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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 朱時宜 | |
dc.contributor.author | Yi-Jen Chen | en |
dc.contributor.author | 陳怡蓁 | zh_TW |
dc.date.accessioned | 2021-05-20T21:09:29Z | - |
dc.date.available | 2013-08-22 | |
dc.date.available | 2021-05-20T21:09:29Z | - |
dc.date.copyright | 2011-08-22 | |
dc.date.issued | 2011 | |
dc.date.submitted | 2011-08-20 | |
dc.identifier.citation | [1] M. Ferray and et al. Multiple-harmonic conversion of 1064 nm radiation in rare
gases. Journal of Physics B: Atomic, Molecular and Optical Physics, 21(3):L31, 1988. [2] P. B. Corkum and F. Krausz. Attosecond science. Nature Physics, 3(6):381--387, 2007. [3] A. M. March. Strong field studies of cesium using intense mid-infrared light. PhD thesis, Stony Brook University, 2009. [4] E. P. Power, A. M. March, F. Catoire, E. Sistrunk, K. Krushelnick, P. Agostini, and L. F. DiMauro. Xfrog phase measurement of threshold harmonics in a keldysh-scaled system. Nature Photonics, 4(6):352--356, 2010. [5] J. E. Sansonetti. Wavelengths, transition probabilities, and energy levels for the spectra of cesium (cs i--cs lv). Journal of Physical and Chemical Reference Data, 38(4):761--923, 2009. [6] P. Colosimo, G. Doumy, C. I. Blaga, J. Wheeler, C. Hauri, F. Catoire, J. Tate, R. Chirla, A. M. March, G. G. Paulus, H. G. Muller, P. Agostini, and L. F. DiMauro. Scaling strong-field interactions towards the classical limit. Nature Physics, 4(5): 386--389, 2008. [7] Zenghu Chang, Andy Rundquist, Haiwen Wang, Margaret M. Murnane, and Henry C. Kapteyn. Generation of coherent soft x rays at 2.7 nm using high harmonics. Physical Review Letters, 79(16):2967, 1997. [8] Ch. Spielmann, N. H. Burnett, S. Sartania, R. Koppitsch, M. Schnürer, C. Kan, M. Lenzner, P. Wobrauschek, and F. Krausz. Generation of coherent x-rays in the water window using 5-femtosecond laser pulses. Science, 278(5338):661--664, 1997. [9] E. Goulielmakis, M. Schultze, M. Hofstetter, V. S. Yakovlev, J. Gagnon, M. Uiberacker, A. L. Aquila, E. M. Gullikson, D. T. Attwood, R. Kienberger, F. Krausz, and U. Kleineberg. Single-cycle nonlinear optics. Science, 320(5883):1614--1617, 2008. [10] E. Gustafsson, T. Ruchon, M. Swoboda, T. Remetter, E. Pourtal, R. Lopez-Martens, P. Balcou, and A. L'Huillier. Broadband attosecond pulse shaping. Optics Letters, 32(11):1353--1355, 2007. [11] L. V. Keldysh. Ionization in field of a strong electromagnetic wave. Soviet Physics Jetp-Ussr, 20(5):1307--, 1965. [12] P. B. Corkum. Plasma perspective on strong field multiphoton ionization. Physical Review Letters, 71(13):1994, 1993. [13] Jeffrey L. Krause, Kenneth J. Schafer, and Kenneth C. Kulander. High-order harmonic generation from atoms and ions in the high intensity regime. Physical Review Letters, 68(24):3535, 1992. [14] A. Lhuillier, K. J. Schafer, and K. C. Kulander. Theoretical aspects of intense field harmonic-generation. Journal of Physics B-Atomic Molecular and Optical Physics, 24(15):3315--3341, 1991. [15] H. Soifer, P. Botheron, D. Shafir, A. Diner, O. Raz, B. D. Bruner, Y. Mairesse, B. Pons, and N. Dudovich. Near-threshold high-order harmonic spectroscopy with aligned molecules. Physical Review Letters, 105(14):143904, 2010. [16] D. C. Yost, T. R. Schibli, J. Ye, J. L. Tate, J. Hostetter, M. B. Gaarde, and K. J. Schafer. Vacuum-ultraviolet frequency combs from below-threshold harmonics. Nature Physics, 5(11):815--820, 2009. [17] W. Nicklich, Kumpfm, uuml, H. ller, H. Walther, X. Tang, Huale Xu, and P. Lambropoulos. Above-threshold ionization of cesium under femtosecond laser pulses: New substructure due to strongly coupled bound states. Physical Review Letters, 69(24):3455, 1992. [18] B. Sheehy, J. D. D. Martin, L. F. DiMauro, P. Agostini, K. J. Schafer, M. B. Gaarde, and