請用此 Handle URI 來引用此文件：
http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/43147完整後設資料紀錄
| DC 欄位 | 值 | 語言 |
|---|---|---|
| dc.contributor.advisor | 馬鴻文 | |
| dc.contributor.author | Hung-Jen Su | en |
| dc.contributor.author | 蘇宏仁 | zh_TW |
| dc.date.accessioned | 2021-06-15T01:39:23Z | - |
| dc.date.available | 2009-07-16 | |
| dc.date.copyright | 2009-07-16 | |
| dc.date.issued | 2009 | |
| dc.date.submitted | 2009-07-15 | |
| dc.identifier.citation | 1. Agency for Toxic Substances and Disease Registry, ToxFAQs™: Chemical Agent Briefing Sheets (CABS), Arsenic. (2006)
2. Brunner P. H. and Rechberger H., “Practical Handbook of Material Flow Analysis”, Lewis Publishers. (2003) 3. Concawe. Air pollutant emission estimation methods for EPER and PRTR reporting by refineries (revised), Prepared by the CONCAWE Air Quality Management Group’s Special Task Force on Emission Reporting Methodologies (STF-64), P. Goodsell (Technical Coordinator), Report no. 9/05R, Brussels April (2006) 4. Carapella, S.. 'Arsenic and arsenic alloys.' Kirk-Othmer encyclopedia of chemical technology. pp.262–274. (2002) 5. Cooper, P., R. MacVicar, et al. Relating CCA fixation to leaching of CCA components from treated products. The International Research Group on Wood Preservation, IRG/WP/50045. (1995) 6. Chilvers, D.C. Peterson, P.J. Global cycling of arsenic. Scientific Committee for problems of the environment (SCOPE) Workshop on metal cycling in the environment. Toronto, Canada. (1984) 7. Duker, A. A., E. J. M. Carranza, and M. Hale. Arsenic geochemistry and health. Environ. Int. 31. pp. 631–641. (2004) 8. Dutre, V. and C. Vandecasteele. 'Solidification/stabilisation of arsenic-containing waste: leach tests and behaviour of arsenic in the leachate.' Waste Management vol. 15. Issue1. pp.55-62. (1995) 9. Ecoinvent database for life cycle analysis of emissions and materials, data vers. 2.0 ; SwissCenter for LifeCycle Inventories:Zurich, Switzerland,( 2007) 10. European Environment Agency (EEA). Feasibility assessment of using the substance f low analysis methodology for chemicals information at macro level.(2007) 11. Lassen, C., & Hansen, E. Paradigm for substance flow analyses—Guide for SFAs carried out for the Danish EPA. Danish Environmental Protection Agency, Environmental Project No. 577. Retrieved from http://www.mst.dk. (2000) 12. Fuessle, R. and M. Taylor. 'Stabilization of arsenic-and barium-rich glass manufacturing waste.' Journal of Environmental Engineering vol.126 Issue3 pp.272-278. (2000) 13. Graedel, T.E. and Allenby, B.R., Industrial Ecology, Prentice Hall, Englewood Cliffs, NJ. (1995) 14. Haberl, H. 'The global socioeconomic energetic metabolism as a sustainability problem.' Energy. Vol. 31. Issue.1. pp. 87-99. (2006) 15. J. Thomas Hindmarsh . Charles O. Abernathy . Environmental Aspects of Arsenic Toxicity.(2002) 16. Jain, A. and R. Sareen. 'E-waste assessment methodology and validation in India.' Journal of Material Cycles and Waste Management vol. 8. Issue1. pp.40-45. (2006) 17. Jockel W.; Hartje J. Datenerhebung uber die Emissionen Umwelt-gefahrdenden Schwermetalle. Forschungsbericht 91-1-4 02 588; TuV Rheinland e.V. Koln. (1991) 18. Kakitani, T., T. Hata, et al. 'Designing a purification process for chromium-, copper-and arsenic-contaminated wood.' Waste Management Vol. 26 Issue 5. pp. 453-458. (2006) 19. Krausmann, F. and H. Haberl. 'The process of industrialization from the perspective of energetic metabolism Socioeconomic energy flows in Austria 1830–1995.' Ecological Economics vol. 41. Issue 2. pp.177-201. (2002) 20. Lindau, L. 'Emissions of arsenic in Sweden and their reduction.' Environmental Health Perspectives vol.19. Issue 25. (1977) 21. Magalhaes, A. C. F. Arsenic. An environmental problem limited by solubility. Pure Appl. Chem. 74:1843–1850. (2002) 22. Mattigod, S., D. Rai, et al. 'Geochemical factors controlling the mobilization of inorganic constituents from fossil fuel combustion residues: II. Review of the minor elements.' Journal of Environmental Quality Vol. 19 Issue 2. pp.188. (1990) 23. Meij, and te Winkel. 