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http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/60792完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 林清富(Ching-Fuh Lin) | |
| dc.contributor.author | Jiun-Jie Chao | en |
| dc.contributor.author | 趙俊傑 | zh_TW |
| dc.date.accessioned | 2021-06-16T10:30:24Z | - |
| dc.date.available | 2018-08-27 | |
| dc.date.copyright | 2013-08-27 | |
| dc.date.issued | 2013 | |
| dc.date.submitted | 2013-08-14 | |
| dc.identifier.citation | Chapter1
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Liu, Electroluminescence and photoluminescence studies on carrier radiative and nonradiative recombinations in metal-oxide-silicon tunneling diodes, Journal of Applied Physics 93 (2003) 4253-4259. | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/60792 | - |
| dc.description.abstract | 由於能源耗損與環保議題的因素下，可再生的替代能源越顯重要。在眾多的再生能源當中，由於太陽能其來源最為豐沛且潔淨，而極具潛力。太陽能的研究發展在全球越來越扮演著極為重要的角色且持續不斷的增加。目前，薄膜型太陽能電池被視作為最具潛力可以改變太陽能發電成本架構的太陽能電池種類，而在眾多薄膜型太陽能電池的種類當中，有機無機混成太陽能電池由於同時具備了無機材料與有機材料的優點，而引發了研究熱潮。在本論文中，研究主題將涵蓋了以砷化鎵作為材料的混成太陽能電池、固態染料敏化太陽能電池、以及熱載子太陽能電池。在以砷化鎵作為材料的混成太陽能電池方面，我們完成了一種結合透明導電高分子PEDOT:PSS與垂直型態n型砷化鎵奈米線的一種新型混成太陽能電池。在製作以二氧化鈦奈米柱作為光電極的固態染料敏化太陽能電池方面，研究結果顯示，具有足夠密集的二氧化鈦奈米柱陣列可同時提供足夠的染料吸附以及有效的載子收集能力。在熱載子太陽能電池的研究方面，我們製作了一種可收集熱載子的光電轉化新型裝置，其結構包含了一有機電洞傳輸層、一有機電子傳輸層、以及一層以金屬做為材料的光吸收層，此元件所量測到的極大開路電壓，可證實的確收集到具高能量的電子與電洞。 | zh_TW |
| dc.description.abstract | For both energy consumption and environmental reasons, the importance of alternative renewable energy sources has increased in significance. Among various renewable energy, solar energy holds tremendous potential because it is the most abundant and cleanest energy. The research and development of solar cells are playing a significant role all over the world and have continuously increased. Nowadays, thin-film solar cells are considered to have the potential to revolutionize the cost structure of photovoltaic electricity generation. For several types of thin-film solar cells, the organic-inorganic hybrid solar cell has attracted a great deal of interest because it takes both advantages of organic and inorganic materials. In this thesis, the contents include the study of GaAs-based hybrid solar cells, solid-state dye-sensitized solar cells, and hot carrier solar cells. For GaAs-based hybrid solar cells, we demonstrate a new type of hybrid solar cell based on a heterojunction between PEDOT:PSS and vertically aligned n-type GaAs nanowire arrays. Form our TiO2 nanorod based solid-state dye-sensitized solar cell, the results show that solar cells with sufficiently dense arrays of long TiO2 nanorods can give good dye loading and the efficient carrier collection. For the hot carrier solars, we demonstrate a new type of hot-carrier photo-electric conversion apparatus, which comprises an organic hole transportation layer, an organic electron transportation layer, and a light-absorbing metal layer. This achieved high open-circuit voltage is the strong evidence that this device has collected the high-energy electrons and holes. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-16T10:30:24Z (GMT). No. of bitstreams: 1 ntu-102-F94943042-1.pdf: 5629073 bytes, checksum: a26ba3b80359d5ce650a2860b3b60534 (MD5) Previous issue date: 2013 | en |
| dc.description.tableofcontents | Chapter 1 Introduction 1
