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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 李達源(Dar-Yuan Lee) | |
dc.contributor.author | You-Ren Li | en |
dc.contributor.author | 李祐任 | zh_TW |
dc.date.accessioned | 2021-06-08T01:02:08Z | - |
dc.date.copyright | 2020-09-22 | |
dc.date.issued | 2020 | |
dc.date.submitted | 2020-08-12 | |
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dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/18376 | - |
dc.description.abstract | 由於鎵與銦近年來被廣泛使用於半導體產業,在環境水體及土壤中皆有濃度高於背景值,以及鎵與銦共同污染的情形發生,因此存在透過食物鏈進入人體造成健康危害的風險。鋁是廣泛分布於地殼中的元素,在酸性條件下有效性高,會影響植株生長及養分平衡,由於鎵、銦與鋁有部分的化學性質相似,且對植物造成的毒害症狀類似,加上鋁也會與土壤表面的鎵和銦競爭吸附位置,因此鋁、鎵與銦在土壤溶液中物種分布及植物吸收方面的交互作用值得被探討。本實驗目的為藉由水耕栽培的方式,了解水稻幼苗在鎵/銦與鋁共存下的交互作用對鎵和銦累積之影響。實驗之水耕液pH值調整為4.0,處理包含鋁與鎵共存、鋁與銦共存、鎵與銦共存以及鋁、鎵和銦個別的處理,選用水稻栽培種為台稉九號(Oryza sativa L. cv Taikeng 9),植株於處理條件下生長暴露21天,後續分析植體中鋁、鎵、銦及植物營養元素的含量。結果顯示在鋁與鎵共存下,水稻幼苗生長抑制主要是來自鋁的毒害,鋁的存在會與鎵競爭,導致植體中鎵的總累積量減少,降低根部對鎵的吸收,並促使鎵由根部往地上部轉運;鋁與銦共存時的症狀和鎵與銦共存時相同,植株生長皆受到銦毒害影響為主,鋁或鎵的存在對於銦的吸收、轉移及累積皆不存在明顯的交互作用;銦則會抑制鎵的總累積量,限制植株根部鎵的吸收,並促使鎵由根部往地上部的傳輸。水耕液中鋁、鎵和銦對於檸檬酸的結合能力不同,當鎵/銦與鋁共存時對於溶液中檸檬酸的競爭是導致物種及有效性發生交互作用的主要因素,特別是鎵與檸檬酸的結合能力強,因此在鋁與鎵共存時具有明顯的競爭行為。本研究結果指出當鎵/銦與鋁共存時需特別考慮到其與有機酸之間的錯合能力,進而影響其對於植株的毒性及累積情形。 | zh_TW |
dc.description.abstract | Gallium (Ga) and indium (In) compounds are widely used in semiconductor manufacturing industry. The discharge of Ga/In may result in the concentrations of Ga/In in groundwater and soil be higher than the background value and cause Ga/In co-contamination. Human beings might expose to Ga and In through the food chain and health hazards. Aluminum (Al) is the common metal element in the earth’s crust. In acid soils, dissolution of Al minerals leads to increase the concentration of soluble Al that are rhizotoxic to plant. Ga, In and Al have similar chemical properties and phytotoxic symptoms. Moreover, Al and Ga might compete for the adsorption sites on the soil colloid surfaces. Therefore, it’s important to investigate the interaction between Al, Ga and In. The objective of this study was to determine the effects of Ga/In and Al coexistence on the accumulation of Ga and In in rice seedlings grown in solution cultures. The treatments included Al/Ga coexistence, Al/In coexistence, and Ga/In coexistence. Rice seedlings (Oryza sativa L. cv Taikeng 9) were exposed to treatments for 21 days. After harvesting, the concentration of Al, Ga, In and nutrients element in the plant were analyzed by ICP-OES and ICP-MS. The results indicated that under Al/Ga coexistence, the growth inhibition of rice seedlings was mainly due to the Al toxicity. The presence of Al might inhibit the absorption of Ga, resulting in decreasing the accumulation of Ga in plant, and promoting the root-to-shoot translocation of Ga. The phenotype of rice seedlings in Al/In coexistence were similar to that of Ga/In coexistence, plant was affected by In phytotoxicity. The presence of Al or Ga had no significant effect on the absorption, translocation and