K. C. Kulander. High harmonic generation at long wavelengths. Physical Review Letters, 83(25):5270, 1999. [19] B. Sheehy, T. O. Clatterbuck, C. Lyng, J. D. D. Martin, D. W. Kim, L. F. DiMauro, M. B. Gaarde, K. J. Schafer, P. Agostini, and K. C. Kulander. Strong field physics in a scaled interaction. Laser Physics, 11(2):226--230, 2001. [20] Mette B. Gaarde and Kenneth J. Schafer. Enhancement of many high-order harmonics via a single multiphoton resonance. Physical Review A, 64(1):013820, 2001. [21] G. Doumy, J. Wheeler, E. Sistrunk, A. DiChiara, T. A. Miller, E. Power, A. M. March, F. Catoire, C. Blaga, I. Lachko, C. Roedig, R. Chirla, K. Krushelnick, P. Agostini, and L. F. DiMauro. High harmonic generation from long wavelength drivers. In Lasers Electro Optics The Pacific Rim Conference on Lasers and Electro-Optics, 2009. CLEO/PACIFIC RIM '09. Conference on, pages 1--2. [22] T. O. Clatterbuck, C. Lynga, P. Colosimo, J. D. D. Martin, B. Sheehy, L. F. Di- Mauro, P. Agostini, and K. C. Kulander. Scaled intense laser-atom physics: the long wavelength regime. Journal of Modern Optics, 50:441--450, 2003. [23] T. O. Clatterbuck, Lyng, aring, C., P. M. Paul, L. F. DiMauro, M. B. Gaarde, K. J. Schafer, P. Agostini, K. C. Kulander, and I. Walmsley. Yield and temporal characterization of high-order harmonics from intense midinfrared excitation of a cesium vapor. Physical Review A, 69(3):033807, 2004. [24] M. Lewenstein, Ph Balcou, M. Yu Ivanov, Anne L'Huillier, and P. B. Corkum. Theory of high-harmonic generation by low-frequency laser fields. Physical Review A, 49(3):2117, 1994. [25] P. Salières, B. Carré, L. Le Déroff, F. Grasbon, G. G. Paulus, H. Walther, R. Kopold, W. Becker, D. B. Milošević, A. Sanpera, and M. Lewenstein. Feynman's pathintegral approach for intense-laser-atom interactions. Science, 292(5518):902--905, 2001. [26] Zhangjin Chen, Toru Morishita, Anh-Thu Le, and C. D. Lin. Analysis of twodimensional high-energy photoelectron momentum distributions in the single ionization of atoms by intense laser pulses. Physical Review A, 76(4):043402, 2007. [27] Shih-I. Chu and Dmitry A. Telnov. Beyond the floquet theorem: generalized floquet formalisms and quasienergy methods for atomic and molecular multiphoton processes in intense laser fields. Physics Reports, 390(1-2):1--131, 2004. [28] X. M. Tong and S. I. Chu. Theoretical study of multiple high-order harmonic generation by intense ultrashort pulsed laser fields: A new generalized pseudospectral time-dependent method. Chemical Physics, 217(2-3):119--130, 1997. [29] Jeffrey L. Krause, Kenneth J. Schafer, and Kenneth C. Kulander. Calculation of photoemission from atoms subject to intense laser fields. Physical Review A, 45(7): 4998, 1992. [30] G. H. Yao and S. I. Chu. Generalized pseudospectral methods with mappings for bound and resonance state problems. Chemical Physics Letters, 204(3-4):381--388, 1993. [31] D. A. Telnov and S. I. Chu. Multiphoton detachment of h- near the one-photon threshold: Exterior complex-scaling-generalized pseudospectral method for complex quasienergy resonances. Physical Review A, 59(4):2864--2874, 1999. [32] J. Y. Wang, S. I. Chu, and C. Laughlin. Multiphoton detachment of h- .2. intensitydependent photodetachment rates and threshold behavior - complex-scaling generalized pseudospectral method. Physical Review A, 50(4):3208--3215, 1994. [33] M. R. Hermann and J. A. Fleck. Split-operator spectral method for solving the timedependent schrodinger-equation in spherical coordinates. Physical Review A, 38(12): 6000--6012, 1988. [34] Xiao-Min Tong and Shih-I. Chu. Time-dependent approach to high-resolution spectroscopy and quantum dynamics of rydberg atoms in crossed magnetic and