'Trace elements in world steam coal and their behaviour in Dutch coal-fired power stations: A review.' International Journal of Coal Geology Vol.77. Issue 3-4 pp.289-293. (2009) 24. P Ruetschi. Aging mechanisms and service life of lead–acid batteries. Journal of Power Sources. vol. 127. Issue1-2, pp.33-44.(2004) 25. Piver, WT. Mobilization of arsenic by natural and industrial processes. Biological and Environmental Effects of Arsenic (BA Fowler, Ed.), Elsevier, Amsterdam. pp.1–50. (1983) 26. Salomone, R., F. Mondello, et al. 'An Eco-balance of a Recycling Plant for Spent Lead–Acid Batteries.' Environmental Management vol. 35. Issue 2, pp. 206-219. (2005) 27. Sadler, R., H. Olszowy, et al. 'Soil and water contamination by arsenic from a tannery waste.' Water, Air, & Soil Pollution Vol. 78. Issue. 1. pp. 189-198. (1994) 28. Stigter, J., H. de Haan, et al. 'Determination of cadmium, zinc, copper, chromium and arsenic in crude oil cargoes.' Environmental Pollution Vol. 107, Isuue. 3. pp.451-464. (2000) 29. Sullivan, R. and U. States. Preliminary Air Pollution Survey of Arsenic and Its Compounds: A Literature Review, US Dept. of Health, Education, and Welfare, Public Health Service, Consumer Protection and Environmental Health Service, National Air Pollution Control Administration. (1969) 30. Tchounwou, P., J. Centeno, et al. 'Arsenic toxicity, mutagenesis, and carcinogenesis–a health risk assessment and management approach.' Molecular and cellular biochemistry. Vol. 255. Issue. 1. pp.47-55. (2004) 31. Terazono, A. and Y. Moriguchi, International Secondary Material Flows within Asia. Journal of Industrial Ecology; Vol. 8 Issue 4, pp.10-12, (2004) 32. U.S.EPA. Locating And Estimating Air Emissions From Sources Of Arsenic And Arsenic Compounds.(1998) 33. U.S. EPA. Arsenic. In: Intermedia Priority Pollutant Guidance Documents. Washington, D.C. U.S. Environmental Protection Agency, Office of Pesticides and Toxic Substances.(1982) 34. U.S. Department of Health and Human Resources. Toxicological Profile for Arsenic, Draft Update. Public Health Service. Agency for Toxic Substances and Disease Registry. (1992) 35. U.S. EPA. Arsenic Occurrence in Public Drinking Water Supplies. (2000) 36. Viereck-Gotte, L. and Herget, J. Zur Geochemie der Boden industriell gepragter urbaner Gebiete. In: Matschullat, J., Tobschall, H.J. and Voigt, H.J. Editors, Geochemie und umwelt. Relevante prozesse in atmo-, pedo- und hydrosphare Springer, Berlin. pp. 127–150. (1997) 37. World Health Organization (WHO), Regional Publications, European Series, Regional Office for Europe. Part II. Evaluation of Human Health Risks , 6.1 Arsenic.(2000) 38. World Health Organization (WHO), Arsenic And Arsenic Compounds.(2001) 39. WRI,”the Weight of Nations : Material Outflows from Industrial Economies,World Resources Institute, Washington D.C “p.p.13~17.(2000) 40. Zhang, J., J. Liu, et al. 'Comparison of the fixation of heavy metals in raw material, clinker and mortar using a BCR sequential extraction procedure and NEN7341 test.' Cement and Concrete Research vol. 38. Issue. 5. pp.675-680. (2008). 41. Oivind Tryland, Jon Oznevad. Materialstromanalyse av arsen. Vurdering av alternativ. Berdal Stromme a.s. ISBN -82-7655-056-8. (1992) 42. 劉鎮宗， “砷與生態環境的關係”，科學月刊，第26 卷，第一期，第134-140頁，(1995)。 43. 陳建仁，從台灣的砷經驗，展望世界未來，科學人，(2004)。 44. 張尊國，2006，「台北市農地土壤重金屬砷含量調查及查證計畫」，臺北市政府環境保護局。 45. 李宜欣，自農業資變遷初探淡水河流域之物質流課題，碩士論文，國立台灣大學環境工程研究所，(2001)。 46. 洪克銘，台灣中油公司物質流分析之評估應用，中技社97年度秋季環境與能源國際研討會，(2008)。 47. 陳信榮，中鋼公司物質流評估應用，中技社97年度秋季環境與能源國際研討會，(2008)。 48. 陳麗如，「物質流-鎘在台灣生活圈中之流向與流量初探」，碩士論文，國立台灣大學環境工程研究所，(2003)。 49. 洪慧倫，台灣戴奧辛物質流分析，碩士論文，國立台灣大學環境工程研究所(2007)。 50. 陳必晟，“台灣地區鉻之物質流分析與風險評估”，碩士論文，國立台灣大學環境工程學研究所 (2003)。 51. 邱弘毅，台灣地區砷、汞、鎘及其化合物之用途及用量研究調查，中華衛誌，第13卷，第2期(1994)。 52. 王俊傑，“台灣產業環境衝擊關聯分析與永續消費型態探討”，碩士論文，國立台灣大學環境工程學研究所 (2008) 53. 李錦地，砷在本省的污染問題，科學月刊，第11卷，第7期，第70頁(1980) 54. 王彥令，李榮昌. 河南某雄黃—雌黃礦石的選礦富集。化工礦山技術第22卷，第6期，第21-22頁，(1993)。 55. 中興工程顧問公司，「固定污染源毒性空氣污染物(戴奧辛及重金屬)排放清冊調查及管制計畫」，研究計畫EPA-96-FA12-03-A115，行政院環境保護署(2007)。 