請用此 Handle URI 來引用此文件:
http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/53971完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 林正芳 | |
| dc.contributor.author | Szu-Yu Wu | en |
| dc.contributor.author | 吳偲瑀 | zh_TW |
| dc.date.accessioned | 2021-06-16T02:35:06Z | - |
| dc.date.available | 2018-07-29 | |
| dc.date.copyright | 2015-07-29 | |
| dc.date.issued | 2015 | |
| dc.date.submitted | 2015-07-28 | |
| dc.identifier.citation | Aiken, G.R., McKnight, D.M., Thorn, K.A. and ThurmanE.M. (1992) Isolation of hydrophilic organic acids from water using nonionic macroporous resins. Organic Geochemistry, 18(4), 567-574.
Al-Degs, Y.S., El-Barghouthi, M.I., El-Sheikh, A.H. and Walker, G.M. (2008) Effect of solution ph, ionic strength, and temperature on adsorption behavior of reactive dyes on activated carbon. Dyes and Pigments, 77(1), 16-24. Álvarez-Uriarte, J.I., Iriarte-Velasco, U., Chimeno-Alanís, N. and González-Velasco, J.R. (2010) The effect of mixed oxidants and powdered activated carbon on the removal of natural organic matter. Journal of Hazardous Materials, 181, 431-437. Amy, G.L., Tan, L. and Davis, M.K. (1991) The effects of ozonation and activated carbon adsorption on trihalomethane speciation. Water Research, 25(2), 191-203. APHA (1992) Standard methods for the examination of water and wastewater. American Public Health Association, American Water Works Association, Water Environment Federation, Washington D.C., Barker, D.J. and Stuckey, D.C. (1999) A review of soluble microbial products (smp) in wastewater treatment systems. Water Research, 33(14), 3063-3082. Becker, W.C. and O'Melia, C.R. (2001) Ozone: Its effect on coagulation and filtration. Water Science and Technology, 1(4), 81-88. Bose, P. and Reckhow, D.A. (2007) The effect of ozonation on natural organic matter removal by alum coagulation. Water Research, 41, 1524-1533. Chang, C.-Y., Hsieh, Y.-H., Lin, Y.-M., Hu, P.-Y., Liu, C.-C. and Wang, K.-H. (2001) The organic precursors affecting the formation of disinfection by-products with chlorine dioxide. Chemosphere, 44(5), 1153-1162. Chang, S.D. and Singer, P.C. (1991) The impact of ozonation on particle stability and the removal of toc and thm precursors. WATER RESOURCES, 83(3), 71-80. Chiang, P.C., Chang, E.E. and Liang, C.H. (2002) Nom characteristics and treatabilities of ozonation processes. Chemosphere, 46(8), 929-946. Childress, A.E. and Elimelech, M. (1996) Effect of solution chemistry on the surface charge of polymeric reverse osmosis and nanofiltration membranes. Journal of Membrane Science, 119(2), 253-268. Chingombe, P., Saha, B. and Wakeman, R.J. (2005) Surface modification and characterisation of a coal-based activated carbon. Carbon, 43, 3143-3155. Ciora Jr., R.J. and Liu, P.K.T. (2003) Ceramic membranes for environmental related applications. Fluid: Particle Separation Journal, 15, 51-61. Cornel, P.K., Summers, R.S. and Roberts, P.V. (1986) Diffusion of humic acid in dilute aqueous solution. Journal of Colloid and Interface Science, 110(1), 149-163. Dong, Y., Chen, S., Zhang, X., Yang, J., Liu, X. and