electric fields. Physical Review A, 61(3):031401, 2000. [35] Juan J. Carrera, X. M. Tong, and Shih-I. Chu. Creation and control of a single coherent attosecond xuv pulse by few-cycle intense laser pulses. Physical Review A, 74(2):023404, 2006. [36] Juan J. Carrera and Shih-I. Chu. Extension of high-order harmonic generation cutoff via coherent control of intense few-cycle chirped laser pulses. Physical Review A, 75(3):033807, 2007. [37] X. Chu, S. I. Chu, and C. Laughlin. Spectral and temporal structures of high-order harmonic generation of na in intense mid-ir laser fields. Physical Review A, 6401(1):- -, 2001. [38] D. A. Telnov and S. I. Chu. Ab initio study of the orientation effects in multiphoton ionization and high-order harmonic generation from the ground and excited electronic states of h(2)(+). Physical Review A, 76(4), 2007. [39] X. Chu and S. I. Chu. Self-interaction-free time-dependent density-functional theory for molecular processes in strong fields: High-order harmonic generation of h-2 in intense laser fields. Physical Review A, 6302(2):--, 2001. [40] J. Heslar, D. Telnov, and S. I. Chu. High-order-harmonic generation in homonuclear and heteronuclear diatomic molecules: Exploration of multiple orbital contributions. Physical Review A, 83(4), 2011. [41] Shih-I. Chu. Quasienergy formalism for intense field multiphoton ionization of atoms induced by circularly polarized radiation. Chemical Physics Letters, 54(2): 367--372, 1978. [42] B. Sundaram and P. W. Milonni. High-order harmonic-generation - simplified model and relevance of single-atom theories to experiment. Physical Review A, 41(11): 6571--6573, 1990. [43] X. M. Tong and S. I. Chu. Probing the spectral and temporal structures of high-order harmonic generation in intense laser pulses. Physical Review A, 6102(2):--, 2000. [44] Y. Mairesse, A. de Bohan, L. J. Frasinski, H. Merdji, L. C. Dinu, P. Monchicourt, P. Breger, M. Kovacev, R. Taieb, B. Carre, H. G. Muller, P. Agostini, and P. Salieres. Attosecond synchronization of high-harmonic soft x-rays. Science, 302(5650):1540- -1543, 2003. [45] G. Doumy, J. Wheeler, C. Roedig, R. Chirla, P. Agostini, and L. F. DiMauro. Attosecond synchronization of high-order harmonics from midinfrared drivers. Physical Review Letters, 102(9):093002, 2009. [46] Mette Gaarde. Time-frequency representations of high order harmonics. Opt. Express, 8(10):529--536, 2001. [47] James A. Hostetter, Jennifer L. Tate, Kenneth J. Schafer, and Mette B. Gaarde. Semiclassical approaches to below-threshold harmonics. Physical Review A, 82(2): 023401, 2010. 49 [48] Philippe Antoine, Bernard Piraux, and Alfred Maquet. Time profile of harmonics generated by a single atom in a strong electromagnetic field. Physical Review A, 51(3):R1750, 1995. | |
dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/10200 | - |
dc.description.abstract | 在這篇論文中,我們從非微擾的量子力學觀點,研究銫原子在中程紅外強場雷射中產生高次諧波(high-order harmonic generation, HHG)的現象。我們建立了一個和角動量量子數有關的模型勢能,精準地描述了銫原子的電子結構。我們以時變廣義擬譜方法(time-dependent generalized pseudospectral method, TDGPS)有效率且準確地求解了三維的時變薛丁格方程式。
除了預期的奇數高次諧波外,由於銫原子6s與np能階間的強耦合,我們得到的高次諧波頻譜顯示了一些額外的結構。經由傅立業(Fourier)及小波(wavelet)分析,我們更進一步探索了高次諧波的時間與光譜特性。藉此我們可以瞭解在不同能量範圍之高次諧波產生的主要機制,特別是低閾值與近閾值(below- and near-threshold)高次諧波的產生。 | zh_TW |
dc.description.abstract | In this thesis, we present a non-perturbative quantum study of high-order harmonic generation (HHG) of Cesium atoms in intense mid-infrared laser pulses. An accurate angular-momentum--dependent model potential is constructed for the high-precision description of the Cs atom electronic structure. The three-dimensional time-dependent Schr'{o}dinger equation is solved accurately and efficiently by means of the time-dependent generalized pseudospectral (TDGPS) method.