56. 卓志銘，焚化爐飛灰之資源化研究，碩士論文，大同大學化學工程研究所(2004)。 57. 方鴻源，陳韋廷，「電子業廢棄鎵金屬之純化再利用」，研究計畫：NSC-95-2221-E-224-039-，行政院國家科學委員會，(2006)。 58. 張簡宜芳，台灣地區造紙業二氧化碳排放變動效果因素分析，碩士論文，嘉南藥理科技大學環境工程與科學系所，(2008)。 網頁連結: ATSDR(Agency for Toxic Substances and Disease Registry) http://www.atsdr.cdc.gov/ USEPA Integrated Risk Information System(IRIS)資料庫 http://cfpub.epa.gov/ncea/iris/index.cfm USEPA WebFIRE (Technology Transfer Network Clearinghouse for Inventories & Emissions Factors) http://cfpub.epa.gov/oarweb/index.cfm?action=fire.main 環保署毒理資料庫 http://flora2.epa.gov.tw/prog/database.asp 行政院主計處 http://www.dgbas.gov.tw/mp.asp?mp=1 國際貿易局進出口產商基本資要查詢 http://fbfh.trade.gov.tw/rich/test/comindex.asp 中華民國進出口貿易統計 http://cus93.trade.gov.tw/bftweb/fsci/ 經濟部能源局 http://www.moeaboe.gov.tw/ 經濟部礦務局 http://www.mine.gov.tw/ 環保署資源回收基管會 資源回收網 http://recycle.epa.gov.tw/epa/index.asp | |
| dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/43147 | - |
| dc.description.abstract | 砷被廣泛、多元地應用於玻璃製造、木材防腐業及半導體、光電業等多項產業製程、產品中，在經濟活動的使用上有其必要性。但是，砷及其化合物具有致癌及非致癌之毒害特性；因此，在無法有效禁止砷及其化合物的使用下，有必要針對砷進行流布及流向分析、探討。
研究以物質流分析方法分別對砷於人類經濟活動之應用以及因人類活動所造成砷之環境釋放進行探討，以建構出台灣砷物質流網路模型；再者，利用物質流分析特性探討砷之使用時間趨勢、地區分布以及相關產業結構。最後將物質流分析結果整合投入產出分析方法，以投入產出分析方法連結環境及產業間關係，說明台灣砷產業使用現況，進一步探討砷於產業間投入產出之關聯性。 研究顯示，經濟圈主要使用量為玻璃製造業、水泥業、鉛蓄電池、木材防腐業以及半導體、光電業等五項產業，在環境砷釋放上，則是以水泥業、煤礦使用、原油煉解以及金屬礦物冶煉為主要污染釋放熱點。將物質流分析結果進行多年趨勢探討，說明砷物質之產業結構變化。 比較投入產出分析結果，發現非金屬礦物製品、其他金屬、電力等部門為每單位產值所需砷的使用量及環境釋放量較高者。含砷產業之環境負荷放大效應部分，服務業相較於製造業及初級產業有著較高的環境境負荷的累積、放大現象。在產業關聯性分析，發現同樣是以非金屬礦物製品、其他金屬、電力及石油煉製品等產業之前後關聯性較高(包含向前關聯、向後關聯)，以及將產業消費內容回歸到家計消費，發現在住、行及服務等產業類別有著高環境砷釋放量及使用量。最後比較砷之PTB、區域投入產出及消費型態之地區分布，發現高生活消費地區(如台北市、台中市、高雄市)之低環境砷釋放量，而部分低消費地區(花蓮縣、雲林縣)卻負擔高砷相關產業，即承受高環境砷負荷量，呈現出區域間存在著環境不公的現象。 | zh_TW |
| dc.description.abstract | Arsenic and its compounds are widely applied in multiple industrial processes and products such as glasses, semiconductors and optoelectronics production, and wood preservatives. However, arsenic and its compounds have been characterized with both carcinogenic and non-carcinogenic toxicities. Therefore, flows of arsenic should be
analyzed because of their indispensability in a wide range of industrial processes. This study applied material flow analysis to investigate both the application of arsenic in human economic activities and the environmental release of arsenic due to human activities to build up the material flow network model of arsenic. The study also investigated the temporal pattern of arsenic usage, spatial distribution, and related industrial structure by using material flow analysis. Furthermore, the results of material flow analysis were integrated with Input-Output Analysis method to link environmental burden with industrial structure. Through the integrated analysis, current status of arsenic usage in Taiwan can be interpreted, and the input-output correlation of arsenic among industries can be further identified. Based on the results of material flow analysis, arsenic and its compounds are mainly applied in glasses, cement, lead acid batteries, semiconductors and optoelectronics production and wood preservatives industries in the anthroposphere. As for the environmental release, major releasing hotspots are cements production, coal burning, oil and metal mineral refining processes. Multiple-year trend of arsenic flow were further dipcted to examine the industrial structural change in arsenic use. According to the results of input-output analysis, the sectors of non-metal mineral products, other metals, and electricity have greater arsenic use and environmental release per output value. As for amplification effect of environmental burdens from arsenic-containing industries, service industry revealed greater accumulation and amplification effects of environmental burdens than manufacturing and primary industries. The results also showed that the sectors of non-metal mineral products, other metals, electricity, and petroleum refining products have greater industrial linkages, including forward and backward linkages. When industrial consumption