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完整後設資料紀錄
DC 欄位 | 值 | 語言 |
---|---|---|
dc.contributor.advisor | 吳章甫(Chang-Fu Wu) | |
dc.contributor.author | Wei-Cheng Tsai | en |
dc.contributor.author | 蔡瑋珹 | zh_TW |
dc.date.accessioned | 2021-06-16T23:41:01Z | - |
dc.date.available | 2020-03-12 | |
dc.date.copyright | 2020-03-12 | |
dc.date.issued | 2020 | |
dc.date.submitted | 2020-02-18 | |
dc.identifier.citation | Andreae, M. O., and Gelencsér, A. (2006). Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols. Atmos. Chem. Phys., 6(10), 3131-3148.
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Z., and Schauer, J. J. (2006). Composition and sources of carbonaceous aerosols at three contrasting sites in Hong Kong. Journal of Geophysical Research: Atmospheres, 111(D20). Zielinska, B., Sagebiel, J., McDonald, J. D., Whitney, K., and Lawson, D. R. (2004). Emission rates and comparative chemical composition from selected in-use diesel and gasoline-fueled vehicles. J Air Waste Manag Assoc, 54(9), 1138-1150. 吳欣育. (2018). 利用受體模式評估都會區細懸浮微粒上多環芳香烴濃度與來源貢獻垂直分布. 臺灣大學, Available from Airiti AiritiLibrary database. (2018年) 郭承彬, 馮立婷, 曹永杰, 張寶額, and 吳章甫. (2012). 應用絕對主成分分析於開徑式傅立葉轉換紅外光光譜儀監測資料以探討異味物質氨之排放污染源. [Application of APCA for Investigation of Odor Emission Sources of Ammonia with OP-FTIR Monitoring Data]. 勞工安全衛生研究季刊, 20(4), 499-511. 羅紹齊. (2014). 餐飲業細懸浮微粒排放與化學成份分析. 朝陽科技大學, Available from Airiti AiritiLibrary database. (2014年) | |
dc.identifier.uri | http://tdr.lib.ntu.edu.tw/jspui/handle/123456789/65405 | - |
dc.description.abstract | 空氣污染在近年已經逐漸被視為重要議題。許多研究已經探討附著於空氣中細懸浮微粒(Particulate matters, PM2.5)上的非極性有機物質(Nonpolar organic compounds, NPOCs)。都市內有許多人居住在大樓內,但是暴露於空氣污染物的垂直面變化仍需要進一步的探討。本研究於2018年10月至2019年1月在臺北市區內的一棟大樓三個不同樓層(低、中、高樓層)的陽台架設採樣點。每週兩次於所有採樣點同時在石英纖維濾紙上採集二十四小時的PM2.5樣本,總共採集72個樣本。本研究分析的非極性有機物質包含24種Polycyclic aromatic hydrocarbons (PAHs)、16種Hopanes、12種Steranes、23種Alkanes、10種iso-/anteiso-alkanes,使用熱脫附氣相層析質譜法 (TD–GC/MS)分析並量化這些化學物質。為了瞭解這些污染物質的來源,本研究回顧這些有機物質來源之文獻,並搭配主成分分析(Principal component analysis, PCA)作為受體模式解析污染源。
大氣中濃度最高的有機物質族群在本研究中為Alkanes(10.08±4.51 ng/m3),而具有致癌風險的PAHs的濃度則為0.70±0.59 ng/m3,占所有分析的非極性有機物濃度5%。在垂直面上,Alkanes在中樓層有最高濃度,然而PAHs、Hopanes、Steranes和iso-/anteiso-alkanes濃度則隨著樓層升高而遞減。主成分分析結果顯示主要影響採樣點的污染源為多種石化燃燒活動(交通燃燒排放、天然氣燃燒等)和交通相關的揚塵。關於PAHs的風險估計,採樣期間平均致癌風險為1.46*10-6,比美國環保署建議的暴露風險標準10-6還要高。這項研究探討臺北市內附著在PM 2.5的非極性有機物質濃度變化。了解污染物於大氣中的濃度分布情況與潛在貢獻來源將有助於設計有效的控制策略。 | zh_TW |
dc.description.provenance | Made available in DSpace on 2021-06-16T23:41:01Z (GMT). No. of bitstreams: 1 ntu-109-R06844003-1.pdf: 2380690 bytes, checksum: b5151b4de76660fd8890eab181612491 (MD5) Previous issue date: 2020 | en |
dc.description.tableofcontents | 致謝 ii
中文摘要 iii 英文摘要 iv 目錄 v 表次 vi 圖次 vii Chapter 1 介紹 1 Chapter 2 本研究分析物質的環境意義文獻回顧 5 2.1 PAHs 5 2.2 Hopanes、Steranes 5 2.3 Alkanes 6 2.4 支鏈烷烴類 6 Chapter 3 材料與方法 8 3.1 研究地區 8 3.2 採樣策略 8 3.2.1 採樣地點 8 3.2.2 採樣方法 9 3.3 化學物質分析 9 3.4 污染源解析 10 3.4.1定性污染源與資料前處理 11 3.5 PAHs風險估計 12 Chapter 4 結果與討論 14 4.1非極性有機物質濃度分布與探討 14 4.1.1 PAHs 14 4.1.2 Hopanes、Steranes 15 4.1.3 Alkanes 15 4.1.4 iso-/anteiso-alkanes 15 4.2 主成分分析結果與討論 16 4.3 各種類物質於垂直面濃度分布 18 4.4 PAHs風險估計 19 4.4.1 PAHs濃度風險估計與比較 19 4.4.2 濃度風險低估限制 19 4.5 PAHs揮發性與降解討論 20 4.6 研究限制 22 Chapter 5 結論與展望 23 Chapter 6 參考文獻 39 Chapter 7 附錄 48 附錄1. 放入主成分分析物質之雜訊比 48 附錄2. 主成分分析因素結構負荷量 49 附錄3. 非極性有機物質之族群濃度時序性分布圖 51 附錄4. 本研究分析非極性有機物質之環境意義、來源文獻回顧 53 | |
dc.language.iso | zh-TW | |
dc.title | 探討都市中細懸浮微粒上非極性有機物質濃度分布與污染源解析 | zh_TW |
dc.title | Evaluating the concentration distribution and source apportionment of non-polar organic compounds on fine particulate matter in an urban area | en |
dc.type | Thesis | |
dc.date.schoolyear | 108-1 | |
dc.description.degree | 碩士 | |
dc.contributor.oralexamcommittee | 蔡詩偉(Shih-Wei Tsai),陳志傑(Chih-Chieh Chen) | |
dc.subject.keyword | 細懸浮微粒(PM2.5)上的非極性有機物質(NPOC),源解析,主成分分析(PCA),PAHs風險估計, | zh_TW |
dc.subject.keyword | non-polar organic compounds(NPOC) for fine particulate matters(PM2.5),source apportionment,principal component analysis(PCA),risk estimate of PAHs, | en |
dc.relation.page | 59 | |
dc.identifier.doi | 10.6342/NTU202000513 | |
dc.rights.note | 有償授權 | |
dc.date.accepted | 2020-02-19 | |
dc.contributor.author-college | 公共衛生學院 | zh_TW |
dc.contributor.author-dept | 環境與職業健康科學研究所 | zh_TW |
顯示於系所單位: | 環境與職業健康科學研究所 |
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