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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 何國川(Kuo-Chuan Ho) | |
dc.contributor.author | Hsiao-Han Lai | en |
dc.contributor.author | 賴筱涵 | zh_TW |
dc.date.accessioned | 2021-06-15T05:05:03Z | - |
dc.date.available | 2020-06-18 | |
dc.date.copyright | 2010-07-30 | |
dc.date.issued | 2010 | |
dc.date.submitted | 2010-07-26 | |
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dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/46354 | - |
dc.description.abstract | Polymer light-emitting diodes (PLEDs), as a branch of organic electroluminescence (OEL), are mainly fabricated by solution based wet process. To improve device performance, multilayer structured device is absolute necessary. However, the choices of solvents are limited; this means that the “like dissolves like effect” had to be carefully avoided or the predeposited layer will be destroyed by the incoming layer.
In this thesis, we have demonstrated an all solution process to fabricate multilayer layer structured PLEDs. By carefully selecting the materials and solvents used in each layer, the interfacial mixing issue can be avoided. The first part aimed at the optimization of multilayer structured PLEDs. Poly(9,9-dioctylfluorene-co-N-(4-butylphenyl)-diphenylamine) (TFB, dissolved in p-xylene) acts as hole injection layer, Green B (dissolved in toluene) is the emissive polymer where TiOx (diluted with 2-ethoxyethanol) can be taken as electron injection layer. The maximum current efficiencies of single-, double- and triple-layer PLEDs are 6.42, 8.29 and 10.36 cd/A, respectively. The total increment is 61.4% from single-layer to triple-layer devices. Therefore, with better charge balance, the device lifetime is increased significantly from 4.48×103 h of single-layer device to 5.75×105 h for triple-layer device. In the second part, the effect of surface roughening via adding prism sheet is considered. The efficiencies, color shifts and spectra of PLEDs are affected by varying the thickness of the emissive layers. In our optical configuration, the output of electroluminescence intensity is given by the product of optical response of device structure and photoluminescence of Green B. We had combined the experimental results with the theoretical simulation to optimize the device structure by considering the optical design and the opto-electronic characteristics. The optical cavity was tuned by changing the thickness of TiOx to achieve the best current efficiency with the conventional prism sheet. Consequently, we demonstrated a PLED device with 72.6% enhancement in current efficiency by applying both the TiOx layer and prism sheet. | en |
dc.description.provenance | Made available in DSpace on 2021-06-15T05:05:03Z (GMT). No. of bitstreams: 1 ntu-99-R97549024-1.pdf: 3720941 bytes, checksum: 2ec412484ae4432f8b6ec3e7facc009b (MD5) Previous issue date: 2010 | en |
dc.description.tableofcontents | Chapter 1 Introduction 1
1-1 Evolution and Application of Conducting Polymers 1 1-1-1 The Development of Conducting Polymers 1 1-1-2 Band Theory 5 1-2 Organic Electroluminescence 11 1-2-1 History of Organic Electroluminescence 11 1-2-2 Properties of OLED and PLED 14 1-3 Mechanisms of PLED Operation 16 1-4 Optics 22 1-4-1 Colorimetry 22 1-4-2 Optical Property of PLED 24 Chapter 2 Literatures Review 28 2-1 General Methods to Fabricate Solid Thin Films 28 2-1-1 Spin Coating 28 2-1-2 Dip Coating 29 2-1-3 Meniscus Coating 30 2-1-4 Spray Coating 31 2-1-5 Inkjet Printing 32 2-1-6 Transfer Printing 33 2-1-7 Electrophoretic Deposition 34 2-1-8 Organic Vapor Phase Deposition 35 2-2 Multilayer Structured PLEDs 38 2-3 Reviews of OELs Simulation 43 2-3-1 Classical Ray Optics 43 2-3-2 Classical Electromagnetics 44 2-3-3 Quantum Mechanics 45 2-3-4 Combined Classical and Quantum Mechanical Micro Cavity 46 2-4 Constrains and Motivations 47 2-5 Framework 51 Chapter 3 Experiments 52 3-1 Chemicals 52 3-2 Instruments 53 3-3 Device Fabrication 54 3-3-1 Substrate Preparation 54 3-3-2 Spin Coating of Each Layer 55 3-3-3 Cathodic Thermal Deposition 57 3-4 Characteristics Measurements 58 3-4-1 Opto-electronic Characteristics 58 3-4-2 Luminescent Characteristics 60 3-4-3 Physical Properties 61 Chapter 4 Results and Discussions 62 4-1 Performance of Different Structure Devices 62 4-1-1 Characteristics of Double-layer Devices 62 4-1-2 Characteristics of Triple-layer Devices 69 4-1-3 Comparison among Different Structure Devices 76 4-1-4 Lifetime 81 4-2 Physical Analysis of Materials 84 4-2-1 Energy Level Analysis 84 4-2-2 Micro Morphologies 88 4-2-3 Film Thickness 92 4-3 Optical Simulation 97 Chapter 5 Conclusions and Suggestions 105 5-1 Conclusions 105 5-2 Suggestions 106 Chapter 6 References 107 | |
dc.language.iso | en | |
dc.title | 以全溶液製程製作多層結構高分子發光二極體 | zh_TW |
dc.title | All Solution Process for Multilayer Structured Polymer Light-emitting Diodes | en |
dc.type | Thesis | |
dc.date.schoolyear | 98-2 | |
dc.description.degree | 碩士 | |
dc.contributor.coadvisor | 朱治偉(Chih-Wei Chu) | |
dc.contributor.oralexamcommittee | 周澤川(Tse-Chuan Chou),林正嵐(Cheng-Lan Lin) | |
dc.subject.keyword | 全溶液製程,光萃取效率,微共振腔,多層結構,旋轉塗佈,高分子發光二極體, | zh_TW |
dc.subject.keyword | all solution process,extraction efficiency,micro cavity,multilayer structured,polymer light-emitting diodes,spin coating, | en |
dc.relation.page | 123 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2010-07-27 | |
dc.contributor.author-college | 工學院 | zh_TW |
dc.contributor.author-dept | 高分子科學與工程學研究所 | zh_TW |
顯示於系所單位: | 高分子科學與工程學研究所 |
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