Meng, G. (2006) Fabrication and characterization of low cost tubular mineral-based ceramic membranes for micro-filtration from natural zeolite. Journal of Membrane Science, 281, 592-560. Ebie, K., Li, F., Azuma, Y., Yuasa, A. and Hagishit, T. (2001) Pore distribution effect of activated carbon in adsorbing organic micropollutants from natural water. Water Research, 35(1), 167-180. Edzwald, J.K. (1993) Coagulation in drinking water treatment: Particles, organics and coagulants. Water Science and Technology, 27(11), 21-36. Evansa, P.J., Birda, M.R., Pihlajamäkib, A. and Nyströmb, M. (2008) The influence of hydrophobicity, roughness and charge upon ultrafiltration membranes for black tea liquor clarification. Journal of Membrane Science, 313(1-2), 250-259. Fan, L., Harris, J.L., Roddick, F.A. and Booker, N.A. (2001) Influence of the characteristics of natural organic matter on the fouling of microfiltration membranes. Water Research, 35(18), 4455-4463. Flemming, H.-C., Schaule, G., Griebe, T., Schmit, J. and Tamachkiarowa, A. (1997) Biofouling-the achilles heel of membrane processes. Desalination, 113(2-3), 215-226. Haberkamp, J., Ruhla, A.S., Ernstb, M. and Jekela, M. (2007) Impact of coagulation and adsorption on doc fractions of secondary effluent and resulting fouling behaviour in ultrafiltration. Water Research, 41, 3794-3601. Ho, L. and Newcombe, G. (2005) Effect of nom, turbidity and floc size on the pac adsorption of mib during alum coagulation. Water Research, 39(15), 3668-3676. Hofs, B., Ogier, J., Vries, D., Beerendonk, E.F. and Cornelissen, E.R. (2011) Comparison of ceramic and polymeric membrane permeability and fouling using surface water. Separation and Purification Technology, 79(3), 365-375. Hsu, C.-H., Jeng, W.-L., Chang, R.-M., Chien, L.-C. and Han, B.-C. (2001) Estimation of potential lifetime cancer risks for trihalomethanes from consuming chlorinated drinking water in taiwan Environmental Research, 85(2), 77-83. Humbert, H., Gallard, H., Suty, H. and Croué, J.-P. (2008) Natural organic matter (nom) and pesticides removal using a combination of ion exchange resin and powdered activated carbon (pac). Water Research, 42(6-7), 1635-1649. Jekel, M.R. (1985) Interactions of humic acids and aluminum salts in the flocculation process. Water Research, 20(12), 1535-1543. Kang, I.-J., Yoon, S.-H. and Lee, C.-H. (2002) Comparison of the filtration characteristics of organic and inorganic membranes in a membrane-coupled anaerobic bioreactor. Water Research, 36(7), 1803-1814. Kilduff, J.E., Karanfil, T., Chin, Y.-P. and Weber, W.J. (1996) Adsorption of natural organic polyelectrolytes by activated carbon: A size-exclusion chromatography study. Environmental Science and Technology, 30(4), 1336-1344. Korshina, G., Chowb, C.W.K., Fabrisb, R. and Drikas, M. (2009) Absorbance spectroscopy-based examination of effects of coagulation on the reactivity of fractions of natural organic matter with varying apparent molecular weights. Water Research, 43, 1541-1549. Kristiana, I., Joll, C. and Heitz, A. (2011) Powdered activated carbon coupled with enhanced coagulation for natural