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  1. NTU Theses and Dissertations Repository
  2. 理學院
  3. 海洋研究所
請用此 Handle URI 來引用此文件: http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/55449
完整後設資料紀錄
DC 欄位值語言
dc.contributor.advisor魏慶琳(Ching-Ling Wei)
dc.contributor.authorWei-Li Linen
dc.contributor.author林韋利zh_TW
dc.date.accessioned2021-06-16T04:03:05Z-
dc.date.available2018-02-04
dc.date.copyright2015-02-04
dc.date.issued2014
dc.date.submitted2014-10-13
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Buesseler, K.O., Benitez-Nelson, C.R., Moran, S.B., Burd, A., Charette, M., Cochran, J.K., Coppola, L., Fisher, N.S., Fowler, S.W., Gardner, W.D., Guo, L.D., Gustafsson, O., Lamborg, C., Masque, P., Miquel, J.C., Passow, U., Santschi, P.H., Savoye, N., Stewart, G., Trull, T., 2006. An assessment of particulate organic carbon to thorium-234 ratios in the ocean and their impact on the application of Th-234 as a POC flux proxy. Marine Chemistry 100: 213-233.
Burd, A.B., Moran, S.B., Jackson, G.A., 2000. A coupled adsorption-aggregation model of the POC/Th-234 ratio of marine particles. Deep-Sea Research Part I 47: 103-120.
Chen, W.F., Cai, P.H., Dai, M.H., Wei, J.F., 2008. Th-234/U-238 disequilibrium and particulate organic carbon export in the northern South China Sea. Journal of Oceanography 64: 417-428.
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Dunne, J.P., Murray, J.W., Rodier, M., Hansell, D.A., 2000. Export flux in the western and central equatorial Pacific: zonal and temporal variability. Deep-Sea Research Part I 47: 901-936.
Guo, L.D., Hung, C.C., Santschi, P.H., Walsh, I.D., 2002. Th-234 scavenging and its relationship to acid polysaccharide abundance in the Gulf of Mexico. Marine Chemistry 78: 103-119.
Guo, L.D., Santschi, P.H., Baskaran, M., 1997. Interactions of thorium isotopes with colloidal organic matter in oceanic environments. Colloids and Surfaces a-Physicochemical and Engineering Aspects 120: 255-271.
Heyraud, M., Fowler, S.W., Beasley, T.M., Cherry, R.D., 1976. Polonium-210 in Euphausiids - Detailed Study. Marine Biology 34: 127-136.
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Hung, C.C., Gong, G.C., 2010. POC/Th-234 ratios in particles collected in sediment traps in the northern South China Sea. Estuarine Coastal and Shelf Science 88: 303-310.
Hung, C.C., Gong, G.C., Santschi, P.H., 2012. Th-234 in different size classes of sediment trap collected particles from the Northwestern Pacific Ocean. Geochimica Et Cosmochimica Acta 91: 60-74.
Hung, C.C., Guo, L.D., Roberts, K.A., Santschi, P.H., 2004. Upper ocean carbon flux determined by the Th-234 approach and sediment traps using size-fractionated POC and Th-234 data from the Gulf of Mexico. Geochemical Journal 38: 601-611.
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Murray, J.W., Young, J., Newton, J., Dunne, J., Chapin, T., Paul, B., McCarthy, J.J., 1996. Export flux of particulate organic carbon from the central equatorial pacific determined using a combined drifting trap Th-234 approach. Deep-Sea Research Part II 43: 1095-1132.
Nozaki, Y., Tsubota, H., Kasemsupaya, V., Yashima, M., Ikuta, N., 1991. Residence times of surface-water and particle-reactive Pb-210 and Po-210 in the East China and Yellow Seas. Geochimica Et Cosmochimica Acta 55: 1265-1272.
Nozaki, Y., Tsunogai, S., 1976. Ra-226, Pb-210 and Po-210 disequilibria in western North-Pacific. Earth and Planetary Science Letters 32: 313-321.
Passow, U., 2002. Transparent exopolymer particles (TEP) in aquatic environments. Progress in Oceanography 55: 287-333.
Passow, U., Dunne, J., Murray, J.W., Balistrieri, L., Alldredge, A.L., 2006. Organic carbon to Th-234 ratios of marine organic matter. Marine Chemistry 100: 323-336.
