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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 劉懷勝(Hwai-Shen Liu) | |
dc.contributor.author | Yi-Chun Liao | en |
dc.contributor.author | 廖翊淳 | zh_TW |
dc.date.accessioned | 2021-06-15T11:19:47Z | - |
dc.date.available | 2021-02-20 | |
dc.date.copyright | 2021-02-20 | |
dc.date.issued | 2021 | |
dc.date.submitted | 2021-02-08 | |
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(2004). 錯流式旋轉填充床之特性研究. 國立臺灣大學化學工程學研究所學位論文 郭林雅, 祁貴生, 劉有智, 邱錦堂, 蘇法雙. (2019). 液體初始分散對錯流旋轉填料床傳質性能的影響. 中北大學學報(自然科學版)(02). 陳敬銘. (2006). 錯流式旋轉填充床中質傳之研究. 國立臺灣大學化學工程學研究所學位論文 董梅英, 祁貴生, 劉有智, 郭強, 宋彬, 王探. (2015). 錯流旋轉填料床傳質特性影響因素的實驗研究. 過程工程學報(06). 劉奕瑩. (2008). 旋轉填充床之疏水性有機揮發物質的質傳研究. 國立臺灣大學化學工程學研究所學位論文 蔡詞伊. (2011). 以矽油加水在旋轉填充床吸收甲苯之研究. 國立臺灣大學化學工程學研究所學位論文 | |
dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/49220 | - |
dc.description.abstract | 現今的工業排放廢氣中常會含有親水性和親油性的有機揮發性氣體(VOCs)。為了同時處理這種工業廢氣,我們實驗室先前的研究以水跟矽油在旋轉填充床(RPB)中吸收甲苯和異丙醇氣體,結果表明這是可行且有效的方法,同時也發現了加入矽油會使水對異丙醇的吸收效率下降;反之加入水會使矽油吸收甲苯的效率提升。 我們將水吸收親水性VOCs和矽油吸收親油性VOCs的質傳係數經驗迴歸式延展到油水系統,發現當把水跟矽油的物理性質視為各自獨立比視為混合的結果要更符合事實。但在此前提下,經驗迴歸式得到的KGa跟實驗得到的KGa仍有超過30%的誤差。為了校正此誤差,我們定義出 和 來代表添加第二種溶液與添加前的有效氣液接觸面積的比值,並得到 和 的經驗迴歸式。之後我們基於矽油跟水的流態性質和monte carlo方法估算出 和 。最後將水吸收親水性VOCs和矽油吸收親油性VOCs的質傳係數經驗迴歸式分別乘上 跟 ,使得KGa的估計值和實驗值的誤差大多落在30%內。 油水混合液吸收異丙醇、油水混合液吸收甲苯的質傳經驗迴歸式如下: (K_G a)/(D_G a_t^2 )=0.0186〖Re〗_G^0.389 〖Re〗_L^0.534 〖Gr〗_G^0.245 H_y^(-0.185) α_water (K_G a)/(D_G a_t^2 )=0.0231〖Re〗_G^0.315 〖Re〗_L^0.389 〖Gr〗_G^0.248 H_y^(-0.31) α_oil α_water=0.14L_o^(-1.08) L_w^0.23 φ^0.83 α_oil=2.21-1.21φ | zh_TW |
dc.description.abstract | The VOCs (volatile organic compounds) emitted from industries may often include both hydrophobic and hydrophilic compounds. For the purpose of absorbing these VOCs simultaneously, we use mixture of water and silicone oil as the adsorbent to absorb isopropanol (IPA) and toluene in rotating packed bed (RPB). In our previous work, the experiments were successfully demonstrated intensified mass transfer by centrifugal force as expected. However, it was found that the absorption fraction of toluene by water/silicone oil system was higher than those of toluene by oil only for most result. In contrast, most of the absorption fraction of isopropanol by water/silicone oil system was lower than those of isopropanol by water only. This phenomeon may be attributed to coalescence of water and oil liquid drops in void of the bed or the similar effects, resulting in the change of surface area. In order to obtain the overall mass transfer coefficient (KGa) for water and oil in this mixed absorbents system numerically, we extended the correlations of KGa of isopropanol/water and toluene/silicone oil system to the dual absorbents system, it was found that the best results were obtained when physical properties of each absorbents were taken individually. This indicated that considering the two absorbents as a mixture is unnecessary. Result might imply that water and silicone oil absorb VOCs separately in the RPB. Under this premise, estimations of KGa are not satisfactory, still over 30% error. Therefore, the enhancement factors ('α' _'oil' and 'α' _'water' ) representing the change of surface area for water and silicone oil in dual absorbent system were defined