organic matter removal and disinfection by-product control: Application in a western australian water treatment plant. Chemosphere, 83, 661-668. Langlais, B., Reckhow, D. and DR, B. (1991) Ozone in water treatment: Application and engineering. Lewis Publishers, Larry B, B., Jerry A, L. and Eric A, N. (2001) Nature and transformation of dissolved organic matter in treatment wetlands. Environmental Science and Technology, 35(24), 4805-4817. Lee, S.J., Dilaver, M., Park, P.-K. and Kim, J.-H. (2013) Comparative analysis of fouling characteristics of ceramic and polymeric microfiltration membranes using filtration models. Journal of Membrane Science, 432, 97-105. Leenheer, J.A. and Croue, J.P. (2003) Characterizing aquatic dissolved organic matter. Environmental Science and Technology, 37(1), 18-27. Li, Q. and Elimelech, M. (2004) Organic fouling and chemical cleaning of nanofiltration membranes: Measurements and mechanisms. Environmental Science and Technology, 38(17), 4683-4694. Lin, C.-F., Huang, Y.-J. and Hao, O.J. (1999) Ultrafiltration processes for removing humic substances: Effect of molecular weight fractions and pac treatment. Water Research, 33(5), 1252-1265. Lin, C.-F., Lin, A.Y.-C., Chandan, P.S. and Tsai, C.-Y. (2009) Effects of mass retention of dissolved organic matter and membrane pore size on membrane fouling and flux decline. Water Research, 43(2), 389-394. Liu, H., Wang, D., Wang, M., Tang, H. and Yang, M. (2007) Effect of pre-ozonation on coagulation with ipf-pacls: Role of coagulant speciation. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 294(1-3), 1111-1118. Matilainen, A., Vieno, N. and Tuhkanen, T. (2006) Efficiency of the activated carbon filtration in the natural organic matter removal. Environment International, 32(3), 324-331. Matilainen, A., Vepsäläinen, M. and Sillanpää, M. (2010) Natural organic matter removal by coagulation during drinking water treatment: A review. Advances in Colloid and Interface Science, 159 197-206. Metzger, U., Le-Clech, P., Stuetz, R.M., Frimmel, F.H. and Chen, V. (2007) Characterisation of polymeric fouling in membrane bioreactors and the effect of different filtration modes. Journal of Membrane Science, 301(1-2), 180-190. Meunier, L., Canonic, S. and Gunten, U.v. (2006) Implications of sequential use of uv and ozone for drinking water quality. Water Research, 40(9), 1864-1878. Moulin, C., Bourbigot, M.M., Tazipain, A. and Bourdon, F. (1991) Design and performance of membrane filtration installations – capacity and product quality for drinking-water applications. Environmental Technology, 12, 841-859. Najm, I., Tate, C. and Selby, D. (1998) Optimizing enhanced coagulation with pac: A case study. Carbon, 90(10), 88-96. Najm, I.N., Patania, N.L., Jacangelo, J.G. and Krasner, S.W. ( 1994) Evaluating surrogates for disinfection by-products Journal - American Water Works Association, 86, Number 6, 98-106. Newcombe, G. (2006) Chapter 8: Removal of natural organic material and algal metabolites using activated carbon. Interface Science and Technology, 10, 133-154. Oh, H.K., Takizawa, S., Ohgaki, S., Katayama, H., Oguma, K. and