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| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 郭茂坤(Mao-Kuen Kuo) | |
| dc.contributor.author | Huang-Chih Chen | en |
| dc.contributor.author | 陳皇志 | zh_TW |
| dc.date.accessioned | 2021-06-16T10:20:34Z | - |
| dc.date.available | 2013-11-05 | |
| dc.date.copyright | 2013-11-05 | |
| dc.date.issued | 2013 | |
| dc.date.submitted | 2013-08-16 | |
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| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/60524 | - |
| dc.description.abstract | 本研究單顆金和銀奈米殼球的平均螢光增益，matryoshka奈米粒子自身plasmonic Fano resonance現象及其各種螢光增益，最後探討雙顆銀奈米殻球各種表面電漿子共振模態(SPR)與螢光增益。根據Maxwell電磁理論作為基礎，利用Mie理論與並矢格林函數，整理單顆球型奈米粒子受平面波與電偶極波源的電磁場解析解，除此之外，並使用多重多極展開法做為計算方法，處理雙顆散射體的電磁場。最後定義激發效率、量子效率、螢光增益以及考慮螢光分子隨機分佈、任意極化方向的平均螢光增益。
螢光增益與螢光分子位置、震盪方向、入射平面波極化方向、電漿共振模態彼此有密切的關係。考慮一般實驗螢光分子均勻分布、極化方向難以控制的情況，以平均螢光增益(AEF)的概念來解釋各種散射體的光學特性較為恰當。另外，再加入史托克位移(Stokes shift)效應，討論單顆與雙顆多層奈米球對螢光增益的影響。 matryoshka奈米粒子此結構內核黃金與外殼黃金發生內外不對稱結構電漿子模態耦合現象，在近場吸收頻譜中會有局部峰值，而稱為plasmonic Fano resonance，此兩不對稱結構彼此發生了牽引交互作用，造成金屬內耗吸收的能量增強，而在遠場會有Fano dip產生，且內外耦合會混雜出多種電漿子共振模態，bonding mode與anti-bonding mode，然而若如果改變結構尺寸，使得耦合增強，那麼Fano factor (q)的絕對值會上升。最後一部份雙顆銀奈米殼球，若將他們靠越近也會有耦合(bonding)現象，但不是Fano resonance，此外此結構就像一個奈米天線一樣，容易激發出雙顆長軸共振dipole mode。 | zh_TW |
| dc.description.abstract | In this thesis, we discuss the surface plasmonic modes and interactions among fluorescent molecules, visible light and gold nanoshells (GNSs) or silver nanoshells (SNSs), the nanomatryoshka partical (Au-SiO2-Au), the silver nanoshell dimer. Based on Maxwell's equations, analytical solutions of the field excited by a plane wave and the electric dipole source out of the multi-layer spherical structure result from Mie theory and dyadic Green’s functions respectively. The multiple-multipole (MMP) method was used to solve fields of the dimer case. In addition, we also define the excitation rate, quantum yield, enhancement factor (EF) and average enhancement factor (AEF).
The enhancement factor (EF) has very much to do with the plasmonic modes, the arbitrary orientation, the location of molecules and the polarization of the incident wave. The concept of AEF can avoid overestimating or underestimating fluorescent intensity because it is hard to control the location and orientation of molecules in experiment. Furthermore, with Stokes shift effect, we observe the difference of AEF between three kinds of nanoparticles: nanoshells, nanomatryoshka and the nanoshell dimer. For the structure of nanomatryoshka, plasmon modes of the inner Au core and the outer Au shell hybridize two different modes, forming a lower energy narrow bonding mode and a higher energy broad anti-bonding mode. The modes of two asymmetry structures couple each other and induce a plasmonic Fano resonance and Fano dip, which appearing on the peak of the absorption spectra and the local minimum of the scattering spectra respectively due to the destructive interference of the two modes. However, if we change the dimension of nanomatryoshka to enhence the coupling of the two modes, the absolute value of Fano factor (q) will increase. Finally, for Ag nanoshell dimer, if we decrease their gap, they would couple each other (bonding) rather than Fano resonance. Furthermore, the nanoshell dimer is like a nanoantenna and easily excited longitudinal dipole mode. | en |
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| dc.description.tableofcontents | 第一章 緒論.............................................. 1
1.1前言................................................. 1 1.2文獻回顧.............................................. 2 1.3本文內容.............................................. 6 第二章 電磁理論與Mie解析解理論.............................. 8 2.1 Maxwell方程式與邊界條件............................... 8 2.2 Helmholtz方程與球向量波函數............................ 10 2.3平面波於核-殼球奈米散射體之散射........................... 13 2.4平面波於多層球(核-殻-殼)奈米散射體之散射................... 17 2.5散射截面積效率、吸收截面積效率、消散截面積效率、激發效率....... 21 第三章 電偶極與球形奈米散射體作用解析解 ........................26 3.1電偶極波源場與並矢格林函數............................... 26 3.2電偶極位於核-殼球奈米散射體外之散射........................ 29 3.3電偶極位於多層球(核-殻-殼)奈米散射體外之散射................ 35 3.4雙電偶極於奈米散射體外之散射.............................. 