具液晶及自組裝態有機光電半導體之特性探討與元件應用

Su-Hao Liu; 劉書豪

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完整後設資料紀錄

DC 欄位	值	語言
dc.contributor.advisor	吳忠幟
dc.contributor.author	Su-Hao Liu	en
dc.contributor.author	劉書豪	zh_TW
dc.date.accessioned	2021-06-15T07:10:25Z	-
dc.date.available	2015-10-21
dc.date.copyright	2010-10-21
dc.date.issued	2010
dc.date.submitted	2010-10-16
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dc.identifier.uri	http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/48723	-
dc.description.abstract	有機發光二極體可利用分子的單一排列方向而產生偏極化光，同時有機薄膜電晶體和有機太陽能電池也有著材料可塑性的特殊需求，如特定的分子排列方向以達到更高的效率。而上所述例子，皆可透過液晶特性加以達成。所以近年來有越來越多的研究致力於發展具有液晶或自組裝態的有機材料，以期能控制有機分子的排列方向。本論文中，我們研究了四種具有液晶態的有機分子。在第二章結果中，經由液晶態的輔助，我們展示了兩種具有自組裝能力的有機材料，該材料是當時在相同類型下第一個具有液晶特性的有機材料，同時我們研究他們的光物理及電荷傳輸特性。在第三章中，我們透過液晶態材料主客系統的配向方式，成功地製作出第一個偏極化的磷光有機發光二極體。而在第四章中，我們利用具液晶態並在固態下擁有高光量子效率的白金錯合物以溶液製程製作有機發光二極體，元件的外部量子效率高達17.6％。我們深信開發並研究具有液晶特性的有機分子將會是未來創造新穎且有潛力的有機光電元件的重要關鍵。	zh_TW
dc.description.abstract	OLEDs can produce polarized electroluminescence via aligning the light-emitting molecules, and the performance of organic thin-film transistors and organic photovoltaic cells can also be improved by aligning the active molecules. Liquid crystal (LC) phases can be applied to achieve these purposes. In this thesis, we studied four organic materials possessing LC phases. In chapter two, we studied the photophysical and charge-transport properties of two self-assembly materials with LC phases. They were the first kind of their own family possessing LC properties. In chapter three, we successfully fabricated the first polarized phosphorescent OLED by using a mesogenic host/guest system. In chapter four, we reported efficient solution-processed phosphorescent OLEDs using a Pt(II) complex with LC properties and high photoluminescence (PL) quantum yields in the solid state. We truly believe that exploiting and studying the organic materials with LC properties will be a key factor to create novel organic electro-optical devices in the future.	en
dc.description.provenance	Made available in DSpace on 2021-06-15T07:10:25Z (GMT). No. of bitstreams: 1 ntu-99-D94943026-1.pdf: 7776694 bytes, checksum: 7db7b0f664fa03c58c6be72efc1f7d19 (MD5) Previous issue date: 2010	en
dc.description.tableofcontents	Contents 致謝..............................................................................................................................................................I 摘要.............................................................................................................................................................II ABSTRACT……………………………………………………………………………………………...III CONTENTS……………………………………………………………………………………………...IV LISTS OF FIGURES VII LISTS OF TABLES XI CHAPTER 1 INTRODUCTION 1 1.1 GENERAL OVERVIEW OF ORGANIC MATERIALS AND ORGANIC DEVICES 1 1.2 LIQUID CRYSTALLINE MATERIALS FOR ORGANIC DEVICES 5 1.3 THESIS ORGANIZATION 8 REFERENCES 9 FIGURES 15 CHAPTER 2 PHOTOPHYSICAL AND CHARGE TRANSPORT STUDIES OF SELF-ASSEMBLED, LIQUID CRYSTAL DIBENZO[G,P]CHRYSENE AND ALUMINUM COMPLEX 17 2.1 INTRODUCTION 17 2.2 INVESTIGATION OF DIBENZO[G,P]CHRYSENE 4 19 2.2.1 Materials 19 2.2.2 Experimental 20 2.2.3 Results and Discussions 24 2.2.4 Summary 26 2.3 INVESTIGATION OF 1-DIC16 26 2.3.1 Materials 26 2.3.2 Experimental 27 2.3.3 Results and Discussions 29 2.3.4 Summary 32 REFERENCE 33 FIGURES 36 CHAPTER 3 POLARIZED PHOSPHORESCENT ORGANIC LIGHT-EMITTING DEVICES ADOPTING MESOGENIC HOST-GUEST SYSTEM 48 3.1 INTRODUCTION 48 3.2 EXPERIMENTAL 51 3.2.1 Materials 