Yu, M.J. (2007) Removal of organics and viruses using hybrid ceramic mf system without draining pac. Desalination, 202, 191-200. Owen, D.M., Amy, G.L., Chowdhury, Z.K., Paode, R., McCoy, G. and Viscosil, K. (1995) Nom characterization and treatability. American Water Works Association, 87(1), 46-64. Pelekani, C. and Snoeyink, V.L. (1999) Competitive adsorption in natural water: Role of activated carbon pore size. Water Research, 33(5), 1209-1220. Pham, A.N., Rose, A.L., Feitz, A.J. and Waite, T.D. (2006) Kinetics of fe(iii) precipitation in aqueous solutions at ph 6.0–9.5 and 25 c. Geochimica et Cosmochimica Acta, 70, 640-651. Piccolo, A. (2002) The supramolecular structure of humic substances: A novel understanding of humus chemistry and implications in soil science. Advances in Agronomy, 75, 57-135. Rodríguez-reinoso, F. (1998) The role of carbon materials in heterogeneous catalysis Carbon, 36(3), 159-174. Selcuk, H., Rizzo, L., Belgiorno, V., Nikolaou, A.N., Bekbolet, M. and Meric, S. (2007) Dbps formation and toxicity monitoring in different origin water treated by ozone and alum/pac coagulation. Desalination, 210, 31-44. Sharp, E.L., Parsons, S.A. and Jefferso, B. (2006) The impact of seasonal variations in doc arising from a moorland peat catchment on coagulation with iron and aluminium salts. Environmental Pollution, 140, 436-444. Siddiqui, M.S., Amy, G.L. and Murphy, B.D. (1997) Ozone enhanced removal of natural organic matter from drinking water sources. Water Research, 31(12), 3098-3106. Singer, P.C. (1990) Assessing ozonation research needs in water treatment. 82(10), 78-88. Summers, R.S. and Roberts, P.V. (1988) Activated carbon adsorption of humic substances: Ii. Size exclusion and electrostatic interactions. Journal of Colloid and Interface Science, 122(2), 382-389. Szlachta, M. and Adamski, W. (2009) Effects of natural organic matter removal by integrated processes: Alum coagulation and pac-adsorption. Water Science and Technology, 59(10), 1951-1958. Thurman, E.M. (1985) Organic geochemistry of natural waters: M. Nijhoff., Tomaszewska, M., Mozi, S. and Morawski, A.W. (2004) Removal of organic matter by coagulation enhanced with adsorption on pac. Desalination, 161(1), 79-89. Treguer, R., Tatin, R., Couvert, A., Wolbert, D. and Tazi-Pain, A. (2010) Ozonation effect on natural organic matter adsorption and biodegradation – application to a membrane bioreactor containing activated carbon for drinking water production. Water Research, 44, 781-790. Tsuru, T. (2001) Inorganic porous membranes for liquid phase separation. Separation and Purification Methods, 30, 191-201. Uyak, V., Yavuz, S., Toroz, I., Ozaydin, S. and Genceli, E.A. (2007) Disinfection by-products precursors removal by enhanced coagulation and pac adsorption. Desalination, 216, 334-335. Volk, C., Bell, K., Ibrahim, E., Verges, D., Amy, G. and LeChevallier, M. (2000) Impact of enhanced and optimized coagulation on removal of organic matter and its biodegradable fraction in drinking water. Water Research, 34(12), 3247-3258. von Gunten, U. and