was allocated into household consumption, housing, transportation, and service industries generated greatest arsenic use and environmental releases. Finally, comparing data of physical trade balance (PTB) of arsenic, regional input-output analysis and distribution of consumption patterns in different regions in Taiwan, high consumption regions (e. g. Taipei City, Taichung City, and Kaohsiung City) were found to bear lower arsenic environmental releases, whereas some low consumption regions (e. g. Hualien County and Yunlin County) bear high environmental burden of arsenic due to industries with high arsenic intensity within these regions. The results demonstrated the environmental inequity among regions in Taiwan. | en |
| dc.description.provenance | Made available in DSpace on 2021-06-15T01:39:23Z (GMT). No. of bitstreams: 1 ntu-98-R96541208-1.pdf: 2314843 bytes, checksum: 23f9c13063036ae94efaeda1009b16a8 (MD5) Previous issue date: 2009 | en |
| dc.description.tableofcontents | 頁次
摘要 ................................................................................................................................. i Abstract ........................................................................................................................ iii 表目錄 ........................................................................................................................ viii 圖目錄 ............................................................................................................................ x 第一章 緒論 .................................................................................................................. 1 1.1 研究背景 ........................................................................................................ 1 1.2 研究目的 ........................................................................................................ 3 1.3 研究架構 ........................................................................................................ 4 第二章 文獻回顧 .......................................................................................................... 6 2.1 砷之基本特性 ................................................................................................ 6 2.1.1 砷及其化合物的物理化學性質 .......................................................... 6 2.1.2 砷的毒理特性 ...................................................................................... 8 2.1.3 砷的應用與經濟圈釋放 .................................................................... 10 2.1.4 環境中砷的流布 ................................................................................ 11 2.2 物質流分析 .................................................................................................. 14 2.2.1 物質流概念 ........................................................................................ 14 2.2.2 物質流分析之應用 ............................................................................ 14 2.2.3 物質流之類別及步驟 ........................................................................ 15 2.3 投入產出分析方法 ...................................................................................... 24 第三章 研究方法 ........................................................................................................ 27 3.1 研究步驟 ...................................................................................................... 27 3.2 經濟圈內之物質流分析 .............................................................................. 29 3.2.1 砷物質之網路模型 ........................................................................... 31 3.2.2 含砷資料盤查分析 ........................................................................... 34 3.3 環境圈物質流及釋放資訊 .......................................................................... 39 3.3.1 空氣 ................................................................................................... 39 3.3.2 水體 ................................................................................................... 40 3.3.3 廢棄物 ............................................................................................... 