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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 蔣本基(Pen-Chi Chiang) | |
dc.contributor.author | Yen-Syun Chen | en |
dc.contributor.author | 陳彥勛 | zh_TW |
dc.date.accessioned | 2021-06-16T05:42:38Z | - |
dc.date.available | 2025-07-14 | |
dc.date.copyright | 2020-08-03 | |
dc.date.issued | 2020 | |
dc.date.submitted | 2020-07-24 | |
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dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/56694 | - |
dc.description.abstract | 近幾年,隨著電子科技產品的快速發展,「都市礦山」成了最新穎的名詞,意謂著從產生的電子廢棄物中回收其中的貴重金屬。本研究和優勝奈米公司合作,優勝奈米公司發展高銅回收率之技術,然而其中的溶銅製程會產生大量的氮氧化物,造成人體和環境的危害。因此本計畫引入超重力旋轉床,藉由離心力所產生之高質傳特性,並搭配適當之氧化劑和吸收劑將氮氧化物去除。對於平均濃度1127 ppm之入口氮氧化物濃度,本研究之最高去除效率可達91.4%,對應之條件為使用臭氧為氧化劑和氫氧化鈉為吸收劑,超重力因子152、氣液比0.83和pOH 1.22。經反應曲面法可得到一更好之操作條件: 超重力因子131、氣液比0.837和pOH 1.22,此條件應用至實際廢印刷電路板溶銅試驗所產生平均濃度349.3 ppm之氮氧化物亦可達95.54%之去除效率。本研究也發展理論和經驗模式來和實際實驗數值比較其誤差。最後,本研究提出Pcap針對能源消耗和去除效率做鏈結,也針對成本效益分析,並提出最佳之操作條件,期盼能提供未來做利用超重力旋轉床去除氮氧化物之研究進行優化、實廠化和全面性分析之實際案例。 | zh_TW |
dc.description.abstract | Over the past several decades, significant developments have taken place in the field of urban mining, namely recovering invaluable metal from electronic waste. U-win company developed latest technology to effectively and efficiently screw out the precious copper within them. A copper dissolution process is inevitable, and a large amount of nitrogen oxides would be produced and therefore a state-of-art equipment, rotating packed bed, which could largely enhance the gas-liquid mass transfer through centrifugal force was applied and appropriate oxidants and absorbents were added to grade down NOx emission. The highest removal efficiency achieved in this study was 91.4%, when using ozone as oxidants, high gravity factor of 152, gas-to-liquid ratio of 0.83, and pOH of 1.22 dealing with average NOx concentration 1127 ppm. In addition, theoretical as well as empirical models were advanced to compare with experimental results. A motivational approach to examine a clean production technology with the integration of NOx removal efficiency and energy consumption as NOx capture capacity was also established and cost benefit analysis was also accomplished, providing a reference for optimizing, scaling up and comprehensively evaluating for NOx emission control via rotating packed bed. | en |
dc.description.provenance | Made available in DSpace on 2021-06-16T05:42:38Z (GMT). No. of bitstreams: 1 U0001-2407202016344900.pdf: 3422227 bytes, checksum: 112336da23b808cb73969886527fa102 (MD5) Previous issue date: 2020 | en |
dc.description.tableofcontents | Acknowledgement iii 中文摘要 iv Abstract v Table of Content vi Table of Figures ix List of Tables xiii Comments for Oral Defense xv Nomenclature xix Chapter 1. Introduction 1-1 1-1 Background 1-1 1-2 Objectives 1-4 Chapter 2. Literature Review 2-1 2-1 Waste Electrical and Electronic Equipment (WEEE) 2-1 2-2 Physicochemical Characteristics of Nitrogen Oxides 2-7 2-2-1 Solubilities of Nitrogen Oxides 2-8 2-2-2 Exposure and Impacts 2-9 2-3 Removal of Nitrogen Oxides – Oxidation/Absoprtion 2-11 2-3-1 Ozone Oxidation/Absorption 2-14 2-3-2 Hydrogen Perooxide Oxidation/Absorption 2-16 2-3-3 Chlorine Dioxide Oxidation/Absorption 2-17 2-4 HiGee Technology: Principles and Practices 2-21 2-4-1 Principles: Mass Transfer 2-21 2-4-2 Performance of Nitrogen Oxides Removal via RPB 2-26 Chapter 3. Materials and Methods 3-1 3-1 Research Framework 3-1 3-2 Materials 3-2 3-2-1 Materials 3-2 3-2-2 Apparatus 3-5 3-3 Methods 3-9 3-3-1 Experimental Design 3-9 3-3-2 Nitrogen Oxides Removal Efficiency 3-13 3-4 Analytical Methods 3-15 3-4-1 Air Pollutants Analyzer PG-350 3-15 3-4-2 Cost Benefit Analysis 3-16 Chapter 4. Results and Discussion 4-1 4-1 Evaluation of NOx Removal efficiency 4-1 4-1-1 Identification of NOx Emission from Copper Dissolution Process 4-1 4-1-2 Preliminary Evaluation of NOx Removal Using RPB Scrubbing without Chemicals 4-4 4-1-3 Comparison of Different Oxidants for NOx Removal 4-5 4-2 NOx Removal Efficiency Enhancement 4-8 4-2-1 Combination of Oxidants and Absorbents on NOx Removal 4-8 4-2-2 Effect of Gas Liquid Ratio and High Gravity Factor on NOx Removal 4-21 4-2-3 Determination of Maximum Achievable Removal Efficiency (MARE) 4-26 4-2-4 Evaluation of Actual Waste PCBs Copper Dissolution Process 4-29 4-3 Development of Kinetics and Mass Transfer Model 4-33 4-3-1 Overall Mass Transfer Coefficient (KGa), Height of Transfer Unit (HTU) and Surface Area of Transfer Unit (ATU) 4-33 4-3-2 Kinetics of Copper Dissolution Process 4-39 4-3-3 Theoretical Overall Mass Transfer Coefficient (KGa) Validation 4-43 4-3-4 Empirical Model Establishment 4-46 4-4 Energy Consumption and Cost Benefit Analysis 4-49 4-4-1 Energy Consumption for NOx Removal Process 4-50 4-4-2 Cost Benefit Analysis 4-52 Chapter 5. Conclusions and Recommendations 5-1 5-1 Conclusions 5-1 5-2 Recommendations 5-2 References I Appendix VII | |
dc.language.iso | en | |
dc.title | 利用超重力旋轉填充床去除於模擬廢印刷電路板銅回收製程中所排放氮氧化物之研究 | zh_TW |
dc.title | Nitrogen Oxides Removal from Simulated Waste Printed Circuit Board Copper Dissolution Process via a Rotating Packed Bed | en |
dc.type | Thesis | |
dc.date.schoolyear | 108-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 顧洋(Young Ku),陳奕宏(Yi-Hung Chen),林逸彬(Yi-Pin Lin),潘述元(Shu-Yuan Pan) | |
dc.subject.keyword | 氮氧化物減量,銅溶解製程,超重力技術,空污能源鏈結,成本效益分析, | zh_TW |
dc.subject.keyword | High-gravity rotating packed bed,NOx reduction,Copper dissolution,Air-energy nexus,Cost benefit analysis, | en |
dc.relation.page | 115 | |
dc.identifier.doi | 10.6342/NTU202001832 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2020-07-25 | |
dc.contributor.author-college | 工學院 | zh_TW |
dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
顯示於系所單位: | 環境工程學研究所 |
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