1-1 The era of fossil energy 1 1-2 Solar energy 4 1-3 Basic principle of solar cell operation 6 1-3-1 Solar irradiation 7 1-3-2 Photovoltaic effect 8 1-4 Hybrid solar cells 11 1-4-1 GaAs-based hybrid solar cells 12 1-4-2 Dye-sensitized solar cells 13 1-5 Hot carrier solar cells 15 1-6 Objective and aim of this study 18 1-7 Thesis overview 21 1-8 References 24 Chapter 2 Controlled formation of well-aligned GaAs nanowires with a high aspect ratio on transparent substrates 27 2-1 Introduction 28 2-2 Experimental procedures 29 2-2-1 Formation of the monolayer of SiO2 nanoparticles 30 2-2-2 Using the monolayer of SiO2 nanoparticles as the dry-etch mask 33 2-3 Transfer of GaAs nanowires onto the glass receiver substrate 37 2-4 Optical properties of GaAs nanowires 41 2-5 Summary 46 2-6 References 47 Chapter 3 GaAs nanowire/poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) hybrid solar cells 50 3-1 Introduction 51 3-2 Experimental procedures 53 3-2-1 Dry-etching to fabricate GaAs NW arrays with the inductively coupled plasma reactive ion etching system 54 3-2-2 Hemispherical reflectance measurement of GaAs NW arrays 57 3-2-3 Attaching GaAs NW arrays onto the PEDOT:PSS conductive polymer layer coated on ITO glass 59 3-3 J-V characteristics of the GaAs NW/PEDOT:PSS solar cells 59 3-4 The trends in cell performance for GaAs NW/PEDOT:PSS hybrid solar cells 63 3-5 Summary 67 3-6 References 68 Chapter 4 GaAs nanowire/poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) hybrid solar cells with incorporating electron blocking poly(3-hexylthiophene) layer 71 4-1 Introduction 72 4-2 Experimental procedures 74 4-2-1 Attaching GaAs NW arrays onto the PEDOT:PSS conductive polymer layer coated on ITO glass 75 4-2-2 Spinning P3HT in advance onto the fabricated GaAs nanowire arrays 76 4-3 Morphology & Hemispherical reflectance measurement of GaAs NW arrays 77 4-4 J-V characteristics of the GaAs nanowire/P3HT/CleviosTM P HC V4solar cells 82 4-5 Contact morphology between organic materials and GaAs nanowire arrays 89 4-6 Summary 91 4-7 References 91 Chapter 5 The Efficient Vacuum-Assisted Method to Improve the Pore-Filling of Hole Transporting Material in TiO2 Nanorod Based Solid-State Dye-Sensitized Solar Cells 95 5-1 Introduction 96 5-2 Hydrothermal synthesis of TiO2 nanorods 98 5-3 Device fabrication of solar cells 102 5-4 SEM images of as-grown TiO2 nanorods and morphology of P3HT infiltration 104 5-5 Crystallization feature of as-grown TiO2 nanorods 106 5-6 J-V characteristics of three types of fabricated cells with different treatment at D149-TiO2/P3HT interface 108 5-7 J-V characteristics of fabricated cells with TiO2 nanorods grown by the two-step growth process 110 5-8 J-V characteristics of fabricated cells with/without the P3HT vacuum-assisted infiltration 112 5-9 Summary 114 5-10 References 115 Chapter 6 Hot Carrier Solar Cells 121 6-1 Introduction 121 6-2 Proposed hot-carrier photo-electric conversion apparatus 125 6-3 Device fabrication and the corresponding J–V characteristics 129 6-4 Summary 139 6-5 References 141 Chapter 7 Conclusions 142 | |
| dc.language.iso | en | |
| dc.subject | 砷化鎵奈米線陣列 | zh_TW |
| dc.subject | 砷化鎵型態混成太陽能電池 | zh_TW |
| dc.subject | 二氧化鈦奈米柱 | zh_TW |
| dc.subject | 固態染料敏化太陽能電池 | zh_TW |
| dc.subject | 熱載子太陽能電池 | zh_TW |
| dc.subject | TiO2 nanorod | en |
| dc.subject | GaAs-based hybrid solar cell | en |
| dc.subject | solid-state dye-sensitized solar cell | en |
| dc.subject | hot carrier solar | en |
| dc.subject | GaAs nanowire array | en |
| dc.title | 奈米結構型態有機無機混成太陽能電池 | zh_TW |
| dc.title | Nanostructured Organic-Inorganic Hybrid Solar Cells | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 101-2 | |
| dc.description.degree | 博士 | |
| dc.contributor.oralexamcommittee | 李嗣涔(Si-Chen Lee) | |
| dc.subject.keyword | 砷化鎵奈米線陣列,砷化鎵型態混成太陽能電池,二氧化鈦奈米柱,固態染料敏化太陽能電池,熱載子太陽能電池, | zh_TW |
| dc.subject.keyword | GaAs nanowire array,GaAs-based hybrid solar cell,TiO2 nanorod,solid-state dye-sensitized solar cell,hot carrier solar, | en |
| dc.relation.page | 146 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2013-08-15 | |
| dc.contributor.author-college | 電機資訊學院 | zh_TW |
| dc.contributor.author-dept | 光電工程學研究所 | zh_TW |
| 顯示於系所單位： | 光電工程學研究所 | |
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