41 3.5輻射效率、非輻射效率、量子效率............................ 43 3.6無史托克位移(Non-Stokes shift)與 史托克位移(Stokes shift)現象........................... 44 3.7螢光增益與平均螢光增益(EEF; AEF)......................... 45 第四章 多重中心展開法(MMP)處理電磁場問題...................... 53 4.1 MMP的基本觀念........................................ 53 4.2利用MMP表示奈米粒子的電磁場與計算方法...................... 54 4.3奇異值拆解法求解電磁場未知係數............................ 57 第五章 數值結果與分析討論................................... 64 5.1奈米殼球(Nanoshell)散射體之平均螢光增益................... 66 5.1.1 Au Nanoshell..................................... 68 5.1.1.1無史托克位移現象(Non-Stokes shift)................. 68 5.1.1.2史托克位移現象(Stokes shift)....................... 75 5.1.2 Ag Nanoshell..................................... 78 5.1.2.1無史托克位移現象(Non-Stokes shift)................. 78 5.1.2.2史托克位移現象(Stokes shift)....................... 89 5.2 matryoshka (Au-SiO2-Au)奈米散射體.................... 93 5.2.1平面波波源與模態分析.................................. 94 5.2.2電偶極波源與模態分析.................................. 104 5.2.2.1單一電偶極(single dipole)......................... 104 5.2.2.2雙顆電偶極(bi-dipole)............................. 120 5.2.3螢光增益............................................ 128 5.2.3.1無史托克位移現象(Non-Stokes shift)................. 129 5.2.3.2史托克位移現象(Stokes shift)....................... 138 5.3雙顆銀奈米殼球(Ag Nanoshell Dimer)奈米散射體............. 140 5.3.1平面波波源.......................................... 141 5.3.2電偶極波源.......................................... 152 5.3.3螢光增益............................................ 160 5.3.3.1無史托克位移現象(Non-Stokes shift)................. 161 5.3.3.2史托克位移現象(Stokes shift)....................... 163 第六章 結論與未來展望...................................... 170 6.1結論................................................. 170 6.2未來展望.............................................. 171 附錄A 平面波於核-殼球奈米散射體之散射......................... 172 附錄B 平面波於多層球奈米散射體之散射.......................... 175 附錄C 電偶極位於核-殼球奈米散射體外之散射...................... 179 附錄D 電偶極位於多層球奈米散射體外之散射....................... 184 附錄E 電偶極任一震盪方向對球形散射體之輻射效率、非輻射效率的化簡... 190 附錄F 解析解與MMP邊界電磁場的比較............................ 193 參考文獻................................................. 195 | |
| dc.language.iso | zh-TW | |
| dc.subject | 並矢格林函數 | zh_TW |
| dc.subject | 表面電漿子共振 | zh_TW |
| dc.subject | 多重多極展開法 | zh_TW |
| dc.subject | 雙顆奈米殼散射體 | zh_TW |
| dc.subject | matryoshka奈米粒子 | zh_TW |
| dc.subject | Fano resonance | zh_TW |
| dc.subject | Fano dip | zh_TW |
| dc.subject | Mie理論 | zh_TW |
| dc.subject | 螢光分子 | zh_TW |
| dc.subject | 激發效率 | zh_TW |
| dc.subject | 量子效率 | zh_TW |
| dc.subject | 平均螢光增益 | zh_TW |
| dc.subject | Stokes shift | zh_TW |
| dc.subject | bonding與anti-bonding mode | zh_TW |
| dc.subject | Fano factor | zh_TW |
| dc.subject | Fano factor | en |
| dc.subject | dyadic Green’s functions | en |
| dc.subject | surface plasmonic modes | en |
| dc.subject | MMP | en |
| dc.subject | nanoshell dimer | en |
| dc.subject | nanomatryoshka | en |
| dc.subject | Fano resonance | en |
| dc.subject | Fano dip | en |
| dc.subject | Mie theory | en |
| dc.subject | fluorescence molecule | en |
| dc.subject | excitation rate | en |
| dc.subject | quantum yield | en |
| dc.subject | average enhancement factor | en |
| dc.subject | Stokes shift | en |
| dc.subject | bonding and anti-bonding mode | en |
| dc.title | 單顆和雙顆多層奈米粒子之表面電漿子模態分析與對螢光分子的螢光增益之研究 | zh_TW |
| dc.title | Plasmon Modes of Multi-layered Nanoparticles & Dimer and Their Surface Enhanced Fluorescence | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 101-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 廖駿偉(Jiunn-Woei Liaw),鄧崇任 | |
| dc.subject.keyword | Mie理論,並矢格林函數,表面電漿子共振,多重多極展開法,雙顆奈米殼散射體,matryoshka奈米粒子,Fano resonance,Fano dip,Fano factor,螢光分子,激發效率,量子效率,平均螢光增益,Stokes shift,bonding與anti-bonding mode, | zh_TW |
| dc.subject.keyword | Mie theory,dyadic Green’s functions,surface plasmonic modes,MMP,nanoshell dimer,nanomatryoshka,Fano resonance,Fano dip,Fano factor,fluorescence molecule,excitation rate,quantum yield,average enhancement factor,Stokes shift,bonding and anti-bonding mode, | en |
| dc.relation.page | 202 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2013-08-16 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 應用力學研究所 | zh_TW |
| 顯示於系所單位： | 應用力學研究所 | |
文件中的檔案：
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| ntu-102-1.pdf 未授權公開取用 | 23.69 MB | Adobe PDF |
系統中的文件，除了特別指名其著作權條款之外，均受到著作權保護，並且保留所有的權利。