Elovitz, M.S. (1999) Hydroxyl radical/ozone ratios during ozonation processes. I. The rct concept. Ozone: Science and Engineering, 21, 239-271. Wert, E.C., Rosario-Ortiz, F.L., Drury, D.D. and Snyder, S.A. (2007) Formation of oxidation byproducts from ozonation of wastewater. Water Research, 41(7), 1481-1491. Wert, E.C., Gonzales, S., Dong, M.M. and Rosario-Ortiz, F.L. (2011) Evaluation of enhanced coagulation pretreatment to improve ozone oxidation efficiency in wastewater. Water Research, 45, 5191-5200. Yan, M., Wang, D., You, S., Qu, J. and Tang, H. (2006) Enhanced coagulation in a typical north-china water treatment plant. Water Research, 40, 3621-3628. Yan, M., Wan, D., Shi, B., Wang, M. and Yan, Y. (2007) Effect of pre-ozonation on optimized coagulation of a typical north-china source water. Chemosphere, 69(11), 1695-1703. Zhan, X., Gao, B., Yue, Q., Liu, B., Xu, X. and Li, Q. (2010) Removal natural organic matter by coagulation–adsorption and evaluating the serial effect through a chlorine decay mode. Journal of Hazardous Materials, 183(1-3), 279-287. Zhao, Z.-Y., Gu, J.-D., Li, H.-B., Li, X.-Y. and Leung, K.M.-Y. (2009) Disinfection characteristics of the dissolved organic fractions at several stages of a conventional drinking water treatment plant in southern china. Journal of Hazardous Materials, 172, 1099- Zhu, H.T., Wen, X.H. and Huang, X. (2008) Pre-ozonation for dead-end microfiltration of the secondary effluent: Suspended particles and membrane fouling. Desalination, 231, 166-175. 行政院環境保護署 (1997) 飲用水水源水質標準,第五條. 林玠佑 (2014). 強化混凝結合薄膜系統去除消毒程序前肢水中溶解性有機質 國立台灣大學環境工程學研究所碩士論文 | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/53971 | - |
| dc.description.abstract | 金門太湖為太湖淨水場之水源,水源中含高濃度之有機物質,無法有效地利用現有之傳統淨水程序去除,因此為提升太湖淨水場出水水質,本研究擬以混凝-薄膜-臭氧,進一步去除快濾單元出水之溶解性有機物質(Dissolved organic matter, DOM),以達我國飲用水水質4 mg TOC /L之標準。Lin(2014)以吸附混凝去除有機質,利用陶瓷膜,無沉澱直接過濾混凝膠羽,其出水DOC仍然高於4 mg TOC /L。本研究延續該實驗,今以原吸附混凝接續陶瓷膜過濾之淨水程序為基礎,再增加臭氧處理,觀察DOC之變化,利用優選反洗程序,延長陶瓷膜過濾使用時間,為解析有機組成之去除與殘留,本研究分析各流程殘餘有機物之親疏水性分布與分子量大小,提供金門太湖淨水場實際應用參考。
優選臭氧順序與劑量為:吸附混凝後以陶瓷膜過濾水中膠羽,再以0.8 mg ozone/ mg DOC之臭氧處理有機物質,此優選程序可將快濾出水由10.87 mg TOC /L降至1.57 mg TOC /L,結果可達我國飲用水水質4 mg TOC /L標準,為使陶瓷膜使用時間增長,反洗程序以每兩小時操作一次,優選反洗程序為三次物理反洗結合一次化學反洗,可將透膜壓差恢復至100%。吸附混凝可去除64%之疏水性有機物質及44%之親水性有機物質,臭氧處理後,疏水性有機物質去除率可達88 %,親水性有機物質去除率可達78 %。分子量大小分布之探討,經粉狀活性碳後,分子量介於3,000 – 300 Da有機物質有較高之去除率;混凝後,分子量介於30,000 – 3,000 Da有機物質有較高之去除率;臭氧對於分子量介於10,000 – 3,000 Da與1,000 – 300 Da有機物質有較高之去除率。 | zh_TW |
| dc.description.abstract | The removal of dissolved organic matter (DOM) by conventional treatment processes in drinking water treatment plants (DWTPs) has been ineffective in Tai-lake on Kinmen. In this study, various advanced treatments were tested for DOM removal. Combined the result by Lin., (2014), this year, Enhanced coagulation, Powdered activated carbon (PAC), ceramic membrane (CM), and ozone were used in various combinations to effect removal of DOM in the DWTP in Kinmen, Taiwan. The rapid sand filtration effluent from the Tai Lake DWTP of Kinmen, Taiwan with DOC of 10.87 mg/L was treated with poly aluminum chloride (PACL) as a coagulant and DOC reduction