40 3.3.2 資源回收 ........................................................................................... 41 3.4 結合經濟圈及環境圈之砷物質流 .............................................................. 42 3.4.1 砷之生命週期模型建立 ................................................................... 42 3.4.2 砷物質流結果分析及質量平衡 ....................................................... 46 3.5 物質流投入產出分析方法 .......................................................................... 47 3.6 物質流及相關指標 ...................................................................................... 52 第四章 結果與討論 .................................................................................................... 55 4.1 砷物質流結果分析 ...................................................................................... 55 4.1.1 砷之經濟體流布及流量 ................................................................... 55 4.1.2 砷之環境釋放分析 ........................................................................... 63 4.1.3 結合經濟圈及環境圈之砷物質流分析結果 ................................... 68 4.2 砷物質流之時間因子分析 .......................................................................... 72 4.3 含砷物質進出口量之地區分布 .................................................................. 78 4.4 砷物質產業活動與需求之環境衝擊 .......................................................... 82 4.4.1 單位最終需求環境排放潛勢 ........................................................... 82 4.4.2 砷應用產業之環境釋放關聯分析 ................................................... 85 4.4.3 產業之乘數效應 ............................................................................... 88 4.4.4 最終需求與環境衝擊分析 ............................................................... 89 4.4.5 家計需求之砷物質之使用及環境釋放分布 ................................... 90 4.5 各縣市砷物質使用及環境釋放比較 .......................................................... 91 4.5.1 砷物質之消費型態分布 ................................................................... 91 4.5.2 砷物質之區域 IO環境釋放分布 ..................................................... 93 4.6 誤差探討 ...................................................................................................... 95 5.1 結論 .............................................................................................................. 96 5.2 建議 .............................................................................................................. 98 參考文獻 ...................................................................................................................... 99 附錄一 含砷物質之國內產銷 .................................................................................. 104 附錄二 含砷物質之進出口資料 .............................................................................. 106 附錄三台灣砷物質貿易趨勢 .................................................................................... 111 附錄四 產業關聯部門定義 ...................................................................................... 113 附錄五 消費支出調查 .............................................................................................. 119 | |
| dc.language.iso | zh-TW | |
| dc.subject | 國內物質消費 | zh_TW |
| dc.subject | 物質流分析 | zh_TW |
| dc.subject | 投入產出分析 | zh_TW |
| dc.subject | 砷 | zh_TW |
| dc.subject | Arsenic | en |
| dc.subject | Domestic Material Consumption | en |
| dc.subject | Substance flow analysis | en |
| dc.subject | Input-Output Analysis | en |
| dc.title | 台灣地區砷之物質流分析 | zh_TW |
| dc.title | Substance Flow Analysis of arsenic in Taiwan | en |
| dc.type | Thesis | |
| dc.date.schoolyear | 97-2 | |
| dc.description.degree | 碩士 | |
| dc.contributor.oralexamcommittee | 李公哲,張慶源 | |
| dc.subject.keyword | 物質流分析,投入產出分析,砷,國內物質消費, | zh_TW |
| dc.subject.keyword | Substance flow analysis,Input-Output Analysis,Arsenic,Domestic Material Consumption, | en |
| dc.relation.page | 124 | |
| dc.rights.note | 有償授權 | |
| dc.date.accepted | 2009-07-15 | |
| dc.contributor.author-college | 工學院 | zh_TW |
| dc.contributor.author-dept | 環境工程學研究所 | zh_TW |
| 顯示於系所單位： | 環境工程學研究所 | |
文件中的檔案：
| 檔案 | 大小 | 格式 | |
|---|---|---|---|
| ntu-98-1.pdf 未授權公開取用 | 2.26 MB | Adobe PDF |
系統中的文件，除了特別指名其著作權條款之外，均受到著作權保護，並且保留所有的權利。