accumulation of In. However, In inhibited the accumulation of Ga, decreased the absorption of Ga in the root, and promoted the translocation of Ga from root to shoot. The stability constants of Al, Ga and In binding to citrate were different. Ga preferred to complex with citrate, which cause the availability of Ga decreased in Al/Ga coexistence solution. According to the results of this study, it’s necessary to consider the stability constants of Al and Ga/In complex with organic acids, which might significantly affect the toxicity and accumulation of Ga/In in plants when Ga/In and Al coexistence. | en |
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dc.description.tableofcontents | 摘要 I Abstract II 圖目錄 VI 表目錄 VIII 第一章 緒論 1 1.1 鎵 1 1.1.1 鎵的應用、來源與污染 1 1.1.2 鎵對人體和動物之危害 3 1.1.3 鎵對植物生長之影響 5 1.1.4 環境中鎵的分布與特性 6 1.2 銦 9 1.2.1 銦的應用、來源與污染 9 1.2.2 銦對人體和動物之危害 10 1.2.3 銦對植物生長之影響 11 1.2.4 環境中銦的分布與特性 12 1.3 臺灣對鎵與銦的管制現況 15 1.4 鋁 16 1.4.1 鋁的特性及在環境中的分布 16 1.4.2 鋁對植物生長之影響 19 1.5 研究目的 21 第二章、材料與方法 22 2.1 水稻幼苗暴露鋁、鎵和銦之試驗 22 2.1.1 水稻育苗 22 2.1.2 鎵/銦與鋁共存暴露之處理 25 2.1.3 水耕液中可溶性鋁、鎵與銦測定 (Kopittke and Blamey, 2016) 25 2.1.4 植體採收 25 2.2 水耕液配製 28 2.3植體分析 30 2.3.1 株高生長量、根伸長量與生質量 30 2.3.2 葉綠素測定 30 2.3.3 植體鋁、鎵、銦和其他營養元素之含量分析 30 2.3.3.1 利用DCB溶液移除根部鐵膜吸持之離子 (Liu et al., 2004) 30 2.3.3.2 植體分解 31 2.3.3.3 添加標準品分析 31 2.3.4 生物濃縮係數、轉移係數與累積量計算 32 2.4 水耕液中鋁、鎵與銦之物種分佈模擬 32 2.5 統計分析 32 第三章、結果與討論 36 3.1 鋁與鎵共存及其個別處理對水稻幼苗之影響 36 3.1.1鋁與鎵共存及其個別處理對水稻幼苗生長情形之影響 36 3.1.2 植體中鎵與鋁的濃度、生物濃縮係數及轉移係數 39 3.1.3 植體中鎵與鋁的累積量 42 3.1.4 水耕液中鋁與鎵物種分佈對水稻幼苗吸收之影響 45 3.1.5 水稻植體營養元素分析 47 3.1.5.1 鋁與鎵共存及其個別處理對植體營養元素磷、鉀、鈣、鎂與硫濃度之影響 48 3.1.5.2 鋁與鎵共存及其個別處理對微量營養元素鐵、錳、銅、鋅與硼濃度之影響 50 3.2 鋁與銦共存及其個別處理對水稻幼苗之影響 52 3.2.1鋁與銦共存及其個別處理對水稻幼苗生長情形之影響 52 3.2.2 植體中銦與鋁的濃度、生物濃縮係數及轉移係數 55 3.2.3 植體中銦與鋁的累積量 58 3.2.4 水耕液中鋁與銦物種分佈對水稻幼苗吸收之影響 60 3.2.5 水稻植體營養元素分析 61 3.2.5.1 鋁與銦共存及其個別處理對植體營養元素磷、鉀、鈣、鎂與硫濃度之影響 62 3.2.5.2 鋁與銦共存及其個別處理對微量營養元素鐵、錳、銅、鋅與硼濃度之影響 62 3.3 鎵與銦共存及其個別處理對水稻幼苗之影響 65 3.3.1鎵與銦共存及其個別處理對水稻幼苗生長情形之影響 65 3.3.2 植體中鎵與銦的濃度、生物濃縮係數及轉移係數 68 3.3.3 植體中鎵與銦的累積量 71 3.3.4 水耕液中鎵與銦物種分佈對水稻幼苗吸收之影響 73 3.3.5 水稻植體營養元素分析 74 3.3.5.1 鎵與銦共存及其個別處理對植體營養元素磷、鉀、鈣、鎂與硫濃度之影響 75 3.3.5.2 鎵與銦共存及其個別處理對微量營養元素鐵、錳、銅、鋅與硼濃度之影響 77 第四章、結論 79 第五章 參考文獻 80 附錄 91 | |
dc.language.iso | zh-TW | |
dc.title | 鎵/銦與鋁共存對水耕栽培水稻中鎵和銦累積之影響 | zh_TW |
dc.title | Effects of Ga/In and Al coexistence on the accumulation of Ga and In in rice seedlings grown in solution cultures | en |
dc.type | Thesis | |
dc.date.schoolyear | 108-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 王尚禮(Shan-Li Wang),鄒裕民(Yu-Min Tzou),莊愷瑋,許健輝(Chien-Hui Syu) | |
dc.subject.keyword | 鋁,鎵,銦,共存,交互作用,水耕栽培,檸檬酸, | zh_TW |
dc.subject.keyword | aluminium,gallium,indium,coexistence,interactions,hydroponic culture,citrate, | en |
dc.relation.page | 96 | |
dc.identifier.doi | 10.6342/NTU202003140 | |
dc.rights.note | 未授權 | |
dc.date.accepted | 2020-08-13 | |
dc.contributor.author-college | 生物資源暨農學院 | zh_TW |
dc.contributor.author-dept | 農業化學研究所 | zh_TW |
顯示於系所單位: | 農業化學系 |
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