Quigley, M.S., Santschi, P.H., Hung, C.C., Guo, L.D., Honeyman, B.D., 2002. Importance of acid polysaccharides for Th-234 complexation to marine organic matter. Limnology and Oceanography 47: 367-377.
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Santschi, P.H., Murray, J.W., Baskaran, M., Benitez-Nelson, C.R., Guo, L.D., Hung, C.C., Lamborg, C., Moran, S.B., Passow, U., Roy-Barman, M., 2006. Thorium speciation in seawater. Marine Chemistry 100: 250-268.
Shannon, L.V., Cherry, R.D., Orren, M.J., 1970. Po-210 and Pb-210 in marine environment. Geochimica Et Cosmochimica Acta 34: 701-711.
Stewart, G., Cochran, J.K., Miquel, J.C., Masque, P., Szlosek, J., Baena, A.M.R.Y., Fowler, S.W., Gasser, B., Hirschberg, D.J., 2007. Comparing POC export from Th-234/U-238 and Po-210/Pb-210 disequilibria with estimates from sediment traps in the northwest Mediterranean. Deep-Sea Research Part I 54: 1549-1570.
Stewart, G., Moran, S.B., Lomas, M.W., Kelly, R.P., 2011. Direct comparison of Po-210, Th-234 and POC particle-size distributions and export fluxes at the Bermuda Atlantic Time-series Study (BATS) site. Journal of Environmental Radioactivity 102: 479-489.
Tateda, Y., Carvalho, F.P., Fowler, S.W., Miquel, J.C., 2003. Fractionation of Po-210 and Pb-210 in coastal waters of the NW Mediterranean continental margin. Continental Shelf Research 23: 295-316.
Tateda, Y., Yamamoto, M., 1997. The residence time of Po-210 and Pb-210 related to plankton in surface waters off Misaki, Japan. Radioprotection-Colloques 32: 163-168.
Wei, C.L., Chen, P.R., Lin, S.Y., Sheu, D.D., Wen, L.S., Chou, W.C., (in press) Distributions of 210Pb and 210Po in surface water surrounding Taiwan: A synoptic observation.Deep-Sea Research Part II, doi: 10.1016/j.dsr2.2014.04.010.
Wei, C.L., Lin, S.Y., Sheu, D.D., Chou, W.C., Yi, M.C., Santschi, P.H., Wen, L.S., 2011. Particle-reactive radionuclides (Th-234, Pb-210, Po-210) as tracers for the estimation of export production in the South China Sea. Biogeosciences 8: 3793-3808.
Wei, C.L., Murray, J.W., 1992. Temporal variations of 234Th activity in the water column of Dabob Bay - Particle Scavenging. Limnology and Oceanography 37: 296-314.
Wei, C.L., Murray, J.W., 1994. The behavior of scavenged isotopes in marine anoxic environments - Pb-210 and Po-210 in the water column of the Black-Sea. Geochimica Et Cosmochimica Acta 58: 1795-1811.
Yang, W.F., Huang, Y.P., Chen, M., Zhang, L., Li, H.B., Liu, G.S., Qiu, Y.S., 2006. Disequilibria between Po-210 and Pb-210 in surface waters of the southern South China Sea and their implications. Science in China Series D-Earth Sciences 49: 103-112.