and they were affected by water flow rate, oil flow rate and oil volume fraction. Then we get the empirical correlation for 'α' _'oil' and 'α' _'water' . In addition, enhancement factors were calculated by monte carlo method. The result of α was evolved and satisfactory correlations KGa were obtained successfully. The mass transfer empirical correlation for IPA-oil/water and toluene-oil/water were found to be: (K_G a)/(D_G a_t^2 )=0.0186〖Re〗_G^0.389 〖Re〗_L^0.534 〖Gr〗_G^0.245 H_y^(-0.185) α_water (K_G a)/(D_G a_t^2 )=0.0231〖Re〗_G^0.315 〖Re〗_L^0.389 〖Gr〗_G^0.248 H_y^(-0.31) α_oil α_water=0.14L_o^(-1.08) L_w^0.23 φ^0.83 α_oil=2.21-1.21φ | en |
dc.description.provenance | Made available in DSpace on 2021-06-15T11:19:47Z (GMT). No. of bitstreams: 1 U0001-0602202116170900.pdf: 8322304 bytes, checksum: 0a3f845c884454f7d49c76d9271b5158 (MD5) Previous issue date: 2021 | en |
dc.description.tableofcontents | 目錄 摘要………… I Abstract…… II 目錄…… IV 圖目錄…….. VII 表目錄….. XVII 第一章 緒論 1 第二章 文獻回顧 3 2-1 旋轉填充床 3 2-1.1 旋轉填充床的構造與設計 4 2-1.2 旋轉填充床的壓降 12 2-1.3 旋轉填充床之液體流態、液滴大小、滯留量與滯留時間 17 2-1.4 旋轉填充床內之液膜質傳係數與氣膜質傳係數 26 2-1.5 旋轉填充床之應用與發展 34 2-2 氣液液(G-L-L)三相系統的吸收 47 2-3 液滴的碰撞 52 2-3.1 相同液滴的碰撞行為 53 2-3.2 不互溶液滴的碰撞行為 58 第三章 分析方法 62 3-1 吸收分率( absorption fraction) 62 3-2 總括氣膜體積質傳係數分析 62 3-2.1 雙膜理論 (two-film theory) 63 3-2.2 錯流式旋轉填充床之總括氣膜質傳係數分析 67 3-3 Enhancement factor E 73 第四章 數據整理 75 4-1 物理性質及參數 75 4-2 以水為吸收劑吸收異丙醇氣體 78 4-2.1 氣體進口濃度對異丙醇吸收效果的影響 78 4-2.2 氣體流量對異丙醇吸收效果的影響 80 4-2.3 轉速對異丙醇吸收效果的影響 83 4-2.4 液體流量對異丙醇吸收效果的影響 84 4-3 以水為吸收劑吸收甲苯氣體 87 4-4 以矽油為吸收劑吸收甲苯 88 4-4.1 氣體進口濃度對甲苯吸收效果的影響 88 4-4.2 氣體流量對甲苯吸收效果的影響 90 4-4.3 轉速對甲苯吸收效果的影響 92 4-4.4 液體流量對甲苯吸收效果的影響 96 4-5 以矽油為吸收劑吸收異丙醇 100 4-6 以矽油和水為吸收劑吸收異丙醇 101 4-6.1 轉速對異丙醇吸收分率的影響 101 4-6.2 矽油流量對異丙醇吸收分率的影響 102 4-7 以矽油和水為吸收劑吸收甲苯 103 4-7.1 轉速對甲苯吸收分率的影響 104 4-7.2 添加水流量對甲苯吸收分率的影響 105 第五章 數據分析與質傳現象探討 108 5-1 以E factor評估矽油加水為吸收劑之吸收效果 108 5-1.1 以矽油和水之溶液為吸收劑吸收甲苯 108 5-1.2 以矽油和水溶液為吸收劑吸收異丙醇 112 5-2 以KGa來分析矽油加水溶液對吸收效果的影響 115 5-2.1 油水溶液吸收系統的KGa計算 115 5-2.2 KGa的經驗迴歸式 120 5-3 對矽油/水吸收甲苯的質傳係數經驗式的校正 135 5-4 對矽油/水吸收異丙醇的質傳經驗迴歸式的校正 142 5-5 與碳酸鉀溶液加入環己烷吸收二氧化碳系統比較 150 5-6 與錯流式填充床吸收其餘VOC氣體的KGa比較 153 第六章 αoil與αwater的計算 157 6-1 矽油和水在旋轉填充床內的流態 157 6-2 基於液滴碰撞計算αoil與αwater 163 第七章 結論 182 參考文獻 184 符號說明 197 附錄A αoil的另一種估算方式 207 附錄B 油水吸收甲苯之實驗數據 213 附錄C 油水吸收異丙醇之實驗數據 228 附錄D 油水系統中,水在RPB中的流態 233 附錄E 油水系統中,矽油在RPB中的流態 238 附錄F 液膜體積佔比對αoil和αwater的影響 243 附錄G 計算KGa之matlab程式 254 附錄H KGa經驗迴歸式之matlab程式 257 附錄I 估算αoil和αwater的matlab程式 270 附錄J 附錄A中計算αoil的程式 282 | |
dc.language.iso | zh-TW | |
dc.title | 錯流式旋轉填充床中油水混合液吸收有機揮發物之分析 | zh_TW |
dc.title | Analysis of VOCs Absorption by Oil and Water Mixture in a Cross-Flow Rotating Packed Bed | en |
dc.type | Thesis | |
dc.date.schoolyear | 109-1 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 陳昱劭(Yu-Shao Chen),江佳穎(Chia-Ying Chiang),林佳璋(Chia-Chang Lin) | |
dc.subject.keyword | 旋轉填充床,吸收,質傳,疏水性揮發有機物,親水性揮發有機物, | zh_TW |
dc.subject.keyword | Rotating packed bed,Absorption,Mass transfer,Hydrophilic VOCs,Hydrophobic VOCs, | en |
dc.relation.page | 284 | |
dc.identifier.doi | 10.6342/NTU202100634 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2021-02-10 | |
dc.contributor.author-college | 工學院 | zh_TW |
dc.contributor.author-dept | 化學工程學研究所 | zh_TW |
顯示於系所單位: | 化學工程學系 |
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