51 3.2.2 Physical Measurements 53 3.2.3 Molecular Alignment 54 3.2.4 Photophysical Measurements 55 3.2.5 Devices Fabrication and Measurements 56 3.3 RESULTS AND DISCUSSION 58 3.3.1 Photophysical properties of N-series Pt(II) complexes 58 3.3.2 Molecular alignment and polarized transitions of neat films of N-series Pt(II) complexes 60 3.3.3 Photophysical properties of mixture films of F(MB)5:N-series Pt(II) complexes 62 3.3.4 Molecular alignment and polarized transition in mixture films of F(MB)5: N-series Pt(II) complexes 64 3.3.5 EL characteristics of PPOLED 65 3.4 CONCLUSIONS 68 REFERENCE 69 FIGURES 74 CHAPTER 4 SOLUTION-PROCESSABLE LIQUID CRYSTAL PLATINUM(II) COMPLEX FOR EFFICIENT PHOSPHORESCENT ORGANIC LIGHT-EMITTING DIODES 85 4.1 INTRODUCTION 85 4.2 EXPERIMENTAL 88 4.2.1 Materials 88 4.2.2 Physical Measurements 88 4.2.3 Photophysical characterization 89 4.2.4 Devices Fabrication and Measurements 90 4.3 RESULTS AND DISCUSSION 91 4.3.1 LC Characteristics of 1087 91 4.3.2 Photophysical properties of 1087 in solution and in neat film 92 4.3.3 Orange-red OLED using neat films of 1087 93 4.3.4 Photophysical characteristics of mCP:1087 Guest-Host films 95 4.3.5 Green-yellow OLED using mCP:1087 Guest-Host films 96 4.4 CONCLUSIONS 99 REFERENCE 100 FIGURES 106 CHAPTER 5 SUMMARY AND FUTURE DIRECTIONS 117 5.1 SUMMARY 117 5.2 FUTURE DIRECTIONS 120 Lists of Figures FIGURE 1.1 CHARGE TRANSPORT IN A BILAYER OLED. 15 FIGURE 1.2 THE SCHEMATIC STRUCTURE OF A TYPICAL BOTTOM-CONTACT OFET. 16 FIGURE 1.3 MOLECULAR ARRANGEMENTS IN A (A) DISCOTIC, (B) NEMATIC, OR (C) SMECTIC LIQUID CRYSTAL. 16 FIGURE 2.1 THE STRUCTURE OF COMPOUND 4. 36 FIGURE 2.2 THE SCHEMATIC SAMPLE CONFIGURATION FOR POLARIZED OPTICAL MICROSCOPY OBSERVATION. 36 FIGURE 2.3 THE EXPERIMENT SETUP OF (A) ORTHYSCOPY: EACH PIXEL CORRESPONDS TO A DOT OF SPECIMEN AND EXAMINATION OF THE TEXTURE OF SPECIMEN, AND (B) CONOSCOPY: EACH PIXEL CORRESPONDS TO A DIRECTION OF SPECIMEN AND EXAMINATION OF THE INTERFERENCE FIGURES PRODUCED BY SPECIMEN. [AFTER PERKINS & HENKE, 1999] 37 FIGURE 2.4 SCHEMATIC TOF TRANSIENT CURRENT VS. TIME: (A) NON-DISPERSIVE CASE, (B) SLIGHTLY DISPERSIVE CASE, (C) DISPERSIVE CASE. 38 FIGURE 2.5 (A) ORTHOSCOPIC AND(B) CONOSCOPIC FIGURE OF COMPOUND 4. INSET: THE FACE-ON CONFIGURATION OF COMPOUND 4. 39 FIGURE 2.6 REPRESENTATIVE TOF TRANSIENT IN DOUBLE LOGARITHMIC PLOTS OF COMPOUND 4 FOR (A) HOLE; (B) ELECTRON, AT E=4.0×105 V/CM. 40 FIGURE 2.7 MOBILITY VS E1/2 FOR COMPOUND 4 AT ROOM TEMPERATURE. 40 FIGURE 2.8 THE STRUCTURE OF 1-DIC16. 41 FIGURE 2.9 THE SCHEMATIC SAMPLE CONFIGURATIONS FOR MOLECULAR ALIGNING TEST: (A) USING RUBBED PVK AS THE ALIGNMENT LAYER, AND (B) USING RUBBED PEDOT AS THE ALIGNMENT LAYER. 41 FIGURE 2.10 OPTICAL MICROGRAPHS OF 1-DIC16 SANDWICHED BETWEEN TWO GLASS SLIDES UNDER THE POLARIZED OPTICAL MICROSCOPE: (A) AT 150
dc.language.iso	zh-TW
dc.title	具液晶及自組裝態有機光電半導體之特性探討與元件應用	zh_TW
dc.title	Investigations of Characteristics and Device Applications of Organic Optoelectronic Semiconductors Having Liquid Crystal and Self-Assembly Properties	en
dc.type	Thesis
dc.date.schoolyear	99-1
dc.description.degree	博士
dc.contributor.oralexamcommittee	季昀,汪根欉,徐秀福,陳俐吟
dc.subject.keyword	有機發光二極體,磷光,偏極化發光,液晶,	zh_TW
dc.subject.keyword	OLEDs,phosphorescence,polarized emission,liquid crystal,	en
dc.relation.page	120
dc.rights.note	有償授權
dc.date.accepted	2010-10-18
dc.contributor.author-college	電機資訊學院	zh_TW
dc.contributor.author-dept	電子工程學研究所	zh_TW
顯示於系所單位：	電子工程學研究所

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