Besides the expected odd harmonics, the calculated HHG spectra show additional structures due to the strong $6s-np$ couplings. The spectral and temporal characteristics of the HHG are further explored through Fourier and the wavelet transformation. As a result, we can investigate the prevailing mechanisms in different energy regimes, especially those contributing to the generation of below- and near-threshold harmonics. | en |
dc.description.provenance | Made available in DSpace on 2021-05-20T21:09:29Z (GMT). No. of bitstreams: 1 ntu-100-R98222033-1.pdf: 2080908 bytes, checksum: 7d70c399927810126c2125de12c8f8f3 (MD5) Previous issue date: 2011 | en |
dc.description.tableofcontents | 中文摘要i
Abstract ii 謝辭iii Contents iv List of Figures vi List of Tables viii 1 Introduction 1 1.1 Strong field physics . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 1 1.2 Fundamentals of HHG . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 1.3 HHG mechanisms in two extremes . . . . . . . . . . . . . . . . . . . . . 3 1.4 Below- and near-threshold harmonics . . . . . . . . . . . . . . . . . . . 8 1.5 Cesium in the mid-infrared laser pulses . . . . . . . . . . . . . . . . . . 8 2 Numerical Methods 10 2.1 Difficulties in solving the HHG problem . . . . . . . . . . . . . . . . . . 10 2.2 The Time-dependent Schrödinger equation . . . . . . . . . . . . . . . . . 11 2.3 Angular-momentum--dependent model potential for Cesium . . . . . . . 12 2.4 Time-dependent generalized pseudospectral method . . . . . . . . . . . . 14 2.5 Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17 3 Results and Discussions 18 3.1 Laser characteristics and quantum dynamics . . . . . . . . . . . . . . . . 18 3.2 Fourier analysis: spectral properties of HHG . . . . . . . . . . . . . . . . 25 3.3 Fourier analysis: temporal properties of the HHG . . . . . . . . . . . . . 31 3.4 Wavelet analysis: spectral and temporal properties of the HHG . . . . . . 34 3.5 Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 39 4 Conclusions and Future Perspectives 41 Bibliography 43 | |
dc.language.iso | en | |
dc.title | 銫原子在中程紅外強場雷射中產生低閾值與近閾值高次諧波機制之探究 | zh_TW |
dc.title | Exploration of the Mechanisms for Below- and Near-Threshold High-Order Harmonic Generation of Cesium Atoms in Intense Mid-Infrared Laser Fields | en |
dc.type | Thesis | |
dc.date.schoolyear | 99-2 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 孔慶昌,鄭王曜,管希聖 | |
dc.subject.keyword | 強場雷射,高次諧波,銫,時變廣義擬譜方法, | zh_TW |
dc.subject.keyword | intense laser,high-order harmonic generation,cesium,time-dependent generalized pseudospectral method, | en |
dc.relation.page | 50 | |
dc.rights.note | 同意授權(全球公開) | |
dc.date.accepted | 2011-08-20 | |
dc.contributor.author-college | 理學院 | zh_TW |
dc.contributor.author-dept | 物理研究所 | zh_TW |
顯示於系所單位: | 物理學系 |
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