邱薰慧,2000。台灣周圍海域浮游生物釙-210 和鉛-210含量及釙-210 之富集現象,國立中山大學海洋地質及化學研究所碩士論文,49 頁。
dc.identifier.urihttp://tdr.lib.ntu.edu.tw/jspui/handle/123456789/55449-
dc.description.abstract為了探討不同粒徑的懸浮顆粒對天然放射核種清除作用的關係,本研究於台灣西南海域採集表水懸浮顆粒進行粒徑分樣共得到九組粒徑大小 (0.45-10 µm、10-63 µm、63-153 µm、>153 µm、202-363 µm、363-500 µm、500-1000 µm、1000-2000 µm、>2000 µm) 之顆粒體,分別測量各組粒徑顆粒體中的234Th、210Pb、210Po活度及有機碳 (POC)、氮 (PN)、無機碳 (PIC)濃度。由234Th、210Pb、210Po重量活度隨顆粒粒徑無系統性變化,可看出三個核種皆屬於表面吸附元素,然而210Po在粒徑大於500 µm時,重量活度有隨顆粒粒徑增加的現象,顯示210Po除了具有表面吸附特性外,也可能隨營養階層累積於顆粒體內。三個核種的分佈係數 (Kd) 在各粒徑懸浮顆粒的親顆粒相對程度顯示之順序為210Po>234Th>210Pb,與文獻呈現之沉降顆粒與三核種的結合順序相同。利用母子核種不平衡模式估算有機碳通量、氮通量、或是無機碳通量時,顆粒體內碳、氮、無機碳與核種濃度 (RN) 的比值 (POC/RN、PN/RN、PIC/RN) 影響準確度最大,而顆粒粒徑大小則是影響POC/RN、PN/RN、PIC/RN變化重要的因子,本研究顯示POC/234Th、PN/234Th、PIC/234Th比值在小粒徑顆粒體的變化範圍皆較拖網所採集之大粒徑顆粒小,並且在0.45-10 µm粒徑顆粒中的變化最小;POC/210Pb、PN/210Pb在0.45-10 µm粒徑顆粒比值變化最小,PIC/210Pb隨顆粒粒徑無系統性變化;POC/210Po、PN/210Po比值在0.45-10 µm粒徑顆粒比值變化最小,而變化幅度隨粒徑增加逐漸變小,PIC/210Po隨顆粒粒徑無系統性關係。與過往在南海所觀測沉降顆粒POC/RN、PN/RN、PIC/RN平均值比較,沉降顆粒與0.45-10 µm粒徑顆粒的比值較相近。本研究210Po/210Pb在不同顆粒粒徑大小下普遍大於1,比值與顆粒粒徑之間並無明顯關係。zh_TW
dc.description.provenanceMade available in DSpace on 2021-06-16T04:03:05Z (GMT). No. of bitstreams: 1
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Previous issue date: 2014
en
dc.description.tableofcontents口試委員會審定書 I
誌謝 II
摘要 III
Abstract IV
目錄 V
圖目錄 VII
表目錄 IX
第一章 緒論 1
1-1 海洋顆粒有機碳垂直輸出通量的重要性 1
1-2 利用親顆粒核種研究海洋清除現象 2
1-3 234Th, 210Pb, 210Po的生地化行為差異 3
1-4 研究目的與動機 4
第二章 實驗方法 5
2-1 航次資訊 5
2-2 現場工作 5
2-3 實驗分析方法 5
2-3.1 實驗室分樣 5
2-3.2 234Th分析 6
2-3.3 210Po分析 6
2-3.3.1 210Po顆粒相分析方法 6
2-3.3.2 210Po溶解相分析方法 7
2-3.4 210Pb分析 7
2-3.5 顆粒態有機碳、氮、無機碳分析方法 7
第三章 實驗結果 9
3-1 顆粒態有機碳、氮、無機碳 9
3-2 234Th活度 9
3-3 210Pb活度 10
3-4 210Po活度 11
第四章 討論 27
4-1 顆粒體組成、大小對重量活度之影響 27
4-2 POC、PN、PIC與放射核種活度比值關係 33
4-3 顆粒體粒徑大小對分佈係數 (Kd) 之影響 40
4-4 不同顆粒粒徑大小下之210Po/210Pb比值 44
第五章 結論 46
參考文獻 48
dc.language.isozh-TW
dc.subject懸浮顆粒zh_TW
dc.subject粒徑zh_TW
dc.subject234Thzh_TW
dc.subject210Pbzh_TW
dc.subject210Pozh_TW
dc.subject210Poen
dc.subjectsuspended particleslen
dc.subjectsizeen
dc.subject234Then
dc.subject210Pben
dc.title海洋懸浮顆粒中210Pb、210Po與234Th濃度與顆粒粒徑之關係zh_TW
dc.title210Pb,210Po, and 234Th in Size - fractionated Marine Particlesen
dc.typeThesis
dc.date.schoolyear103-1
dc.description.degree碩士
dc.contributor.oralexamcommittee溫良碩,洪慶章
dc.subject.keyword懸浮顆粒,粒徑,234Th,210Pb,210Po,zh_TW
dc.subject.keywordsuspended particlesl,size,234Th,210Pb,210Po,en
dc.relation.page53
dc.rights.note有償授權
dc.date.accepted2014-10-14
dc.contributor.author-college理學院zh_TW
dc.contributor.author-dept海洋研究所zh_TW
顯示於系所單位:海洋研究所

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