was measured by DOC and UV absorbance at 254 nm. The molecular size distribution (MSD) of DOM was investigated using gel filtration chromatography (GFC) and its hydrophilic/hydrophobic (HPI/HPO) characteristics using the DAX-8 resin. DOM removal efficiency was improved when EC and PAC were used prior to CM and ozone, resulting in removal of DOC from 10.87 to 1.57 mg TOC /L with corresponding decrease in UV254 from 0.087 to 0.013. The removal efficiencies for DOCHPO and DOCHPI were 88% and 79%, respectively. The PAC could adsorb more low molecular weight (MW) organic matter, and the high MW organic matter could be more efficiently removed by PACL as well as ozone. This process shows promise in improving DOM removal and the potential to increase compliance with the drinking water standard of Taiwan. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-16T02:35:06Z (GMT). No. of bitstreams: 1 ntu-104-R02541104-1.pdf: 1588672 bytes, checksum: 26d18692a405e14fef19feae24b2258c (MD5) Previous issue date: 2015 | en |
| dc.description.tableofcontents | 口試委員審定書 I
誌謝 II 摘要 III Abstract IV 總目錄 V 圖目錄 VIII 表目錄 X 第一章 前言 1 1-1 研究緣起 1 1-2 研究目的 2 1-3 研究內容 3 第二章 文獻回顧 2 2-1 溶解性有機物質 2 2-1-1 溶解性有機物質之組成與特性 2 2-2 混凝結合活性碳 4 2-2-1 混凝 4 2-2-2 粉狀活性碳 4 2-2-3 混凝結合粉狀活性碳 6 2-3 臭氧 7 2-3-1 臭氧處理溶解性有機物質 8 2-4 薄膜技術 10 2-4-1 薄膜之種類及材質 10 2-4-2 陶瓷膜 12 2-4-3 積垢與反沖洗 13 第三章 實驗方法與材料 14 3-1 實驗內容與項目 14 3-1-1 實驗內容 14 3-1-2 實驗項目 14 3-2 實驗流程 15 3-3 實驗材料與設備 18 3-3-1 實驗原水 18 3-3-2 混凝設備 18 3-3-3 臭氧製造機 18 3-3-4 薄膜模組 19 3-3-5 DAX-8設備與藥品 24 3-3-6 膠凝過濾設備與藥品 25 3-4 分析儀器與方法 26 3-4-1 溶解性有機碳 26 3-4-2 紫外光吸收值 26 3-4-3 Specific UV Absorbance 26 3-4-4 液相臭氧濃度 27 3-5 實驗步驟與方法 28 3-5-1 混凝吸附 28 3-5-2 薄膜過濾 28 3-5-3 臭氧處理 29 3-5-4 DAX-8樹脂 31 3-5-5 膠凝過濾 31 第四章 結果與討論 34 4-1 原水水質分析 34 4-2 臭氧反應時間 35 4-3 臭氧劑量 36 4-3-1 臭氧接續吸附混凝 36 4-3-2 吸附混凝接續臭氧 39 4-3-3 優選操作順序 41 4-4 陶瓷膜過濾 44 4-5 親疏水性分布 46 4-6 分子量分布 48 第五章 結論與建議 50 5-1 結論 50 5-2 建議 51 參考文獻 52 | |
| dc.language.iso | zh-TW | |
| dc.subject | 陶瓷膜過濾 | zh_TW |
| dc.subject | 粉狀活性碳 | zh_TW |
| dc.subject | 臭氧 | zh_TW |
| dc.subject | 膠凝過濾層析樹脂 | zh_TW |
| dc.subject | 強化混凝 | zh_TW |
| dc.subject | DAX-8樹脂 | zh_TW |
| dc.subject | Coagulation | en |
| dc.subject | dissolved organic matter | en |
| dc.subject | ozone | en |
| dc.subject | powder activated carbon | en |
| dc.subject | ceramic membrane | en |
| dc.title | 強化混凝-臭氧-薄膜處理提升過濾程序出水
溶解性有機物質之去除 | zh_TW |
| dc.title | Improving Dissolved Organic Matter Removal
by Enhanced Coagulation-Membrane-Ozone Process | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 103-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 駱尚廉,康佩群,吳忠信,侯嘉宏 | |
| dc.subject.keyword | 強化混凝,粉狀活性碳,陶瓷膜過濾,臭氧,DAX-8樹脂,膠凝過濾層析樹脂, | zh_TW |
| dc.subject.keyword | Coagulation,ceramic membrane,dissolved organic matter,ozone,powder activated carbon, | en |
| dc.relation.page | 65 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2015-07-28 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| 顯示於系所單位: | 環境工程學研究所 | |
文件中的檔案:
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| ntu-104-1.pdf 未授權公開取用 | 1.55 MB | Adobe PDF |
系統中的文件,除了特別指名其著作權條款之外,均受到著作權保護,並且保留所有的權利。
