduction may consume TOC. The correlation between TOC/TIC content and AOM or other biogeochemical processes need to be further evaluated. | en |
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| dc.description.tableofcontents | 目錄
口試委員會審定書 i 誌謝 ii 摘要 iii ABSTRACT iv 第一章 緒論 1 1.1 前言 1 1.2 全球甲烷循環 1 1.3 微生物甲烷代謝作用. 2 1.3.1 產甲烷菌（methanogenic archaea）2 1.3.2 好氧型甲烷氧化菌(aerobic methanotrphic bacteria) 3 1.3.3 厭氧型甲烷氧化菌(Anaerobic methanotrophic archaea，ANME) 4 1.4 鐵還原作用 8 1.5 泥火山 9 1.6 研究目的 12 第二章 採樣與實驗方法 15 2.1 採樣地點 15 2.2 採樣方法 15 2.3 沈積物化學分析取 16 2.3.1 鐵物種的萃取 16 2.3.1.1 含鐵礦物的配製 16 2.3.1.2 鐵物種的萃取方法 16 2.3.1.3 鐵含量分析 20 2.3.2 總碳、有機碳與無機碳的分析 21 2.4 儀器誤差 21 第三章 實驗結果 23 3.1 總鐵含量分析結果 23 3.2 易還原氧化鐵含量分析結果 23 3.3 碳酸鐵含量分析結果 25 3.4 碳酸鐵來自易還原氧化鐵中的比例隨深度變化 28 3.5 各岩芯中含鐵礦物的比例 28 3.6 有機碳含量分析結果 33 3.7 無機碳含量分析結果 33 第四章 討論 37 4.1 水化學的濃度變化與進行中的AOM 作用 37 4.3 碳酸鐵含量與比例增加與AOM 作用的關係 38 4.4 有機碳含量變化與 AOM 關係 39 4.5 岩芯中總還原態鐵含量與AOM 作用的關係 40 第五章 結論 45 參考文獻 46 附錄 53 圖目錄 圖1-1、FE3+ 與 FE2+ 轉換，參與的分子與反應。 8 圖1-2、臺灣東部雷公火泥火山噴泥口與岩芯中水化學隨深度變化圖。 13 圖1-3、臺灣東部雷公火泥火山微生物群落結構與菌群豐度隨深度變化圖。 14 圖2-1、臺灣東部雷公火泥火山全景圖。 18 圖2-2、雷公火泥火山採樣位置圖。 19 圖2–3：鐵物種萃取示意圖 20 圖2-4、元素分析儀 22 圖3-1、各岩芯與噴泥口的總鐵含量隨深度變化圖。 24 圖3-2、各岩芯與噴泥口的易還原氧化鐵含量隨深度變化圖。 26 圖3-3、各岩芯與噴泥口的碳酸鐵含量隨深度變化圖。 27 圖3-4、各岩芯之碳酸鐵所佔比例隨深度的變化。 29 圖3-5、各岩芯含鐵礦物柱狀圖 30 圖3-6 各岩芯與噴泥口的有機碳含量隨深度變化圖。 34 圖3-7 各岩芯與噴泥口的無機碳含量隨深度變化圖。 35 圖4-1、各岩芯中AOM 存在的深度範圍。 42 表目錄 表2-1、各岩芯的長度與噴泥口化學資料 15 表3-1、各岩芯與噴泥口的總鐵含量 32 表3-2、各岩芯與噴泥口的易還原氧化鐵含量 32 表3-3、各岩芯與噴泥口的碳酸鐵含量 32 表3-4、各岩芯與噴口的有機碳含量 36 表3-5、各岩芯與噴口的無機碳含量 36 | |
| dc.language.iso | zh-TW | |
| dc.title | 臺灣東部雷公火泥火山中厭氧型甲烷氧化作用與含鐵礦物之關係 | zh_TW |
| dc.title | The relationship between anaerobic oxidation of methane and iron minerals in the Lei-Gong-Huo mud volcano of eastern Taiwan | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 100-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 林立虹(Li-Hung Lin),蘇志杰(Chih-Chieh Su),李孟陽(Meng-Yang Lee) | |
| dc.subject.keyword | 雷公火泥火山,甲烷,厭氧型甲烷氧化作用,鐵還原作用,含鐵礦物, | zh_TW |
| dc.subject.keyword | Lei-Gong-Huo mud volcano,methane,anaerobic oxidation of methane,iron reduction,iron-bearing minerals, | en |
| dc.relation.page | 65 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2012-08-20 | |
| dc.contributor.author-college | 理學院 | zh_TW |
| dc.contributor.author-dept | 海洋研究所 | zh_TW |
| 顯示於系所單位： | 海洋研究所 | |
文件中的檔案：
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| ntu-101-1.pdf 目前未授權公開取用 | 4.83 MB | Adobe PDF |
系統中的文件，除了特別指名其著作權條款之外，均受到著作權保護，並且保留所有的權利。